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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
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Volume 11, issue 18 | Copyright
Atmos. Chem. Phys., 11, 9887-9898, 2011
https://doi.org/10.5194/acp-11-9887-2011
© Author(s) 2011. This work is distributed under
the Creative Commons Attribution 3.0 License.

Research article 26 Sep 2011

Research article | 26 Sep 2011

Inversion of long-lived trace gas emissions using combined Eulerian and Lagrangian chemical transport models

M. Rigby1, A. J. Manning2, and R. G. Prinn1 M. Rigby et al.
  • 1Center for Global Change Science, Massachusetts Institute of Technology, 77 Massachusetts Ave., Cambridge, MA, 02139, UK
  • 2Atmospheric Dispersion Group, UK Met. Office, Exeter, EX1 3PB, UK

Abstract. We present a method for estimating emissions of long-lived trace gases from a sparse global network of high-frequency observatories, using both a global Eulerian chemical transport model and Lagrangian particle dispersion model. Emissions are derived in a single step after determining sensitivities of the observations to initial conditions, the high-resolution emissions field close to observation points, and larger regions further from the measurements. This method has the several advantages over inversions using one type of model alone, in that: high-resolution simulations can be carried out in limited domains close to the measurement sites, with lower resolution being used further from them; the influence of errors due to aggregation of emissions close to the measurement sites can be minimized; assumptions about boundary conditions to the Lagrangian model do not need to be made, since the entire emissions field is estimated; any combination of appropriate models can be used, with no code modification. Because the sensitivity to the entire emissions field is derived, the estimation can be carried out using traditional statistical methods without the need for multiple steps in the inversion. We demonstrate the utility of this approach by determining global SF6 emissions using measurements from the Advanced Global Atmospheric Gases Experiment (AGAGE) between 2007 and 2009. The global total and large-scale patterns of the derived emissions agree well with previous studies, whilst allowing emissions to be determined at higher resolution than has previously been possible, and improving the agreement between the modeled and observed mole fractions at some sites.

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