<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "http://dtd.nlm.nih.gov/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-9-8479-2009</article-id>
<title-group>
<article-title>Evaluating the potential of IASI ozone observations to constrain simulated surface ozone concentrations</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Foret</surname>
<given-names>G.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Hamaoui</surname>
<given-names>L.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Schmechtig</surname>
<given-names>C.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Eremenko</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Keim</surname>
<given-names>C.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dufour</surname>
<given-names>G.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Boynard</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Coman</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Ung</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Beekmann</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Université Paris 12 et 7, UMR CNRS/INSU 7583, Laboratoire Interuniversitaire des Systèmes Atmosphériques/IPSL, Créteil, France</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Institut National de l&apos;Environnement Industriel et des Risques, Chronic Risks Division, Parc Technologique Alata, Verneuil-en-Halatte, France</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>UPMC Université Paris 06, UMR CNRS/INSU 8190, Laboratoire Atmosphères, Milieux, Observations Spatiales/IPSL, Paris, France</addr-line>
</aff>
<pub-date pub-type="epub">
<day>06</day>
<month>11</month>
<year>2009</year>
</pub-date>
<volume>9</volume>
<issue>21</issue>
<fpage>8479</fpage>
<lpage>8491</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys.net/9/8479/2009/acp-9-8479-2009.html">This article is available from http://www.atmos-chem-phys.net/9/8479/2009/acp-9-8479-2009.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys.net/9/8479/2009/acp-9-8479-2009.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/9/8479/2009/acp-9-8479-2009.pdf</self-uri>
<abstract>
<p>A tracer study has been performed for two summers in 2003 and 2004 with a
regional chemistry-transport model in order to evaluate the potential
constraint that tropospheric ozone observations from nadir viewing infrared
sounders like IASI or TES exert on modelled near surface ozone. As these
instruments show high sensitivity in the free troposphere, but low
sensitivity at ground, it is important to know how much of the information
gained in the free troposphere is transferred to ground through vertical
transport processes. Within the European model domain, and within a time
span of 4 days, only ozone like tracers initialised in vertical layers above
500 hPa are transported to the surface. For a tracer initialised between 800 and 700 hPa,
seven percent reaches the surface within one to three days, on
the average over the European model domain but more than double over the
Mediterranean Sea. For this region, trajectory analysis shows that this is
related to strong subsident transport. These results are confirmed by a
second tracer study taking into account averaging kernels related to IASI
retrievals, indicating the potential of these measurements to efficiently
constrain surface ozone values.</p>
</abstract>
<counts><page-count count="13"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> Beer, R.: TES on the Aura mission: Scientific objectives, measurements and analysis overview, IEEE Trans. Geosci. Remote Sens., 44(5), 1102–1105, 2006. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> Bessagnet, B., Menut, L., Aymoz, G., Chepfer, H., and Vautard, R.: Modeling dust emissions and transport within Europe: The Ukraine March 2007 event, J. Geophys. Res., 113, D15202, doi:10.1029/2007JD009541, 2008. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Blond, N. and Vautard R.: Three-dimensional ozone analyses and their use for short-term ozone forecasts, J. Geophys. Res., 109, D17303, doi:10.1029/2004JD004515, 2004. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> Boisgontier, B., Mallet, V., Berroir, J. P., Bocquet, M., Herlin, I., and Sportisse, B.: Satellite data assimilation for air quality forecast, Simul. Model. Pract. Th., 16, 1541–1545, 2008. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Boynard, A., Clerbaux, C., Coheur, P.-F., Hurtmans, D., Turquety, S., George, M., Hadji-Lazaro, J., Keim, C., and Meyer-Arnek, J.: Measurements of total and tropospheric ozone from IASI: comparison with correlative satellite, ground-based and ozonesonde observations, Atmos. Chem. Phys., 9, 6255–6271, 2009. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> Clerbaux, C., Hadji-Lazaro, J., Turquety, S., George, M., Coheur, P.-F., Hurtmans, D., Wespes, C., Herbin, H., Blumstein, D., Tournier, B., and Phulpin, T.: The IASI/MetOp I Mission: First Observations and Highlights of its Potential Contribution to GMES, COSPAR Inf. Bul., Vol. 2007, 19–24, 2007. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> Coheur, P.-F., Barret, B., Turquety, S., Hurtmans, D., Hadji-Lazaro, J., and Clerbaux, C.: Retrieval and characterization of ozone vertical profiles from a thermal infrared nadir sounder, J. Geophys. Res., 110, D24303, doi:10.1029/2005JD005845, 2005. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> Colella P. and Woodward, P. R.: The Piecewise Parabolic Method (PPM) for Gas-Dynamical Simulations, J. Comput. Phys., 54, 174–201, 1984. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Coll, I., Pinceloup, S., Perros, P. E., Laverdet, G., and Le Bras, G.: 3D analysis of high ozone production rates observed during the ESCOMPTE campaign, Atmos. Res., 477–505, 2005. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Cotton, W. R., Alexander, G. D., Hertenstein, R., Walko, R. L., McAnelly, R. L., and Nicholls, M.: Cloud venting – A review and some new global annual estimates, Earth-Sci. Rev., 39, 169–206, 1995. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Dacre, H. F., Gray, S. L., and Belcher, S. E.: A case study of boundary layer ventilation by convection and coastal processes, J. Geophys. Res., 112, D17106, doi:10.1029/2006JD007984, 2007. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Deeter, M. N., Edwards, D. P., Gille, J. C., and Drummond, J. R.: Sensitivity of MOPITT observations to carbon monoxide in the lower troposphere, J. Geophys. Res., 112, D24306, doi:10.1029/2007JD008929, 2007. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Deguillaume, L., Beekmann, M., and Derognat, C.: Uncertainty evaluation of ozone production and its sensitivity to emission changes over the Ile-de-France region during summer periods, J. Geophys. Res., 113, D02304, doi:10.1029/2007JD009081, 2008. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> Doherty, R. M., Stevenson, D. S., Collins, W. J., and Sanderson, M. G.: Influence of convective transport on tropospheric ozone and its precursors in a chemistry-climate model, Atmos. Chem. Phys., 5, 3205–3218, 2005. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Draxler, R. R. and Rolph, G. D.: HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) Model access via NOAA ARL READY Website (http://www.arl.noaa.gov/ready/hysplit4.html), NOAA Air Resources Laboratory, Silver Spring, MD, 2003. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Elbern, H. and Schmidt, H.: Ozone episode analysis by fourdimensional variational chemistry data assimilation, J. Geophys. Res., 106, 3569–3590, 2001. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Eremenko, M., Dufour, G., Foret, G., Keim, C., Orphal, J., Beekmann, M., Bergametti, G., and Flaud, J.-M.: Tropospheric ozone distributions over Europe during the heat wave in July 2007 observed from infrared nadir spectra recorded by IASI, Geophys. Res. Lett., 35, L18805, doi:10.1029/2008GL034803, 2008. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Fiore, A. M., Jacob, D. J., Bey, I., Yantosca, R. M., Field, B. D., and Fusco, A. C.: Background ozone over the United States in summer: Origin, trend, and contribution to pollution episodes, J. Geophys. Res., 107, 4275, doi:10.1029/2001JD000982, 2002. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Forêt, G., Flamant, C., Cautenet, S., Pelon, J., Minvielle, F., Taghavi, M., and Chazette, P.: The structure of the haze plume over the Indian Ocean during INDOEX: tracer simulations and LIDAR observations, Atmos. Chem. Phys., 6, 907–923, 2006. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> Hauglustaine, D. A., Hourdin, F., Walters, S., Jourdain, L., Filiberti, M.-A., Larmarque, J.-F., Holland, E. A.: Interactive chemistry in the Laboratoire de Météorologie Dynamique general circulation model: description and background tropospheric chemistry evaluation, J. Geophys. Res., 109, D04314, doi:10.1029/2003JD003957, 2004. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Henne, S., Dommen, J., Neininger, B., Reimann, S., Staehelin, J., and Prévôt, A. S. H.: Influence of mountain venting in the Alps on the ozone chemistry of the lower free troposphere and the European pollution export, J. Geophys. Res., 110, D22307, doi:10.1029/2005JD005936, 2005. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Hodzic, A., Vautard, R., Chepfer, H., Goloub, P., Menut, L., Chazette, P., Deuzé, J. L., Apituley, A., and Couvert, P.: Evolution of aerosol optical thickness over Europe during the August 2003 heat wave as seen from CHIMERE model simulations and POLDER data, Atmos. Chem. Phys., 6, 1853–1864, 2006. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Honoré, C., Rouil, L., Vautard, R., Beekmann, M., Bessagnet, B., Dufour, A., Elichegaray, C., Flaud, J.-M., Malherbe, L., Meleux, F., Menut, L., Martin, D., Peuch, A., Peuch, V.-H., and Poisson, N.: Predictability of European air quality: Assessment of 3 years of operational forecasts and analyses by the PREVAIR system, J. Geophys. Res., 113, D04301, doi:10.1029/2007JD008761, 2008. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> Kalabokas, P. D., Mihalopoulos, N., Ellul, R., Kleanthous, S., and Repapis, C. C.: An investigation of the meteorological and photochemical factors influencing the background rural and marine surface ozone levels in the Central and Eastern Mediterranean, Atmos. Environ., 42, 7894–7906, 2008. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Keim, C., Eremenko, M., Orphal, J., Dufour, G., Flaud, J.-M., Höpfner, M., Boynard, A., Clerbaux, C., Payan, S., Coheur, P.-F., Hurtmans, D., Claude, H., Dier, H., Johnson, B., Kelder, H., Kivi, R., Koide, T., López Bartolomé, M., Lambkin, K., Moore, D., Schmidlin, F. J., and Stübi, R.: Tropospheric ozone from IASI: comparison of different inversion algorithms and validation with ozone sondes in the northern middle latitudes, Atmos. Chem. Phys. Discuss., 9, 11441–11479, 2009. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> Kowol-Santen, J., Beekmann, M., Schmitgen, S., and Dewey, K.: Tracer analysis of transport from the boundary layer to the free troposphere, Geophys. Res. Lett., 28, 2907–2910, 2001. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> Lawrence, M. G. and Rasch, P. J.: Tracer transport in deep convective updrafts: plume ensemble versus bulk formulations, J. Atmos. Sci., 62, 2880–2894, 2005. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> Lelieveld, J., Berresheim, H., Borrmann, S., et al.: Global Air Pollution Crossroads over the Mediterranean, Science, 298, doi:10.1126, 2002. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> Marenco, A., Thouret, V., Nédélec, P., Smit, H., Helten, M., Kley, D., Karcher, F., Simon, P., Law, K., Pyle, J., Poschmann, G., von Wrede, R., Hume, C., and Cook, T.: Measurement of ozone and water vapor by Airbus in-service aircraft: The MOZAIC airborne program, An overview, J. Geophys. Res., 103, 25631–25642, 1998. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> Monks, P. S., Carpenter, L. J., Penkett, S. A., Ayers, G. P., Gillett, R. W., Galbally, I. E., and Meyer, C. P.: Fundamental ozone photochemistry in the remote marine boundary layer the soapex experiment, measurement and theory, Atmos. Environ., 32, 3647–3664, 1998. </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> Olivié, D. J. L., van Velthoven, P. F. J., Beljaars, A. C. M., and Kelder, H. M.: Comparison between archived and off-line diagnosed convective mass fluxes in the chemistry transport model TM3, J. Geophys. Res., 109, D11303, doi:10.1029/2003JD004036, 2004. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> Parrington, M., Jones, D. B. A., Bowman, K. W., Horowitz, L. W., Thompson, A. M., Tarasick, D. W., and Witte, J. C.: Estimating the summertime tropospheric ozone distribution over North America through assimilation of observations from the Tropospheric Emission Spectrometer, J. Geophys. Res., 113, D18307, doi:10.1029/2007JD009341, 2008. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> Parrington, M., Jones, D. B. A., Bowman, K. W., Thompson, A. M., Tarasick, D. W., Merrill, J., Oltmans, S. J., Leblanc, T., Witte, J. C., and Millet, D. B.: Impact of the assimilation of ozone from the Tropospheric Emission Spectrometer on surface ozone across North America, Geosphys. Res. Lett., 36, L04802, doi:10.1029/2008GL036935, 2009. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> Rodgers, C. D.: Inverse Methods for Atmospheric Sounding : Theory and Practice, World Scientific, Series on Atmospheric, Oceanic and Planetary Physics, 2, Hackensack, N. J., 2000. </mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple"> Rouil, L., Honoré, C., Vautard, R., Beekmann, M., Bessagnet, B., Malherbe, L., Meleux, F., Dufour, A., Elichegaray, C., Flaud, J.-M., Menut, L., Martin, D., Peuch, A., Peuch, V.-H. and Poisson, N.: Prev&apos;air: An Operational Forecasting and Mapping System for Air Quality in Europe, B. Am. Meteorol. Soc., 90, doi: 10.1175/2008BAMS239, 2009. </mixed-citation>
</ref>
<ref id="ref36">
<label>36</label><mixed-citation publication-type="other" xlink:type="simple"> Sinclair, V. A., Gray, S. L., and Belcher, S. E.: Boundary-layer ventilation by baroclinic life cycles, Q. J. R. Meteorol. Soc., 134, 1409–1424, 2008. </mixed-citation>
</ref>
<ref id="ref37">
<label>37</label><mixed-citation publication-type="other" xlink:type="simple"> Szopa, S., Foret, G., Menut, L., and Cozic, A.: Impact of large scale circulation on European summer surface ozone: consequences for modelling forecast, Atmos. Environ., 43, 1189–1195, 2009. </mixed-citation>
</ref>
<ref id="ref38">
<label>38</label><mixed-citation publication-type="other" xlink:type="simple"> Tiedtke, M.: A comprehensive mass flux scheme for cumulus parameterization in large-scale models, Mon. Weather Rev., 117, 1779–1800, 1989. </mixed-citation>
</ref>
<ref id="ref39">
<label>39</label><mixed-citation publication-type="other" xlink:type="simple"> Traub, M., Fischer, H., de Reus, M., Kormann, R., Heland, H., Ziereis, H., Schlager, H., Holzinger, R., Williams, J., Warneke, C., de Gouw, J., and Lelieveld, J.: Chemical characteristics assigned to trajectory clusters during the MINOS campaign, Atmos. Chem. Phys., 3, 459–468, 2003. </mixed-citation>
</ref>
<ref id="ref40">
<label>40</label><mixed-citation publication-type="other" xlink:type="simple"> Vautard, R., Honore, C., Beekmann, M., and Rouil, L.: Simulation of ozone during the August 2003 heat wave and emission control scenarios, Atmos. Environ., 39, 2957–2967, 2005. </mixed-citation>
</ref>
<ref id="ref41">
<label>41</label><mixed-citation publication-type="other" xlink:type="simple"> Vestreng, V., Breivik, K., Adams, M., Wagener, A., Goodwin, J., Rozovskkaya, O., and Pacyna, J. M.: Inventory Review 2005, Emission Data reported to LRTAP Convention and NEC Directive, Initial review of HMs and POPs, Technical report MSC-W 1/2005, ISSN 0804-2446, 2005. </mixed-citation>
</ref>
<ref id="ref42">
<label>42</label><mixed-citation publication-type="other" xlink:type="simple"> Wesely, M. L. and Hicks, B. B.: Some factors that affect the deposition rates of sulfur dioxide and similar gases on vegetation, J. Air Pollut. Control Ass., 27, 1110–1116, 1977. </mixed-citation>
</ref>
<ref id="ref43">
<label>43</label><mixed-citation publication-type="other" xlink:type="simple"> Xoplaki, E.: Climate variability over the Mediterranean, PhD thesis, University of Bern, Switzerland, (http://www.giub.unibe.ch/klimet/docs/phd_xoplaki.pdf), 2000. </mixed-citation>
</ref>
<ref id="ref44">
<label>44</label><mixed-citation publication-type="other" xlink:type="simple"> Ziv, B., Saaroni, H. and Alpert, P.: The factors governing the summer regime over the eastern Mediterranean, Int. J. Climatol., 24, 1859–1871, 2004. </mixed-citation>
</ref>
</ref-list>
</back>
</article>