Atmospheric Chemistry and Physics www.atmos-chem-phys.net 1680-7316 1680-7324 9 22 2009 10.5194/acp-9-8799-2009 http://www.atmos-chem-phys.net/9/8799/2009/ http://www.atmos-chem-phys.net/9/8799/2009/acp-9-8799-2009.html http://www.atmos-chem-phys.net/9/8799/2009/acp-9-8799-2009.pdf 8799 8811 2009-11-19 UV Raman lidar measurements of relative humidity for the characterization of cirrus cloud microphysical properties P. Di Girolamo paolo.digirolamo@unibas.it D. Summa R.-F. Lin T. Maestri R. Rizzi G. Masiello Dipartimento di Ingegneria e Fisica dell'Ambiente, Universitá della Basilicata, viale dell'Ateneo Lucano n. 10, 85100 Potenza, Italy Goddard Earth Sci. and Technology Center, Univ. of Maryland Baltimore County, MD, USA Mesoscale Atmospheric Processes Branch, NASA GSFC, Code 613.1 Building 33, Greenbelt, MD 20771, USA Dipartimento di Fisica, Università di Bologna, viale Berti-Pichat 6/2, 40127 Bologna, Italy Raman lidar measurements performed in Potenza by the Raman lidar system BASIL in the presence of cirrus clouds are discussed. Measurements were performed on 6 September 2004 in the frame of the Italian phase of the EAQUATE Experiment. The major feature of BASIL is represented by its capability to perform high-resolution and accurate measurements of atmospheric temperature and water vapour, and consequently relative humidity, both in daytime and night-time, based on the application of the rotational and vibrational Raman lidar techniques in the UV. BASIL is also capable to provide measurements of the particle backscatter and extinction coefficient, and consequently lidar ratio (at the time of these measurements, only at one wavelength), which are fundamental to infer geometrical and microphysical properties of clouds. A case study is discussed in order to assess the capability of Raman lidars to measure humidity in presence of cirrus clouds, both below and inside the cloud. While air inside the cloud layers is observed to be always under-saturated with respect to water, both ice super-saturation and under-saturation conditions are found inside these clouds. Upper tropospheric moistening is observed below the lower cloud layer. The synergic use of the data derived from the ground based Raman Lidar and of spectral radiances measured by the NAST-I Airborne Spectrometer allows the determination of the temporal evolution of the atmospheric cooling/heating rates due to the presence of the cirrus cloud. Lidar measurements beneath the cirrus cloud layer have been interpreted using a 1-D cirrus cloud model with explicit microphysics. The 1-D simulations indicate that sedimentation-moistening has contributed significantly to the moist anomaly, but other mechanisms are also contributing. This result supports the hypothesis that the observed mid-tropospheric humidification is a real feature which is strongly influenced by the sublimation of precipitating ice crystals. Results illustrated in this study demonstrate that Raman lidars, like the one used in this study, can resolve the spatial and temporal scales required for the study of cirrus cloud microphysical processes and appear sensitive enough to reveal and quantify upper tropospheric humidification associated with cirrus cloud sublimation. 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