Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 10, 2195-2208, 2010
© Author(s) 2010. This work is distributed under
the Creative Commons Attribution 3.0 License.
02 Mar 2010
Physical and optical properties of atmospheric aerosols by in-situ and radiometric measurements
M. Calvello1, F. Esposito1,2, G. Pavese1, and C. Serio2 1Consiglio Nazionale delle Ricerche-Istituto di Metodologie per l'Analisi Ambientale (CNR-IMAA), C. da S. Loja, 85050 Tito Scalo, Potenza, Italy
2Dipartimento di Ingegneria e Fisica dell'Ambiente, Università della Basilicata, Viale dell'Ateneo Lucano n. 10, 85100 Potenza, Italy
Abstract. Physical and optical properties of atmospheric aerosols collected by using a high resolution (1.5 nm) spectroradiometer (spectral range 400–800 nm), a 13-stage Dekati Low Pressure Impactor (size range 30 nm–10 μm), and an AE31 Aethalometer (7 wavelenghts from 370 nm to 950 nm), have been examined in a semi-rural site in Southwest Italy (Tito Scalo, 40°35' N, 15°41' E, 750 m a.s.l.). In particular, daily averaged values of AOD and Ångström turbidity parameters from radiometric data together with mass-size distributions from impactor data and Black Carbon (BC) concentrations have been analyzed from May to October 2008. Furthermore, by inverting direct solar radiances, aerosol columnar number and volume size distributions have been obtained for the same period. The comparison of different observation methods, allowed to verify if, and in what conditions, changes in aerosol properties measured at ground are representative of columnar properties variations. Agreement between columnar and in-situ measurements has been obtained in case of anthropogenic aerosol loading, while in case of Saharan dust intrusions some discrepancies have been found when dust particles were located at high layers in the atmosphere (4–8 km) thus affecting columnar properties more than surface ones. For anthropogenic aerosols, a good correlation has been confirmed through the comparison of fine aerosol fraction contribution as measured by radiometer, impactor and aethalometer, suggesting that, in this case, the particles are more homogeneously distributed over the lower layers of atmosphere and columnar aerosol optical properties are dominated by surface measured component.

Citation: Calvello, M., Esposito, F., Pavese, G., and Serio, C.: Physical and optical properties of atmospheric aerosols by in-situ and radiometric measurements, Atmos. Chem. Phys., 10, 2195-2208,, 2010.
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