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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-9-6005-2009</article-id>
<title-group>
<article-title>Influence of entrainment of CCN on microphysical properties of warm cumulus</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Derksen</surname>
<given-names>J. W. B.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Roelofs</surname>
<given-names>G.-J. H.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Röckmann</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Institute for Marine and Atmospheric Research Utrecht (IMAU), Utrecht University, Utrecht, The Netherlands</addr-line>
</aff>
<pub-date pub-type="epub">
<day>20</day>
<month>08</month>
<year>2009</year>
</pub-date>
<volume>9</volume>
<issue>16</issue>
<fpage>6005</fpage>
<lpage>6015</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
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<abstract>
<p>We use a 1-D cloud model with explicit microphysics and a binned
representation of the aerosol size distribution to investigate the influence
of entrainment of cloud condensation nuclei (CCN) on the microphysical
development of warm cumulus clouds. For a more realistic representation of
cloud drop spectral width, the model separates droplets that grow on aerosol
that is initially present in the cloud from droplets growing on entrained
aerosol. Model results are compared with observations of trade wind cumulus
microphysics from the Rain in Cumulus over the Ocean experiment (RICO,
2004–2005). The results indicate that CCN are entrained throughout the
entire cloud depth, and inside the cloud part of these may be activated.
Compared to a simulation where entrainment of ambient CCN is neglected this
leads to higher cloud droplet number concentrations (CDNC) and a continuous
presence of droplets in the range smaller than ~5 μm that is
consistent with the observations. Cloud dynamics are sensitive to the
entrainment parameter as well as to the applied initial vertical velocity, as
expressed by the liquid water content and cloud top height. However,
simulated cloud drop spectra remain relatively unaffected for the specific
conditions during RICO.</p>
</abstract>
<counts><page-count count="11"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> Albrecht, B A.: Aerosols, cloud microphysics, and fractional cloudiness, Science, 245, 1227–1230, 1989. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> Arabas, S., Pawlowska, H., and Grabowski, W W.: Effective radius and droplet spectral width from in-situ aircraft observations in trade-wind cumuli during RICO, Geophys. Res. Lett., 36, L11803, doi:10.1029/2009GL038257, 2009. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Blyth, A M. and Latham, J.: Airborne studies of the altitudinal variability of the microphysical structure of small, ice-free, Montanan cumulus clouds, Q.\ J. Roy. Meteor. Soc., 116, 1405–1423, doi:10.1002/qj.49711649608, 1990. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> Burnet, F. and Brenguier, J.-L.: Observational study of the entrainment-mixing process in warm convective clouds, J. Atmos. Sci., 64, 1995–2011, 2007. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Charlson, R J., Schwarz, S E., Hales, J M., Cess, R D., Coakley Jr., J. A., Hansen, J E., and Hofmann, D J.: Climate forcing by anthropogenic aerosols, Science, 255, 423–430, 1992. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> Erlick, C., Khain, A., Pinksy, M., and Segal, Y.: The effect of wind velocity fluctuations on drop spectrum broadening in stratocumulus clouds, Atmos.\ Res., 75, 15–45, doi:10.1016/j.atmosres.2004.10.007, 2005. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> Fountoukis, C. and Nenes, A.: Continued development of a cloud droplet formation parameterization for global climate models, J. Geophys. Res., 110, D11212, doi:10.1029/2004JD005591, 2005. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> Gerber, H., Frick, G., Malinowski, S P., Brenguier, J.-L., and Burnet, F.: Holes and entrainment in stratocumulus, J. Atmos. Sci., 62, 443–459, 2005. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Gerber, H., Frick, G., Jensen, J B., and Hudson, J G.: Entrainment, mixing and microphysics in trade-wind cumulus, J. Meteorol. Soc. Jpn., 86A, 87–106, 2008. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Grits, B., Pinsky, M., and Khain, A.: Investigation of small-scale droplet concentration inhomogeneities in a turbulent flow, Meteorol. Atmos. Phys., 92, 191–204, doi:10.1007/s00703-005-0157-4, 2006. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Hänel, G.: The role of aerosol properties during the condensational stage of cloud: A reinvestigation of numerics and microphysics, Beitr. Phys.\ Atmosph., 60, 321–339, 1987. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Heus, T. and Jonker, H. J J.: Subsiding shells around shallow cumulus clouds, J. Atmos. Sci., 65, 1003–1018, doi:10.1175/2007JAS2322.1, 2008. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Heus, T., van Dijk, G., Jonker, H. J J., and van~der Akker, H. E A.: Mixing in shallow cumulus clouds studied by lagrangian particle tracking, J.\ Atmos. Sci., 65, 2581–2597, doi:10.1175/2008JAS2572.1, 2008. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> Hicks, E., Pontikis, C., and Rigaud, A.: Entrainment and mixing processes as related to droplet growth in warm midlatitude and tropical clouds, J.\ Atmos. Sci., 47, 1589–1618, 1990. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Holland, J Z. and Rasmusson, E M.: Measurement of atmospheric mass, energy, and momentum budgets over a 500-kilometer square of tropical ocean, Mon.\ Weather Rev., 101, 44–55, 1973. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Hudson, J G. and Mishra, S.: Relationship between CCN and cloud microphysics variations in clean maritime air, Geophys. Res. Lett., 34, L16804, doi:10.1029/2007GL030044, 2007. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Hudson, J G. and Yum, S S.: Droplet spectral broadening in Marine Stratus, J. Atmos. Sci., 54, 2642–2654, 1997. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Jacobson, M Z.: Fundamentals of Atmospheric Modeling, Cambridge Univ. Press, New York, 1998. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Kreidenweis, S., Walcek, C., Feingold, G., Gong, W., Jacobson, M., Kim, C., Liu, X., Penner, J., Nenes, A., and Seinfeld, J.: Modification of aerosol mass and size distribution due to aqueous phase SO2 oxidation in clouds: Comparisons of several models, J. Geophys. Res., 108, 4213, doi:10.1029/2002JD002697, 2003. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> Krueger, S K., Su, C.-W., and McMurtry, P A.: Modeling entrainment and finescale mixing in cumulus clouds, J. Atmos. Sci., 54, 2697–2712, 1997. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Kulmala, M., Laaksonen, A., Korhonen, P., Ahonen, T., and Baret, J.: The effect of atmospheric nitric acid vapor on cloud condensation nucleus activation, J. Geophys. Res., 98, 22949–22958, 1993. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Lee, S S., Donner, L J., Phillips, V. T J., and Ming, Y.: The dependence of aerosol effects on clouds and precipitation on cloud-system organization, shear and stability, J. Geophys. Res., 113, D16202, doi:10.1029/2007JD009224, 2008. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Leroy, D., Wobrock, W., and Flossmann, A I.: On the influence of the treatment of aerosol particles in different bin microphysical models: A comparison between two different schemes, Atmos. Res., 85, 269–287, doi:10.1016/j.atmosres.2007.01.003, 2007. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> Leroy, D., Wobrock, W., and Flossmann, A I.: The role of boundary layer aerosol particles for the development of deep convective cloud: A high-reolution 3D model with detailed (bin) microphysics applied to CRYSTAL-FACE, Atmos. Res., 91, 62–78, doi:10.1016/j.atmosres.2008.06.001, 2009. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Lohmann, U. and Feichter, J.: Global indirect aerosol effects: a review, Atmos. Chem. Phys., 5, 715–737, 2005. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> Lu, M.-L., Wang, J., Freedman, A., Jonsson, H H., Flagan, R C., McClatchey, R A., and Seinfeld, J H.: Analysis of humidity halos around trade wind cumulus clouds, J. Atmos. Sci., 60, 1041–1059, 2003. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> Meskhidze, N., Nenes, A., Conant, W C., and Seinfeld, J H.: Evolution of a new cloud droplet activation parameterization with in situ data from CRYSTAL-FACE and CSTRIPE, J. Geophys. Res., 110, D16202, doi:10.1029/2004JD005703, 2005. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> Ogura, Y. and Takahashi, T.: Numerical simulation of the life cycle of a thunderstorm cell, Mon. Weather Rev., 99, 895–911, 1971. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> Paluch, I R.: The entrainment mechanism in Colorado cumuli, J. Atmos.\ Sci., 36, 2467–2478, 1979. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> Paluch, I R.: Mixing and the cloud droplet size spectrum: Generalizations from the CCOPE data, J. Atmos. Sci., 43, 1984–1993, 1986. </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> Penner, J E. and Chuang, C C.: The role of entrainment and mixing in altering the relationship between aerosol concentration and cloud drop number concentration, Ninth ARM Science Team Meeting Proceedings, 1999. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> Peter, J R., Blyth, A M., Brooks, B., McQuaid, J B., Lingard, J. J N., and Smith, M H.: On the composition of Caribbean maritime aerosol particles measured during RICO, Q. J. Roy. Meteor. Soc., 134, 1059–1063, doi:10.1002/qj.198, 2008. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> Pinsky, M. and Khain, A.: Fine structure of cloud droplet concentrations as seen from the fast-FSSP measurements. Part II: Results of in situ observations, J. Appl. Meteorol., 42(1), 65–73, 2003. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> Pruppacher, H R. and Klett, J D.: Microphysics of clouds and precipitation, D. Reidel, Dordrecht, 1978. </mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple"> Raga, G B., Jensen, J B., and Baker, M B.: Characteristics of cumulus band clouds off the coast of Hawaii, J. Atmos. Sci., 47, 338–355, 1990. </mixed-citation>
</ref>
<ref id="ref36">
<label>36</label><mixed-citation publication-type="other" xlink:type="simple"> Rauber, R., Stevens, B., Ochs, H., Knight, C., Albrecht, B., Blyth, A., Fairall, C., Jensen, J., Lasher-Trapp, S., Mayol-Bracero, O., Vali, G., Anderson, J., Baker, B., Bandy, A., Burnet, E., Brenguier, J., Brewer, W., Brown, P., Chuang, P., Cotton, W., Girolamo, L D., Geerts, B., Gerber, H., Gške, S., Gomes, L., Heikes, B., Hudson, J., Kollias, P., Lawson, R., Krueger, S., Lenschow, D., Nuijens, L., O&apos;Sullivan, D., Rilling, R., Rogers, D., Siebesma, A., Snodgrass, E., Stith, J., Thornton, D., Tucker, S., Twohy, C., and Zuidema, P.: Rain In Shallow Cumulus over the Ocean: The RICO Campaign, B. Am. Meteorol. Soc., 88, 1912–1928, 2007. </mixed-citation>
</ref>
<ref id="ref37">
<label>37</label><mixed-citation publication-type="other" xlink:type="simple"> Roelofs, G.-J. and Jongen, S.: A model study of the influence of aerosol size and chemical properties on precipitation formation in warm clouds, J. Geophys. Res., 109, D22201, doi:10.1029/2004JD004779, 2004. </mixed-citation>
</ref>
<ref id="ref38">
<label>38</label><mixed-citation publication-type="other" xlink:type="simple"> Roelofs, G.-J. and Kamphuis, V.: Cloud processing, cloud evaporation and Angström exponent, Atmos. Chem. Phys., 9, 71–80, 2009. </mixed-citation>
</ref>
<ref id="ref39">
<label>39</label><mixed-citation publication-type="other" xlink:type="simple"> Roesner, S., Flossmann, A I., and Pruppacher, H R.: The effect on the evolution of the drop spectrum in clouds of the preconditioning of air by successive convective elements, Q. J. Roy. Meteor. Soc., 116, 1389–1403, doi:10.1002/qj.49711649607, 1990. </mixed-citation>
</ref>
<ref id="ref40">
<label>40</label><mixed-citation publication-type="other" xlink:type="simple"> Segal, Y., Pinsky, M., Khain, A., and Erlick, C.: Thermodynamic factors influencing bimodal spectrum formation in cumulus clouds, Atmos. Res., 66, 43–64, 2003. </mixed-citation>
</ref>
<ref id="ref41">
<label>41</label><mixed-citation publication-type="other" xlink:type="simple"> Siebesma, A P. and Cuijpers, J. W M.: Evaluation of parametric assumptions for shallow cumulus convection, J. Atmos. Sci., 52, 650–666, 1995. </mixed-citation>
</ref>
<ref id="ref42">
<label>42</label><mixed-citation publication-type="other" xlink:type="simple"> Siebesma, A P., Bretherton, C S., Brown, A., Chlond, A., Cuxart, J., Duynkerke, P G., Jiang, H., Khairoutdinov, M., Lewellen, D., Moeng, C.-H., Sanchez, E., Stevens, B., and Stevens, D E.: A large eddy simulation intercomparison study of shallow cumulus convection, J. Atmos. Sci., 60, 1201–1219, 2003. </mixed-citation>
</ref>
<ref id="ref43">
<label>43</label><mixed-citation publication-type="other" xlink:type="simple"> Solomon, S., Qin, D., Manning, M., Alley, R B., Berntsen, T., Bindoff, N L., Chen, Z., Chidthaisong, A., Gregory, J M., Hegerl, G C., Heimann, H., Hewitson, B., Hoskins, B J., Joos, F., Jouzel, J., Kattsov, V., Lohmann, U., Matsuno, T., Molina, M., Nichollsand, N., Overpeck, J., Raga, G., Ramaswamy, V., Ren, J., Rusticucci, M., Somerville, R., Stocker, T F., Whetton, P. A. W R., and Wratt, D.: Technical Summary, in: Climate Change 2007: The Physical Science Basis. Contribution of Working Group I to the Fourth Assessment Report of the Intergovernmental Panel on Climate Change, Cambridge Univ. Press, Cambridge, United Kingdom and New York, NY, USA, 2007. </mixed-citation>
</ref>
<ref id="ref44">
<label>44</label><mixed-citation publication-type="other" xlink:type="simple"> Stevens, B., Ackerman, A S., Albrecht, B A., Brown, A R., Chlond, A., Cuxart, J., Duynkerke, P G., Lewellen, D C., Macvean, M K., Neggers, R. A J., Sanchez, E., Siebesma, A P., and Stevens, D E.: Simulation of trade wind cumuli under a strong inversion, J. Atmos. Sci., 58, 1870–1891, 2001. </mixed-citation>
</ref>
<ref id="ref45">
<label>45</label><mixed-citation publication-type="other" xlink:type="simple"> Su, C.-W., Krueger, S K., McMurtry, P A., and Austin, P H.: Linear eddy modeling of droplet spectral evolution during entrainment and mixing in cumulus clouds, Atmos. Res., 47–48, 41–58, 1998. </mixed-citation>
</ref>
<ref id="ref46">
<label>46</label><mixed-citation publication-type="other" xlink:type="simple"> Takahashi, T.: Warm rain, giant nuclei and chemical balance – a numerical model, J. Atmos. Sci., 33, 269–286, 1976. </mixed-citation>
</ref>
<ref id="ref47">
<label>47</label><mixed-citation publication-type="other" xlink:type="simple"> Twomey, S.: The influence of pollution on the shortwave albedo of clouds, J.\ Atmos. Sci., 34, 1149–1154, 1977. </mixed-citation>
</ref>
<ref id="ref48">
<label>48</label><mixed-citation publication-type="other" xlink:type="simple"> Warner, J.: On steady-state one-dimensional models of cumulus convection, J.\ Atmos. Sci., 27, 1035–1040, 1970. </mixed-citation>
</ref>
</ref-list>
</back>
</article>