<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "http://dtd.nlm.nih.gov/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-9-743-2009</article-id>
<title-group>
<article-title>Aerosol effects on clouds and precipitation during the 1997 smoke episode in Indonesia</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Graf</surname>
<given-names>H.-F.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Yang</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Wagner</surname>
<given-names>T. M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Centre for Atmospheric Science, University of Cambridge, Cambridge, UK</addr-line>
</aff>
<pub-date pub-type="epub">
<day>29</day>
<month>01</month>
<year>2009</year>
</pub-date>
<volume>9</volume>
<issue>2</issue>
<fpage>743</fpage>
<lpage>756</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys.net/9/743/2009/acp-9-743-2009.html">This article is available from http://www.atmos-chem-phys.net/9/743/2009/acp-9-743-2009.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys.net/9/743/2009/acp-9-743-2009.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/9/743/2009/acp-9-743-2009.pdf</self-uri>
<abstract>
<p>In 1997/1998 a severe smoke episode due to extensive biomass burning,
especially of peat, was observed over Indonesia. September 1997 was the
month with the highest aerosol burden. This month was simulated using the
limited area model REMOTE driven at its lateral boundaries by ERA40
reanalysis data. REMOTE was extended by a new convective cloud
parameterization mimicking individual clouds competing for instability
energy. This allows for the interaction of aerosols, convective clouds and
precipitation. Results show that in the monthly mean convective
precipitation is diminished at nearly all places with high aerosol loading,
but at some areas with high background humidity precipitation from
large-scale clouds may over-compensate the loss in convective rainfall. The
simulations revealed that both large-scale and convective clouds&apos;
microphysics are influenced by aerosols. Since aerosols are washed and
rained out by rainfall, high aerosol concentrations can only persist at low
rainfall rates. Hence, aerosol concentrations are not independent of the
rainfall amount and in the mean the maximum absolute effects on rainfall
from large scale clouds are found at intermediate aerosol concentrations.
The reason for this behavior is that at high aerosol concentrations rainfall
rates are small and consequently also the anomalies are small. For
large-scale as well as for convective rain negative and positive anomalies
are found for all aerosol concentrations. Negative anomalies dominate and
are highly statistically significant especially for convective rainfall
since part of the precipitation loss from large-scale clouds is compensated
by moisture detrained from the convective clouds. The mean precipitation
from large-scale clouds is less reduced (however still statistically
significant) than rain from convective clouds. This effect is due to
detrainment of cloud water from the less strongly raining convective clouds
and because of the generally lower absolute amounts of rainfall from
large-scale clouds. With increasing aerosol load both, convective and large
scale clouds produce less rain. At very few individual time steps cases were
found when polluted convective clouds produced intensified rainfall via
mixed phase microphysics. However, these cases are not unequivocal and
opposite results were also simulated, indicating that other than
aerosol-microphysics effects have important impact on the results. Overall,
the introduction of the new cumulus parameterization and aerosol-cloud
interaction reduced some of the original REMOTE biases of precipitation
patterns and total amount.</p>
</abstract>
<counts><page-count count="14"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Abdul-Razzak, H. and Ghan, S.: A parameterization of aerosol activation 2, Multiple aerosol types, J. Geophys. Res., 105, 6837–6844, 2000. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Andreae, M. O., Rosenfeld, D., Artaxo, P., et al.: Smoking rain clouds over the Amazon, Science, 303, 1337–1342, doi:10.1126/science.1092779, 2004. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Altaratz, O., Koren, I., Reisin, T., Kostinski, A., Feingold, G., Levin, Z., and Yin, Y.: Aerosols&apos; influence on the interplay between condensation, evaporation and rain in warm cumulus cloud, Atmos. Chem. Phys., 8, 15–24, 2008. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Beheng, K. D.: A parameterization of warm cloud microphysical conversion processes, Atmos. Res., 33, 193–206, 1994. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Berry, E. X.: Modification of the warm rain process, Proc. First Natl. Conf. Weather Modification, Ed. American Meteorological Society, State University of New York, Albany, 81–88, 1968. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Boucher, O. and Lohmann, U.: The sulphate-CCN-cloud albedo effect – A sensitivity study with two general circulation models, Tellus, 47B, 281–300, 1995. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Chuang, C. C. and Penner, J. E.: Effects of anthropogenic sulphate on cloud drop nucleation and optical properties, Tellus, 47, 566–577, 1995. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Dusek, U., Frank, G. P., Helas, G., et al.: &quot;Missing&quot; cloud condensation nuclei in peat smoke, Geophys. Res. Lett., 32, L11802, doi:10.1029/2005GL022473, 2005. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Feingold, G., Cotton, W. R., Kreidenweis, S. M., and Davis, J. T.: The impact of giant condensation nuclei on drizzle formation in stratocumulus: Implications for cloud radiative properties, J. Atmos. Sci., 56, 24, 4100–4117, 1999. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Graf, H.-F. and Gräfe, I.: Die Niederschlagsverteilung im Raum Berlin in Abhängigkeit von Höhenwetterlage und Bodenwindrichtung, (The distribution of precipitation in the Berlin area depending on height weather and surface wind direction), Z. Meteorol., 29, 56–64, 1979. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Graf, H.-F.: The complex interaction of aerosols and clouds, Science, 203, 1309–1311, 27 February 2004. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Graf, H.-F. and Yang, J.: Evaluation of a new convective cloud field model: precipitation over the maritime continent, Atmos. Chem. Phys., 7, 409–421, 2007. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Gras, J. L., Jensen, J. B., Okada, K., Ikegami, M., Zaizen, Y., and Makino, Y.: Some optical properties of smoke aerosol in Indonesian and tropical Australia, Geophys. Res. Lett., 26, 1393–1396, 1999. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Jones, A., Roberts, D. L., and Slingo, A.: A climate model study of indirect radiative forcing by anthropogenic aerosols, Nature, 370, 450–453, 1994. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Kessler, E.: On the distribution and continuity of water substance in atmospheric circulation models, Metero. Monographs, Amer. Meteor. Soc., Boston, MA, 10(32), 84 pp., 1969. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Khain, A., Rosenfeld, D., and Pokrovsky, A.: Aerosol impact on the dynamics and microphysics of deep convective clouds, Q. J. Roy. Meteor. Soc., Part: A, 131, 611, 2639–2663, 2005. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Khain, A. and Pokrovsky, A.: Simulation of effects of atmospheric aerosols on deep turbulent convective clouds using a spectral microphysics mixed-phase cumulus cloud model, Part II: Sensitivity study, J. Atmos. Sci., 61, 24, 2983–3001, 2004. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Laird, N. F., Ochs, H. T., Rauber, R. M., et al.: Initial precipitation formation in warm Florida cumulus, J. Atmos. Sci., 57, 22, 3740–3751, 2000. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Langmann, B.: Numerical modelling of regional scale transport and photochemistry directly together with meteorological process, Atmos. Environ., 34, 3585–3598, 2000. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Langmann, B.: A model study of smoke-haze influence on clouds and warm precipitation formation in Indonesia 1997/1998, Atmos. Environ., 41, 6838–6852, 2007. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Langmann, B. and Graf, H.-F.: Indonesian smoke aerosols from peat fires and the contributiuon from volcanic sulfur emissions, Geophys. Res. Lett., 30, 1547–1550, 2003. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Langmann, B. and Heil, A.: Release and dispersion of vegetation and peat fire emissions in the atmosphere over Indonesia 1997/1998, Atmos. Chem. Phys., 4, 2145–2160, 2004. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Lohmann, U. and Feichter, J.: Global indirect aerosol effects: a review, Atmos. Chem. Phys., 5, 715–737, 2005. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Lohmann, U.: Global anthropogenic aerosol effects on convective clouds in ECHAM5-HAM, Atmos. Chem. Phys., 8, 2115–2131, 2008. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Mori, S., Hamada, J.-I., Tauhid, Y.I., Yamanaka, M.D., Okamoto, N., Murata, F., Sakurai, N., Hashiguchi, H., and Sribimawati, T.: Diurnal Land-Sea Rainfall Peak Migration over Sumatera Island, Indonesian Maritime Continent, Observed by TRMM Satellite and Intensive Rawinsonde Soundings, Mon. Weather Rev., 132, 2021–2039, 2004. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Nober, F. J. and Graf, H. F.: A new convective cloud field model based on principles of self-organisation, Atmos. Chem. Phys., 5, 2749–2759, 2005. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Ogura, Y. and Takahashi, T.: Numerical simulation of the life cycle of a thunderstorm cell, Mon. Weather Rev., 99, 895–911, 1971. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Roeckner, E.: Parameterization of cloud radiative properties in the ECHAM4 model, In WCRP workshop &quot;Cloud microphysics parameterizations in global atmospheric circulation models&quot;, 23–35 May 1995, WCRP=90, Kananskis, Canada, 105–116, 1995. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Seifert, A. and Beheng, K. D.: A two-moment cloud microphysics parameterization for mixed-phase clouds, Part II: Deep convective storms, Meteorol. Atmos. Phys., 92, 67–82, doi:10.1007/s00703-005-0113-3, 2006. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Sundquist, H.: A parameterization scheme for non-convective condensation including prediction of cloud water content, Q. J. Roy. Meteor. Soc., 104, 677–690, 1978. </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Tao, W. K, Li, X. W., Khain, A., Matsui, T., Lang, S., and Simpson, J.: Role of atmospheric aerosol concentration on deep convective precipitation: Cloud-resolving model simulations, J. Geophys. Res.-Atmos. 112, D24S18, doi:10.1029/2007JD008728, 2007. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Tiedtke, M.: A comprehensive mass flux scheme for cumulus cloud parameterisation in lagre-scale models, Q. J. Roy. Meteor. Soc., 117, 1779–1800, 1989. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz Uppala, S. M., Kallberg, P. W., Simmons, A. J., et al.: The ERA-40 re-analysis, Q. J. Roy. Meteor. Soc., 131, 2961–3012, 2005. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz van den Heever, S. C., Carrio, G. G., Cotton, W. R., DeMott, P., and Prenni, A. J.: Impacts of Nucleating Aerosol on Florida Storms, Part I: Mesoscale Simulations, J. Atmos. Sci., 63(7), 1752–1775, 2006. </mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple"> % vor jede Referenz van den Heever, S. C. and Cotton, W. R.: Urban Aerosol Impacts on Downwind Convective Storms, J. Appl. Meteorol. Clim., 46(6), 828–850, 2007. </mixed-citation>
</ref>
</ref-list>
</back>
</article>