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Volume 12, issue 11
Atmos. Chem. Phys., 12, 5129-5145, 2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.

Special issue: Observations and modeling of aerosol and cloud properties...

Atmos. Chem. Phys., 12, 5129-5145, 2012
© Author(s) 2012. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 12 Jun 2012

Research article | 12 Jun 2012

Shortwave radiative forcing and efficiency of key aerosol types using AERONET data

O. E. García1,*, J. P. Díaz1, F. J. Expósito1, A. M. Díaz1, O. Dubovik2, Y. Derimian2, P. Dubuisson2, and J.-C. Roger3 O. E. García et al.
  • 1Grupo de Observación de la Tierra y la Atmósfera (GOTA), Universidad de La Laguna, Tenerife, Spain
  • 2Laboratoire d'Optique Amosphérique, Université des Sciences et Technologies de Lille, Villeneuve d'Ascq, France
  • 3Laboratoire de Météorologie Physique, Université Blaise Pascal, Clermont-Ferrand, France
  • *now at: Centro de Investigación Atmósferica de Izaña (CIAI), Agencia Estatal de Meteorología (AEMET), Spain

Abstract. The shortwave radiative forcing (ΔF) and the radiative forcing efficiency (ΔFeff) of natural and anthropogenic aerosols have been analyzed using estimates of radiation both at the Top (TOA) and at the Bottom Of Atmosphere (BOA) modeled based on AERONET aerosol retrievals. Six main types of atmospheric aerosols have been compared (desert mineral dust, biomass burning, urban-industrial, continental background, oceanic and free troposphere) in similar observational conditions (i.e., for solar zenith angles between 55° and 65°) in order to compare the nearly same solar geometry. The instantaneous ΔF averages obtained vary from −122 ± 37 Wm−2 (aerosol optical depth, AOD, at 0.55 μm, 0.85 ± 0.45) at the BOA for the mixture of desert mineral dust and biomass burning aerosols in West Africa and −42 ± 22 Wm−2 (AOD = 0.9 ± 0.5) at the TOA for the pure mineral dust also in this region up to −6 ± 3 Wm−2 and −4 ± 2 Wm−2 (AOD = 0.03 ± 0.02) at the BOA and the TOA, respectively, for free troposphere conditions. This last result may be taken as reference on a global scale. Furthermore, we observe that the more absorbing aerosols are overall more efficient at the BOA in contrast to at the TOA, where they backscatter less solar energy into the space. The analysis of the radiative balance at the TOA shows that, together with the amount of aerosols and their absorptive capacity, it is essential to consider the surface albedo of the region on which they are. Thus, we document that in regions with high surface reflectivity (deserts and snow conditions) atmospheric aerosols lead to a warming of the Earth-atmosphere system.

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