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Volume 15, issue 1 | Copyright

Special issue: Monitoring atmospheric composition and climate, research in...

Atmos. Chem. Phys., 15, 113-133, 2015
https://doi.org/10.5194/acp-15-113-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 09 Jan 2015

Research article | 09 Jan 2015

Inverse modelling of CH4 emissions for 2010–2011 using different satellite retrieval products from GOSAT and SCIAMACHY

M. Alexe1, P. Bergamaschi1, A. Segers2, R. Detmers3, A. Butz9, O. Hasekamp3, S. Guerlet3, R. Parker4, H. Boesch4, C. Frankenberg5, R. A. Scheepmaker3, E. Dlugokencky6, C. Sweeney7,6, S. C. Wofsy8, and E. A. Kort10 M. Alexe et al.
  • 1European Commission, Joint Research Centre, Institute for Environment and Sustainability, Air and Climate Unit, Ispra, Italy
  • 2Netherlands Organisation for Applied Scientific Research (TNO), Utrecht, the Netherlands
  • 3Netherlands Institute for Space Research (SRON), Utrecht, the Netherlands
  • 4Earth Observation Science Group, Space Research Centre, University of Leicester, Leicester, UK
  • 5Jet Propulsion Laboratory, California Institute of Technology, Pasadena, California, USA
  • 6Global Monitoring Division, NOAA Earth System Research Laboratory, Boulder, Colorado, USA
  • 7CIRES, University of Colorado, Boulder, Colorado, USA
  • 8School of Engineering and Applied Science and Department of Earth and Planetary Sciences, Harvard University, Cambridge, Massachusetts, USA
  • 9Karlsruhe Institute of Technology (KIT), Karlsruhe, Germany
  • 10Department of Atmospheric, Oceanic and Space Sciences, University of Michigan, Michigan, USA

Abstract. At the beginning of 2009 new space-borne observations of dry-air column-averaged mole fractions of atmospheric methane (XCH4) became available from the Thermal And Near infrared Sensor for carbon Observations–Fourier Transform Spectrometer (TANSO-FTS) instrument on board the Greenhouse Gases Observing SATellite (GOSAT). Until April 2012 concurrent {methane (CH4) retrievals} were provided by the SCanning Imaging Absorption spectroMeter for Atmospheric CartograpHY (SCIAMACHY) instrument on board the ENVironmental SATellite (ENVISAT). The GOSAT and SCIAMACHY XCH4 retrievals can be compared during the period of overlap. We estimate monthly average CH4 emissions between January 2010 and December 2011, using the TM5-4DVAR inverse modelling system. In addition to satellite data, high-accuracy measurements from the Cooperative Air Sampling Network of the National Oceanic and Atmospheric Administration Earth System Research Laboratory (NOAA ESRL) are used, providing strong constraints on the remote surface atmosphere. We discuss five inversion scenarios that make use of different GOSAT and SCIAMACHY XCH4 retrieval products, including two sets of GOSAT proxy retrievals processed independently by the Netherlands Institute for Space Research (SRON)/Karlsruhe Institute of Technology (KIT), and the University of Leicester (UL), and the RemoTeC "Full-Physics" (FP) XCH4 retrievals available from SRON/KIT. The GOSAT-based inversions show significant reductions in the root mean square (rms) difference between retrieved and modelled XCH4, and require much smaller bias corrections compared to the inversion using SCIAMACHY retrievals, reflecting the higher precision and relative accuracy of the GOSAT XCH4. Despite the large differences between the GOSAT and SCIAMACHY retrievals, 2-year average emission maps show overall good agreement among all satellite-based inversions, with consistent flux adjustment patterns, particularly across equatorial Africa and North America. Over North America, the satellite inversions result in a significant redistribution of CH4 emissions from North-East to South-Central United States. This result is consistent with recent independent studies suggesting a systematic underestimation of CH4 emissions from North American fossil fuel sources in bottom-up inventories, likely related to natural gas production facilities. Furthermore, all four satellite inversions yield lower CH4 fluxes across the Congo basin compared to the NOAA-only scenario, but higher emissions across tropical East Africa. The GOSAT and SCIAMACHY inversions show similar performance when validated against independent shipboard and aircraft observations, and XCH4 retrievals available from the Total Carbon Column Observing Network (TCCON).

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