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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 14, issue 15
Atmos. Chem. Phys., 14, 7721-7739, 2014
https://doi.org/10.5194/acp-14-7721-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 14, 7721-7739, 2014
https://doi.org/10.5194/acp-14-7721-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 04 Aug 2014

Research article | 04 Aug 2014

Skill in forecasting extreme ozone pollution episodes with a global atmospheric chemistry model

J. L. Schnell1, C. D. Holmes1, A. Jangam1,*, and M. J. Prather1 J. L. Schnell et al.
  • 1Department of Earth System Science, University of California, Irvine, CA 92697-3100, USA
  • *now at: Department of Integrated Environmental Science, Bethune-Cookman University, Daytona Beach, FL, USA

Abstract. From the ensemble of stations that monitor surface air quality over the United States and Europe, we identify extreme ozone pollution events and find that they occur predominantly in clustered, multiday episodes with spatial extents of more than 1000 km. Such scales are amenable to forecasting with current global atmospheric chemistry models. We develop an objective mapping algorithm that uses the heterogeneous observations of the individual surface sites to calculate surface ozone averaged over 1° by 1° grid cells, matching the resolution of a global model. Air quality extreme (AQX) events are identified locally as statistical extremes of the ozone climatology and not as air quality exceedances. With the University of California, Irvine chemistry-transport model (UCI CTM) we find there is skill in hindcasting these extreme episodes, and thus identify a new diagnostic using global chemistry–climate models (CCMs) to identify changes in the characteristics of extreme pollution episodes in a warming climate.

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