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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 13, issue 17
Atmos. Chem. Phys., 13, 8787-8796, 2013
https://doi.org/10.5194/acp-13-8787-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.
Atmos. Chem. Phys., 13, 8787-8796, 2013
https://doi.org/10.5194/acp-13-8787-2013
© Author(s) 2013. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 03 Sep 2013

Research article | 03 Sep 2013

Gravitational separation in the stratosphere – a new indicator of atmospheric circulation

S. Ishidoya1, S. Sugawara2, S. Morimoto3, S. Aoki4, T. Nakazawa4, H. Honda5, and S. Murayama1 S. Ishidoya et al.
  • 1National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba 305-8569, Japan
  • 2Miyagi University of Education, Sendai 980-0845, Japan
  • 3National Institute of Polar Research, Tokyo 190-8518, Japan
  • 4Center for Atmospheric and Oceanic Studies, Tohoku University, Sendai 980-8578, Japan
  • 5Institute of Space and Astronautical Science (ISAS), Japan Aerospace Exploration Agency (JAXA), Sagamihara 252-5210, Japan

Abstract. As a basic understanding of the dynamics of the atmospheric circulation, it has been believed that gravitational separation of atmospheric components is observable only in the atmosphere above the turbopause. However, we found, from our high-precision measurements of not only the isotopic ratios of N2, O2 and Ar but also the mole fraction of Ar, that gravitational separation occurs even in the stratosphere below the turbopause; their observed vertical profiles are in good agreement with those expected theoretically from molecular mass differences. The O2/N2 ratio observed in the middle stratosphere, corrected for gravitational separation, showed the same mean air age as estimated from the CO2 mole fraction. Simulations with a 2-dimensional model of the middle atmosphere indicated that a relationship between gravitational separation and the age of air in the stratosphere would be significantly affected if the Brewer–Dobson circulation was enhanced due to global warming. Therefore, gravitational separation is usable as a new indicator of changes in the atmospheric circulation in the stratosphere.

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