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Volume 15, issue 19
Atmos. Chem. Phys., 15, 11133-11145, 2015
https://doi.org/10.5194/acp-15-11133-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 15, 11133-11145, 2015
https://doi.org/10.5194/acp-15-11133-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 07 Oct 2015

Research article | 07 Oct 2015

On the statistical optimality of CO2 atmospheric inversions assimilating CO2 column retrievals

F. Chevallier F. Chevallier
  • Laboratoire des Sciences du Climat et de l'Environnement, CEA-CNRS-UVSQ, L'Orme des Merisiers, Bat 701, 91191 Gif-sur-Yvette, France

Abstract. The extending archive of the Greenhouse Gases Observing Satellite (GOSAT) measurements (now covering about 6 years) allows increasingly robust statistics to be computed, that document the performance of the corresponding retrievals of the column-average dry air-mole fraction of CO2 (XCO2). Here, we demonstrate that atmospheric inversions cannot be rigorously optimal when assimilating current XCO2 retrievals, even with averaging kernels, in particular because retrievals and inversions use different assumption about prior uncertainty. We look for some practical evidence of this sub-optimality from the view point of atmospheric inversion by comparing a model simulation constrained by surface air-sample measurements with one of the GOSAT retrieval products (NASA's ACOS). The retrieval-minus-model differences result from various error sources, both in the retrievals and in the simulation: we discuss the plausibility of the origin of the major patterns. We find systematic retrieval errors over the dark surfaces of high-latitude lands and over African savannahs. More importantly, we also find a systematic over-fit of the GOSAT radiances by the retrievals over land for the high-gain detector mode, which is the usual observation mode. The over-fit is partially compensated by the retrieval bias-correction. These issues are likely common to other retrieval products and may explain some of the surprising and inconsistent CO2 atmospheric inversion results obtained with the existing GOSAT retrieval products. We suggest that reducing the observation weight in the retrieval schemes (for instance so that retrieval increments to the retrieval prior values are halved for the studied retrieval product) would significantly improve the retrieval quality and reduce the need for (or at least reduce the complexity of) ad-hoc retrieval bias correction.

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Short summary
We demonstrate that the current two-step approach to infer the CO2 surface fluxes from satellite measured radiances, with CO2 retrievals as an intermediate product, is not optimal. This suboptimality corrupts the 4D information flow from the radiance measurements to the surface flux estimates. It is amplified by current retrieval strategies where prior errors are much larger than the performance of prior CO2 simulations used in atmospheric inversions.
We demonstrate that the current two-step approach to infer the CO2 surface fluxes from satellite...
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