Atmospheric Chemistry and Physics www.atmos-chem-phys.net 1680-7316 1680-7324 9 22 2009 10.5194/acp-9-8735-2009 http://www.atmos-chem-phys.net/9/8735/2009/ http://www.atmos-chem-phys.net/9/8735/2009/acp-9-8735-2009.html http://www.atmos-chem-phys.net/9/8735/2009/acp-9-8735-2009.pdf 8735 8743 2009-11-16 On the capability of IASI measurements to inform about CO surface emissions A. Fortems-Cheiney F. Chevallier frederic.chevallier@lsce.ipsl.fr I. Pison P. Bousquet C. Carouge C. Clerbaux P.-F. Coheur M. George D. Hurtmans S. Szopa Laboratoire des Sciences du Climat et de l'Environnement, CEA-CNRS-UVSQ, Gif-sur-Yvette, France UPMC Univ Paris 06, CNRS UMR8190, LATMOS/IPSL, Paris, France Spectroscopie de l'atmosphère, Chimie Quantique et Photophysique, Université Libre de Bruxelles, Brussels, Belgium now at: Division of Engineering and Applied Sciences, Harvard University, Cambridge, Massachusetts, USA Between July and November 2008, simultaneous observations were conducted by several orbiting instruments that monitor carbon monoxide in the atmosphere, among them the Infrared Atmospheric Sounding Instrument (IASI) and Measurements Of Pollution In The Troposphere (MOPITT). In this paper, the concentration retrievals at about 700 hPa from these two instruments are successively used in a variational Bayesian system to infer the global distribution of CO emissions. Starting from a global emission budget of 479 Tg for the considered period, the posterior estimate of CO emissions using IASI retrievals gives a total of 643 Tg, which is in close agreement with the budget calculated with version 3 of the MOPITT data (649 Tg). The regional totals are also broadly consistent between the two inversions. Even though our theoretical error budget indicates that IASI constrains the emissions slightly less than MOPITT, because of lesser sensitivity in the lower troposphere, these first results indicate that IASI may play a major role in the quantification of the emissions of CO. Allen,D., Pickering, K., and Fox-Rabinovitz, M. : Evaluation of pollutant outflow and CO sources during TRACE-P using model-calculated, aircraft-based, and measurements of MOPITT-derived CO concentrations, J. Geophys. Res., 109, D15S03, doi:10.1029/2003JD004250, 2004. Arellano Jr., A. F., Kasibhatla, P. S., Giglio, L., van der Werf, G. R., and Randerson, J. T.: Top-down estimates of global CO sources using MOPITT measurements, Geophys. Res. Lett., 31, L01104, doi:10.1029/2003GL018609, 2004. Bousquet, P., Hauglustaine, D. A., Peylin, P., Carouge, C., and Ciais, P.: Two decades of OH variability as inferred by an inversion of atmospheric transport and chemistry of methyl chloroform, Atmos. Chem. Phys., 5, 2635–2656, 2005. Buchwitz, M., Khlystova, I., Bovensmann, H., and Burrows, J. P.: Three years of global carbon monoxide from SCIAMACHY: Comparison with MOPITT and first results related to the detection of enhanced CO over cities, Atmos. Chem. Phys., 7, 2399–2411,2007. Carmichael, G. R., Tang, Y., Kurata, G., Uno, I., and Streets, D. G.: Evaluating regional emissions estimates using the TRACE-P observations, J.Geophys. Res., 108(D21), 8810, doi:10.1029/2002JD003116, 2003. Chevallier, F., Fisher, M., Peylin, P., Serrar, S., Bousquet, P., Bréon, F.-M., Chédin, A., and Ciais, P.: Inferring \chemCO_2 sources and sinks from satellite observations: method and application to TOVS data, J. Geophys. Res., 110, D24309, doi:10.1029/2005JD006390, 2005. Chevallier, F., Bréon, F.-M., and Rayner, P. J.: Contribution of the Orbiting Carbon Observatory to the estimation of \chemCO_2 sources and sinks: Theoretical study in a variational data assimilation framework, J. Geophys. Res., 112, D09307, doi:10.1029/2006JD007375, 2007. Chevallier, F., Fortems, A., Bousquet, P., Pison, I., Szopa, S., Devaux, M., and Hauglustaine, D.: African CO emissions between years 2000 to 2006 as estimated from MOPITT observations, Biogeosciences, 6, 103–111, 2009. Clerbaux, C., Coheur, P.-F., Hurtmans, D., Barret, B., Carleel, M., Colin, R., Semeniuk, K., McConnell, J.C., Boone, C. and Bernath, P.: Carbon monoxide distribution from the ACE-FTS solar occultation measurements, Geophys. Res. Lett., 32, L16S01, doi:10.1029/2005GL022394, 2005. Clerbaux, C., Edwards, D. P., Deeter, M., Emmons, L., Lamraque, J.-F., Tie, X. X., Massie, S. T., and Gille, J.: Carbon monoxide pollution from cities and urban areas observed by the Terra/MOPITT mission, Geophys. Res. Lett., 35, L103817, doi:10.1029/2007GL032300, 2008. Clerbaux, C., Boynard, A., Clarisse, L., George, M., Hadji-Lazaro, J., Herbin, H., Hurtmans, D., Pommier, M., Razavi, A., Turquety, S., Wespes, C., and Coheur, P.-F.: Monitoring of atmospheric composition using the thermal infrared IASI/MetOp sounder, Atmos. Chem. Phys., 9, 6041–6054, 2009. Crawford, J. H., Heald, C. L., Fuelberg, H. E., Morse, D. M., Sachse, G. W., Emmons, L. K., Gille, J. C., Edward, D. P., Deeter, M. N., Chen, G., Olson, J. R., Connors, V. S., Kittaka, C., and Hamlin, A. J.: Relationship between measurements of MOPITT and in-situ observations of CO based on a large-scale feature sampled during TRACE-P, J.Geophys. Res., 109, D15S04, doi:10.1029/2002JD004308, 2004. Deeter, M. N., Emmons, L. K., Francis, G. L., et al.: Operational carbon monoxide retrieval algorithm and selected results for the MOPITT instrument, J. Geophys. Res., 108(D14), 4399, doi:10.1029/2002JD003186, 2003. Deeter, M. N., Emmons, L. K., Edwards, D. P., Gille, J. C., and Drummond, J. R.: Vertical resolution and information content of CO profiles retrieved by MOPITT, Geophys. Res. Lett., 31, L15112, doi:10.1029/2004GL020235, 2004. Emmons, L. K., Deeter, M. N., Gille, J. C., et al.: Validation of Measurements of Pollution in the Troposphere (MOPITT) CO retrievals with aircraft in situ profiles, J. Geophys. Res., 109, D03309, doi:10.1029/2003JD004101, 2004. Folberth, G. A., Hauglustaine, D. A., Lathière, J., and Brocheto, F.: Interactive chemistry in the Laboratoire de Météorologie Dynamique general circulation model: model description and impact analysis of biogenic hydrocarbons on tropospheric chemistry, Atmos. Chem. Phys., 6, 2273–2319, 2006. George, M., Clerbaux, C., Coheur, P.-F., Hadji-Lazaro, J., Edwards, D., Worden, H., Luo, M., Rinsland, C. P., and Barnet, C.: Carbon monoxide distributions from the IASI/METOP mission: evaluation with other space-borne remote sensors, Atmos. Chem. Phys. Discuss., 9, 9793–9822, 2009. Gilbert, J. C. and Lemaréchal, C.: Some numerical experiments with variable-storage quasi-Newton algorithms, Math. Program., 45, 407–435, 1989. Hauglustaine, D. A., Hourdin, F., Jourdain, L., Filiberti, M.-A., Walters, S., Lamarque, J.-F., and Holland, E. A.: Interactive chemistry in the Laboratoire de Météorologie Dynamique general circulation model: Description and background tropospheric chemistry evaluation, J. Geophys. Res., 109, D04314, doi:10.1029/2003JD003957, 2004. Heald, C. L., Jacob, D. J., Jones, D. B. A., Palmer, P. I., Logan, J. A., Streets, D. G., Sachse, G. W., Gille, J. C., Hoffman, R. N., and Nehrkorn, T.: Comparative inverse analysis of satellite (MOPITT) and aircraft (TRACE-P) observations to estimates Asian sources of carbon monoxide, J. Geophys. Res., 109, D23306, doi:10.1029/2004GL005185, 2004. Hollingsworth, A., Engelen, R. J., Textor, C., et al.: The Global Earth-system Monitoring using Satellite and in-situ data (GEMS) Project: Towards a monitoring and forecasting system for atmospheric composition, B. Am. Meteorol. Soc., 89, 1147–1164, doi:10.1175/2008BAMMS2355.1, 2008. Hourdin, F., Musat, I., Bony, S., et al.: The LMDZ4 general circulation model: climate performance and sensitivity to parametrized physics with emphasis on tropical convection, Clim. Dynam., 27, 787–813, 2006. Levelt, P. F., Hilsenrath, E., Leppelmeier, G. W., van den Oord, G. H. J., Bhartia, P. K., Tamminen, J., de Haan, J. F., and Veefkinf, J. P.: Science objectives of the Ozone Monitoring Instrument, Geo. Rem. Sens., 44, 5, 1199–1208, 2006. Luo, M., Rinsland, C. P., Rodgers, C. D., Logan, J. A., Worden, H., Kulawik, S., Eldering, A., Goldman, A., Shephard, M. W., Gunson, M., and Lampel, M. : Comparison of carbon monoxide measurements by TES and MOPITT: The influence of a priori data and instrument characteristics on nadir atmospheric species retrievals, J. Geophys. Res., 112, D09303, doi:10.1029/2006JD007663, 2007. Ohara, T., Akimoto, H., Kurokawa, J., Horii, N., Yamaji, K., Yan, X., and Hayasaka, T.: An Asian emission inventory of anthropogenic emission sources for the period 1980–2020, Atmos. Chem. Phys., 7, 4419–4444, 2007. Olivier, J. G. J. and Berdowski, J. J. M.: Global emissions sources and sinks, The Climate System, 2001. Palmer, P. I., Jacob, D. J., Jones, D. B. A., Heald, C. L., Yantosca, R. M., Logan, J. A., Sachse, G.W. and Streets, D.G. : Inverting for emissions of carbon monoxide from Asia using aircraft observations over the Western Pacific, J. Geophys. Res., 108(D21), 8828, doi:10.1029/2003JD003397, 2007. Pétron, G., Granier, C., Khattatov, B., Yudin, V., Lamarque, J.-F., Emmons, L., Gille, J., and Edwards, D. P.: Monthly CO surface sources inventory based on the 2000-2001 MOPITT satellite data, Geophys. Res. Lett., 31, L21107, doi:10.1029/2004GL020560, 2004. Pfister, G., Hess, P. G., Emmons, L. K., Lamarque, J.-F., Wiedinmyer, C., Edwards, D. P., Petron, G., Gille, J. C., and Sachse, G. W.: Quantifying CO emissions from the 2004 Alaskan wildfires using MOPITT CO data, Geophys. Res. Lett, 32, L11809, doi:10.1029/2004GL022995, 2004. Pison, I., Bousquet, P., Chevallier, F., Szopa, S., and Hauglustaine, D. A.: Multi-species inversion of \chemCH_4, CO and \chemH_2 emissions from surface measurements, Atmos. Chem. Phys., 9, 5281–5297, 2009. Rodgers, C. D. and Connor, B. J.: Intercomparison of remote sounding instruments, J. Geophys. Res., 108(D3), 4116, doi:10.1029/2002JD002299, 2003. Turquety, S., Hadji-Lazaro, J., Clerbaux, C., Hauglustaine, D. A., Clough, S. A., Cassé, V., Schlüssel, P., and Mégie, G.: Operational trace gas retrieval algorithm for the Infrared Atmospheric Sounding Interferometer, J. Geophys. Res., 109, D21301, doi:10.1029/2004JD004821, 2004. Turquety, S., Logan, J. A., Jacob, D. J., Hudman, R. C., Leung, F. Y., Heald, C. L., Yantosca, R. M., and Wu, S.: Inventory of boreal fire emissions for North America in 2004: importance of peat burning and pyroconvective injection, J. Geophys. Res., 112, D12S03, doi:10.1029/2006JD007281, 2007. Turquety, S., Hurtmans, D., Hadji-Lazaro, J., Coheur, P.-F., Clerbaux, C., Josset, D., and Tsamalis, C.: Tracking the emission and transport of pollution from wildfires using the IASI CO retrievals: analysis of the summer 2007 Greek fires, Atmos. Chem. Phys., 9, 4897–4913, 2009. Van der Werf, G. R., Randerson, J. T., Giglio, L., Collatz, G. J., and Kasibhatla, P. S.: Interannual variability in global biomass burning emission from 1997 to 2004, Atmos. Chem. Phys., 6, 3423–3441, 2006. Wang, Y. X., McElroy, M. B., Wang, T., and Palmer, P. I. : Asian emissions of CO and NOx : constraints from aircraft and Chinese station data, J. Geophys. Res., 109, D24304, doi:10.1029/2004JD005250, 2004.