Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 9, 6055-6075, 2009
© Author(s) 2009. This work is distributed
under the Creative Commons Attribution 3.0 License.
20 Aug 2009
Evolution of stratospheric ozone and water vapour time series studied with satellite measurements
A. Jones1, J. Urban1, D. P. Murtagh1, P. Eriksson1, S. Brohede1, C. Haley2, D. Degenstein3, A. Bourassa3, C. von Savigny4, T. Sonkaew4, A. Rozanov4, H. Bovensmann4, and J. Burrows4 1Department of Radio and Space Science, Chalmers University of Technology, Gothenburg, Sweden
2Department of Earth and Atmospheric Sciences, York University, Toronto, Canada
3University of Saskatchewan, Saskatoon, Canada
4Institute of Environmental Physics, University of Bremen, Germany
Abstract. The long term evolution of stratospheric ozone and water vapour has been investigated by extending satellite time series to April 2008. For ozone, we examine monthly average ozone values from various satellite data sets for nine latitude and altitude bins covering 60° S to 60° N and 20–45 km and covering the time period of 1979–2008. Data are from the Stratospheric Aerosol and Gas Experiment (SAGE I+II), the HALogen Occultation Experiment (HALOE), the Solar BackscatterUltraViolet-2 (SBUV/2) instrument, the Sub-Millimetre Radiometer (SMR), the Optical Spectrograph InfraRed Imager System (OSIRIS), and the SCanning Imaging Absorption spectroMeter for Atmospheric CHartograpY (SCIAMACHY). Monthly ozone anomalies are calculated by utilising a linear regression model, which also models the solar, quasi-biennial oscillation (QBO), and seasonal cycle contributions. Individual instrument ozone anomalies are combined producing an all instrument average. Assuming a turning point of 1997 and that the all instrument average is represented by good instrumental long term stability, the largest statistically significant ozone declines (at two sigma) from 1979–1997 are seen at the mid-latitudes between 35 and 45 km, namely −7.2%±0.9%/decade in the Northern Hemisphere and −7.1%±0.9%/in the Southern Hemisphere. Furthermore, for the period 1997 to 2008 we find that the same locations show the largest ozone recovery (+1.4% and +0.8%/decade respectively) compared to other global regions, although the estimated trend model errors indicate that the trend estimates are not significantly different from a zero trend at the 2 sigma level. An all instrument average is also constructed from water vapour anomalies during 1991–2008, using the SAGE II, HALOE, SMR, and the Microwave Limb Sounder (Aura/MLS) measurements. We report that the decrease in water vapour values after 2001 slows down around 2004–2005 in the lower tropical stratosphere (20–25 km) and has even shown signs of increasing until present. We show that a similar correlation is also seen with the temperature measured at 100 hPa during this same period.

Citation: Jones, A., Urban, J., Murtagh, D. P., Eriksson, P., Brohede, S., Haley, C., Degenstein, D., Bourassa, A., von Savigny, C., Sonkaew, T., Rozanov, A., Bovensmann, H., and Burrows, J.: Evolution of stratospheric ozone and water vapour time series studied with satellite measurements, Atmos. Chem. Phys., 9, 6055-6075, doi:10.5194/acp-9-6055-2009, 2009.
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