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Volume 15, issue 6
Atmos. Chem. Phys., 15, 3217–3239, 2015
https://doi.org/10.5194/acp-15-3217-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 15, 3217–3239, 2015
https://doi.org/10.5194/acp-15-3217-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 23 Mar 2015

Research article | 23 Mar 2015

Seasonal changes in the tropospheric carbon monoxide profile over the remote Southern Hemisphere evaluated using multi-model simulations and aircraft observations

J. A. Fisher et al.
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Achakulwisut, P., Mickley, L. J., Murray, L. T., Tai, A. P. K., Kaplan, J. O., and Alexander, B.: Uncertainties in isoprene photochemistry and emissions: implications for the oxidative capacity of past and present atmospheres and for trends in climate forcing agents, Atmos. Chem. Phys. Discuss., 15, 2197–2246, https://doi.org/10.5194/acpd-15-2197-2015, 2015.
Archibald, A., Jenkin, M., and Shallcross, D.: An isoprene mechanism intercomparison, Atmos. Environ., 44, 5356–5364, 2010.
Arneth, A., Miller, P. A., Scholze, M., Hickler, T., Schurgers, G., Smith, B., and Prentice, I. C.: CO2 inhibition of global terrestrial isoprene emissions: potential implications for atmospheric chemistry, Geophys. Res. Lett., 34, L18813, https://doi.org/10.1029/2007GL030615, 2007a.
Arneth, A., Niinemets, Ü., Pressley, S., Bäck, J., Hari, P., Karl, T., Noe, S., Prentice, I. C., Serça, D., Hickler, T., Wolf, A., and Smith, B.: Process-based estimates of terrestrial ecosystem isoprene emissions: incorporating the effects of a direct CO2-isoprene interaction, Atmos. Chem. Phys., 7, 31–53, https://doi.org/10.5194/acp-7-31-2007, 2007b.
Bates, K. H., Crounse, J. D., St. Clair, J. M., Bennett, N. B., Nguyen, T. B., Seinfeld, J. H., Stoltz, B. M., and Wennberg, P. O.: Gas phase production and loss of isoprene epoxydiols, J. Phys. Chem. A, 118, 1237–1246, 2014.
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The Southern Hemisphere (SH) serves as an important test bed for evaluating our understanding of the processes that drive the composition of the clean background atmosphere. Using data from two aircraft campaigns, combined with four atmospheric chemistry models, we find a large sensitivity in the remote SH to biogenic emissions and their subsequent chemistry and transport. Future model evaluation and measurement campaigns should prioritize reducing uncertainties in these processes.
The Southern Hemisphere (SH) serves as an important test bed for evaluating our understanding of...
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