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Volume 14, issue 4 | Copyright

Special issue: BACCHUS – Impact of Biogenic versus Anthropogenic emissions...

Atmos. Chem. Phys., 14, 1837-1852, 2014
https://doi.org/10.5194/acp-14-1837-2014
© Author(s) 2014. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 17 Feb 2014

Research article | 17 Feb 2014

A sea spray aerosol flux parameterization encapsulating wave state

J. Ovadnevaite1, A. Manders2, G. de Leeuw2,3,4, D. Ceburnis1, C. Monahan1, A.-I. Partanen5, H. Korhonen5, and C. D. O'Dowd1 J. Ovadnevaite et al.
  • 1School of Physics and Centre for Climate and Air Pollution Studies, Ryan Institute, National University of Ireland Galway, University Road, Galway, Ireland
  • 2TNO, Utrecht, The Netherlands
  • 3Finnish Meteorological Institute (FMI), Climate Change Unit, Helsinki, Finland
  • 4Department of Physics, University of Helsinki, Finland
  • 5Kuopio Unit, Finnish Meteorological Institute, Kuopio, Finland

Abstract. A new sea spray source function (SSSF), termed Oceanflux Sea Spray Aerosol or OSSA, was derived based on in-situ sea spray aerosol measurements along with meteorological/physical parameters. Submicron sea spray aerosol fluxes derived from particle number concentration measurements at the Mace Head coastal station, on the west coast of Ireland, were used together with open-ocean eddy correlation flux measurements from the Eastern Atlantic Sea Spray, Gas Flux, and Whitecap (SEASAW) project cruise. In the overlapping size range, the data for Mace Head and SEASAW were found to be in a good agreement, which allowed deriving the new SSSF from the combined dataset spanning the dry diameter range from 15 nm to 6 μm. The OSSA source function has been parameterized in terms of five lognormal modes and the Reynolds number instead of the more commonly used wind speed, thereby encapsulating important influences of wave height, wind history, friction velocity, and viscosity. This formulation accounts for the different flux relationships associated with rising and waning wind speeds since these are included in the Reynolds number. Furthermore, the Reynolds number incorporates the kinematic viscosity of water, thus the SSSF inherently includes dependences on sea surface temperature and salinity. The temperature dependence of the resulting SSSF is similar to that of other in-situ derived source functions and results in lower production fluxes for cold waters and enhanced fluxes from warm waters as compared with SSSF formulations that do not include temperature effects.

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