Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 15, 11117-11132, 2015
https://doi.org/10.5194/acp-15-11117-2015
© Author(s) 2015. This work is distributed under
the Creative Commons Attribution 3.0 License.
Research article
06 Oct 2015
Retrieving microphysical properties of dust-like particles using ellipsoids: the case of refractive index
O. Kemppinen1,2, T. Nousiainen1, S. Merikallio1, and P. Räisänen1 1Earth Observation, Finnish Meteorological Institute, Helsinki, Finland
2Department of Applied Physics, Aalto University, Espoo, Finland
Abstract. Distributions of ellipsoids are often used to simulate the optical properties of non-ellipsoidal atmospheric particles, such as dust. In this work, the applicability of ellipsoids for retrieving the refractive index of dust-like target model particles from scattering data is investigated. This is a pure modeling study, in which stereogrammetrically retrieved model dust shapes are used as targets. The primary objective is to study whether the refractive index of these target particles can be inverted from their scattering matrices using ellipsoidal model particles. To achieve this, first scattering matrices for the target model particles with known refractive indices are computed. First, a non-negative least squares fitting is performed, individually for each scattering matrix element, for 46 differently shaped ellipsoids by using different assumed refractive indices. Then, the fitting error is evaluated to establish whether the ellipsoid ensemble best matches the target scattering matrix elements when the correct refractive index is assumed. Second, we test whether the ellipsoids best match the target data with the correct refractive index, when a predefined (uniform) shape distribution for ellipsoids is assumed, instead of optimizing the shape distribution separately for each tested refractive index. The results show not only that for both of these approaches using ellipsoids with the true refractive index produces good results but also that for each scattering matrix element even better results are acquired by using wrong refractive indices. In addition, the best agreement is obtained for different scattering matrix elements using different refractive indices. The findings imply that retrieval of refractive index of non-ellipsoidal particles whose single-scattering properties have been modeled with ellipsoids may not be reliable. Furthermore, it is demonstrated that the differences in single-scattering albedo and asymmetry parameter between the best-match ellipsoid ensemble and the target particles may give rise to major differences in simulated aerosol radiative effects.

Citation: Kemppinen, O., Nousiainen, T., Merikallio, S., and Räisänen, P.: Retrieving microphysical properties of dust-like particles using ellipsoids: the case of refractive index, Atmos. Chem. Phys., 15, 11117-11132, https://doi.org/10.5194/acp-15-11117-2015, 2015.
Publications Copernicus
Short summary
Combinations of simple mathematical model shapes called ellipsoids are used in many remote sensing and modeling applications to denote dust particles. In this study we investigate how accurately various physical parameters can be retrieved by using ellipsoids. The results show that using ellipsoids can lead to wrong results, while at the same time seeming like they work well. This means that extreme care should be used when using ellipsoids for dust, and extra validation measures should be used.
Combinations of simple mathematical model shapes called ellipsoids are used in many remote...
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