Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 9, 5905-5919, 2009
© Author(s) 2009. This work is distributed
under the Creative Commons Attribution 3.0 License.
19 Aug 2009
Quantifying transport into the lowermost stratosphere using simultaneous in-situ measurements of SF6 and CO2
H. Bönisch1, A. Engel1, J. Curtius1, Th. Birner2, and P. Hoor3 1Institute for Atmospheric and Environmental Sciences, Goethe University Frankfurt, Frankfurt am Main, Germany
2Department of Atmospheric Science, Colorado State University, Fort Collins, CO, USA
3Institute for Atmospheric Physics, University of Mainz, Germany
Abstract. The seasonality of transport and mixing of air into the lowermost stratosphere (LMS) is studied using distributions of mean age of air and a mass balance approach, based on in-situ observations of SF6 and CO2 during the SPURT (Spurenstofftransport in der Tropopausenregion, trace gas transport in the tropopause region) aircraft campaigns. Combining the information of the mean age of air and the water vapour distributions we demonstrate that the tropospheric air transported into the LMS above the extratropical tropopause layer (ExTL) originates predominantly from the tropical tropopause layer (TTL). The concept of our mass balance is based on simultaneous measurements of the two passive tracers and the assumption that transport into the LMS can be described by age spectra which are superposition of two different modes. Based on this concept we conclude that the stratospheric influence on LMS composition is strongest in April with extreme values of the tropospheric fractions (α1) below 20% and that the strongest tropospheric signatures are found in October with α1 greater than 80%. Beyond the fractions, our mass balance concept allows us to calculate the associated transit times for transport of tropospheric air from the tropics into the LMS. The shortest transit times (<0.3 years) are derived for the summer, continuously increasing up to 0.8 years by the end of spring. These findings suggest that strong quasi-horizontal mixing across the weak subtropical jet from summer to mid of autumn and the considerably shorter residual transport time-scales within the lower branch of the Brewer-Dobson circulation in summer than in winter dominates the tropospheric influence in the LMS until the beginning of next year's summer.

Citation: Bönisch, H., Engel, A., Curtius, J., Birner, Th., and Hoor, P.: Quantifying transport into the lowermost stratosphere using simultaneous in-situ measurements of SF6 and CO2, Atmos. Chem. Phys., 9, 5905-5919, doi:10.5194/acp-9-5905-2009, 2009.
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