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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 14, issue 14
Atmos. Chem. Phys., 14, 7681-7692, 2014
https://doi.org/10.5194/acp-14-7681-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 14, 7681-7692, 2014
https://doi.org/10.5194/acp-14-7681-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 31 Jul 2014

Research article | 31 Jul 2014

Variability of NOx in the polar middle atmosphere from October 2003 to March 2004: vertical transport vs. local production by energetic particles

M. Sinnhuber1, B. Funke2, T. von Clarmann1, M. Lopez-Puertas2, G. P. Stiller1, and A. Seppälä3 M. Sinnhuber et al.
  • 1Karlsruhe Institute of Technology, Institute for Meteorology and Climate Research, Karlsruhe, Germany
  • 2Instituto de Astrofìsica de Andalucìa, CSIC, Granada, Spain
  • 3Finish Meteorological Institute FMI, Helsinki, Finland

Abstract. We use NO, NO2 and CO from MIPAS/ENVISAT to investigate the impact of energetic particle precipitation onto the NOx budget from the stratosphere to the lower mesosphere in the period from October 2003 to March 2004, a time of high solar and geomagnetic activity. We find that in the winter hemisphere the indirect effect of auroral electron precipitation due to downwelling of upper mesospheric/lower thermospheric air into the stratosphere prevails. Its effect exceeds even the direct impact of the very large solar proton event in October/November 2003 by nearly 1 order of magnitude. Correlations of NOx and CO show that the unprecedented high NOx values observed in the Northern Hemisphere lower mesosphere and upper stratosphere in late January and early February are fully consistent with transport from the upper mesosphere/lower thermosphere and subsequent mixing at lower altitudes. In the polar summer Southern Hemisphere, we observed an enhanced variability of NO and NO2 on days with enhanced geomagnetic activity, but this seems to indicate enhanced instrument noise rather than a direct increase due to electron precipitation. A direct effect of electron precipitation onto NOx can not be ruled out, but, if any, it is lower than 3 ppbv in the altitude range 40–56 km and lower than 6 ppbv in the altitude range 56–64 km. An additional significant source of NOx due to local production by precipitating electrons below 70 km exceeding several parts per billion as discussed in previous publications appears unlikely.

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