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Volume 15, issue 20
Atmos. Chem. Phys., 15, 11461–11476, 2015
https://doi.org/10.5194/acp-15-11461-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 15, 11461–11476, 2015
https://doi.org/10.5194/acp-15-11461-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 16 Oct 2015

Research article | 16 Oct 2015

The impacts of volcanic aerosol on stratospheric ozone and the Northern Hemisphere polar vortex: separating radiative-dynamical changes from direct effects due to enhanced aerosol heterogeneous chemistry

S. Muthers2,1, F. Arfeuille3, C. C. Raible2,1, and E. Rozanov4,5 S. Muthers et al.
  • 1Climate and Environmental Physics, University of Bern, Bern, Switzerland
  • 2Oeschger Centre for Climate Change Research, University of Bern, Bern, Switzerland
  • 3Suisse Federal Laboratories for Material Science and Technology (Empa) Duebendorf, Switzerland
  • 4Institute for Atmospheric and Climate Science, ETH, Zurich, Switzerland
  • 5Physikalisch-Meteorologisches Observatorium Davos and World Radiation Center (PMOD/WRC), Davos, Switzerland

Abstract. After major volcanic eruptions the enhanced aerosol causes ozone changes due to greater heterogeneous chemistry on the particle surfaces (HET-AER) and from dynamical effects related to the radiative heating of the lower stratosphere (RAD-DYN). We carry out a series of experiments with an atmosphere–ocean–chemistry–climate model to assess how these two processes change stratospheric ozone and Northern Hemispheric (NH) polar vortex dynamics. Ensemble simulations are performed under present day and preindustrial conditions, and with aerosol forcings representative of different eruption strength, to investigate changes in the response behaviour. We show that the halogen component of the HET-AER effect dominates under present-day conditions with a global reduction of ozone (−21 DU for the strongest eruption) particularly at high latitudes, whereas the HET-AER effect increases stratospheric ozone due to N2O5 hydrolysis in a preindustrial atmosphere (maximum anomalies +4 DU). The halogen-induced ozone changes in the present-day atmosphere offset part of the strengthening of the NH polar vortex during mid-winter (reduction of up to −16 m s-1 in January) and slightly amplify the dynamical changes in the polar stratosphere in late winter (+11 m s-1 in March). The RAD-DYN mechanism leads to positive column ozone anomalies which are reduced in a present-day atmosphere by amplified polar ozone depletion (maximum anomalies +12 and +18 DU for present day and preindustrial, respectively). For preindustrial conditions, the ozone response is consequently dominated by RAD-DYN processes, while under present-day conditions, HET-AER effects dominate. The dynamical response of the stratosphere is dominated by the RAD-DYN mechanism showing an intensification of the NH polar vortex in winter (up to +10 m s-1 in January). Ozone changes due to the RAD-DYN mechanism slightly reduce the response of the polar vortex after the eruption under present-day conditions.

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After volcanic eruptions different radiative and chemical processes take place in the stratosphere which perturb the ozone layer and cause pronounced dynamical changes. In idealized chemistry-climate model simulations the importance of these processes and the modulating role of the climate state is analysed. The chemical effect strongly differs between a preindustrial and present-day climate, but the effect on the dynamics is weak. Radiative processes dominate the dynamics in all climate states.
After volcanic eruptions different radiative and chemical processes take place in the...
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