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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 15, issue 1
Atmos. Chem. Phys., 15, 537-561, 2015
https://doi.org/10.5194/acp-15-537-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 15, 537-561, 2015
https://doi.org/10.5194/acp-15-537-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 15 Jan 2015

Research article | 15 Jan 2015

Modeling dust as component minerals in the Community Atmosphere Model: development of framework and impact on radiative forcing

R. A. Scanza1, N. Mahowald1, S. Ghan2, C. S. Zender3, J. F. Kok4, X. Liu2,5, Y. Zhang1,6, and S. Albani1 R. A. Scanza et al.
  • 1Department of Earth and Atmospheric Sciences, Cornell University, Ithaca, New York, USA
  • 2Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland, Washington, USA
  • 3Department of Earth System Science, University of California, Irvine, USA
  • 4Department of Atmospheric and Oceanic Sciences, University of California, Los Angeles, USA
  • 5Department of Atmospheric Science, University of Wyoming, Laramie, Wyoming, USA
  • 6Department of Environmental Science and Engineering, Fudan University, Shanghai, China

Abstract. The mineralogy of desert dust is important due to its effect on radiation, clouds and biogeochemical cycling of trace nutrients. This study presents the simulation of dust radiative forcing as a function of both mineral composition and size at the global scale, using mineral soil maps for estimating emissions. Externally mixed mineral aerosols in the bulk aerosol module in the Community Atmosphere Model version 4 (CAM4) and internally mixed mineral aerosols in the modal aerosol module in the Community Atmosphere Model version 5.1 (CAM5) embedded in the Community Earth System Model version 1.0.5 (CESM) are speciated into common mineral components in place of total dust. The simulations with mineralogy are compared to available observations of mineral atmospheric distribution and deposition along with observations of clear-sky radiative forcing efficiency. Based on these simulations, we estimate the all-sky direct radiative forcing at the top of the atmosphere as + 0.05 Wm−2 for both CAM4 and CAM5 simulations with mineralogy. We compare this to the radiative forcing from simulations of dust in release versions of CAM4 and CAM5 (+0.08 and +0.17 Wm−2) and of dust with optimized optical properties, wet scavenging and particle size distribution in CAM4 and CAM5, −0.05 and −0.17 Wm−2, respectively. The ability to correctly include the mineralogy of dust in climate models is hindered by its spatial and temporal variability as well as insufficient global in situ observations, incomplete and uncertain source mineralogies and the uncertainties associated with data retrieved from remote sensing methods.

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The main purpose of this study was to build a framework in the Community Atmosphere Models version 4 and 5 within the Community Earth System Model to simulate dust aerosols as their component minerals. With this framework, we investigate the direct radiative forcing that results from the mineral speciation. We find that adding mineralogy results in a small positive forcing at the top of the atmosphere, while simulations without mineralogy have a small negative forcing.
The main purpose of this study was to build a framework in the Community Atmosphere Models...
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