Articles | Volume 13, issue 14
https://doi.org/10.5194/acp-13-6663-2013
https://doi.org/10.5194/acp-13-6663-2013
Research article
 | 
15 Jul 2013
Research article |  | 15 Jul 2013

Kinetic regimes and limiting cases of gas uptake and heterogeneous reactions in atmospheric aerosols and clouds: a general classification scheme

T. Berkemeier, A. J. Huisman, M. Ammann, M. Shiraiwa, T. Koop, and U. Pöschl

Related authors

Desorption lifetimes and activation energies influencing gas–surface interactions and multiphase chemical kinetics
Daniel A. Knopf, Markus Ammann, Thomas Berkemeier, Ulrich Pöschl, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 3445–3528, https://doi.org/10.5194/acp-24-3445-2024,https://doi.org/10.5194/acp-24-3445-2024, 2024
Short summary
Volatile oxidation products and secondary organosiloxane aerosol from D5 + OH at varying OH exposures
Hyun Gu Kang, Yanfang Chen, Yoojin Park, Thomas Berkemeier, and Hwajin Kim
Atmos. Chem. Phys., 23, 14307–14323, https://doi.org/10.5194/acp-23-14307-2023,https://doi.org/10.5194/acp-23-14307-2023, 2023
Short summary
Technical note: In situ measurements and modelling of the oxidation kinetics in films of a cooking aerosol proxy using a quartz crystal microbalance with dissipation monitoring (QCM-D)
Adam Milsom, Shaojun Qi, Ashmi Mishra, Thomas Berkemeier, Zhenyu Zhang, and Christian Pfrang
Atmos. Chem. Phys., 23, 10835–10843, https://doi.org/10.5194/acp-23-10835-2023,https://doi.org/10.5194/acp-23-10835-2023, 2023
Short summary
Accelerating models for multiphase chemical kinetics through machine learning with polynomial chaos expansion and neural networks
Thomas Berkemeier, Matteo Krüger, Aryeh Feinberg, Marcel Müller, Ulrich Pöschl, and Ulrich K. Krieger
Geosci. Model Dev., 16, 2037–2054, https://doi.org/10.5194/gmd-16-2037-2023,https://doi.org/10.5194/gmd-16-2037-2023, 2023
Short summary
Aqueous-phase reactive species formed by fine particulate matter from remote forests and polluted urban air
Haijie Tong, Fobang Liu, Alexander Filippi, Jake Wilson, Andrea M. Arangio, Yun Zhang, Siyao Yue, Steven Lelieveld, Fangxia Shen, Helmi-Marja K. Keskinen, Jing Li, Haoxuan Chen, Ting Zhang, Thorsten Hoffmann, Pingqing Fu, William H. Brune, Tuukka Petäjä, Markku Kulmala, Maosheng Yao, Thomas Berkemeier, Manabu Shiraiwa, and Ulrich Pöschl
Atmos. Chem. Phys., 21, 10439–10455, https://doi.org/10.5194/acp-21-10439-2021,https://doi.org/10.5194/acp-21-10439-2021, 2021
Short summary

Related subject area

Subject: Aerosols | Research Activity: Laboratory Studies | Altitude Range: Troposphere | Science Focus: Chemistry (chemical composition and reactions)
Desorption lifetimes and activation energies influencing gas–surface interactions and multiphase chemical kinetics
Daniel A. Knopf, Markus Ammann, Thomas Berkemeier, Ulrich Pöschl, and Manabu Shiraiwa
Atmos. Chem. Phys., 24, 3445–3528, https://doi.org/10.5194/acp-24-3445-2024,https://doi.org/10.5194/acp-24-3445-2024, 2024
Short summary
Molecular analysis of secondary organic aerosol and brown carbon from the oxidation of indole
Feng Jiang, Kyla Siemens, Claudia Linke, Yanxia Li, Yiwei Gong, Thomas Leisner, Alexander Laskin, and Harald Saathoff
Atmos. Chem. Phys., 24, 2639–2649, https://doi.org/10.5194/acp-24-2639-2024,https://doi.org/10.5194/acp-24-2639-2024, 2024
Short summary
Secondary organic aerosol formed by Euro 5 gasoline vehicle emissions: chemical composition and gas-to-particle phase partitioning
Evangelia Kostenidou, Baptiste Marques, Brice Temime-Roussel, Yao Liu, Boris Vansevenant, Karine Sartelet, and Barbara D'Anna
Atmos. Chem. Phys., 24, 2705–2729, https://doi.org/10.5194/acp-24-2705-2024,https://doi.org/10.5194/acp-24-2705-2024, 2024
Short summary
Assessment of the contribution of residential waste burning to ambient PM10 concentrations in Hungary and Romania
András Hoffer, Aida Meiramova, Ádám Tóth, Beatrix Jancsek-Turóczi, Gyula Kiss, Ágnes Rostási, Erika Andrea Levei, Luminita Marmureanu, Attila Machon, and András Gelencsér
Atmos. Chem. Phys., 24, 1659–1671, https://doi.org/10.5194/acp-24-1659-2024,https://doi.org/10.5194/acp-24-1659-2024, 2024
Short summary
Source differences in the components and cytotoxicity of PM2.5 from automobile exhaust, coal combustion, and biomass burning contributing to urban aerosol toxicity
Xiao-San Luo, Weijie Huang, Guofeng Shen, Yuting Pang, Mingwei Tang, Weijun Li, Zhen Zhao, Hanhan Li, Yaqian Wei, Longjiao Xie, and Tariq Mehmood
Atmos. Chem. Phys., 24, 1345–1360, https://doi.org/10.5194/acp-24-1345-2024,https://doi.org/10.5194/acp-24-1345-2024, 2024
Short summary

Cited articles

Abbatt, J. P. D., Lee, A. K. Y., and Thornton, J. A.: Quantifying trace gas uptake to tropospheric aerosol: recent advances and remaining challenges, Chem. Soc. Rev., 41, 6555–6581, https://doi.org/10.1039/C2CS35052A, 2012.
Ammann, M., Rossler, E., Strekowski, R., and George, C.: Nitrogen dioxide multiphase chemistry: uptake kinetics on aqueous solutions containing phenolic compounds, Phys. Chem. Chem. Phys., 7, 2513–2518, https://doi.org/10.1039/B501808K, 2005.
Bates, D. V.: Detection of chronic respiratory bronchiolitis in oxidant-exposed populations: analogy to tobacco smoke exposure, Environ. Health Pers., 101, 217–218, available at: http://www.ncbi.nlm.nih.gov/pmc/articles/PMC1519706/, 1993.
Behr, P., Morris, J. R., Antman, M. D., Ringeisen, B. R., Splan, J. R., and Nathanson, G. M.: Reaction and desorption of HCl and HBr following collisions with supercooled sulfuric acid, Geophys. Res. Lett., 28, 1961–1964, https://doi.org/10.1029/2000GL012716, 2001.
Behr, P., Scharfenort, U., Ataya, K., and Zellner, R.: Dynamics and mass accommodation of HCl molecules on sulfuric acid-water surfaces, Phys. Chem. Chem. Phys., 11, 8048–8055, https://doi.org/10.1039/B904629A, 2009.
Download
Altmetrics
Final-revised paper
Preprint