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<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics</journal_title>
		<journal_url>www.atmos-chem-phys.net</journal_url>
		<issn>1680-7316</issn>
		<eissn>1680-7324</eissn>
		<volume_number>8</volume_number>
		<issue_number>21</issue_number>
		<publication_year>2008</publication_year>
	</journal>
	<doi>10.5194/acp-8-6405-2008</doi>
	<article_url>http://www.atmos-chem-phys.net/8/6405/2008/</article_url>
	<abstract_html>http://www.atmos-chem-phys.net/8/6405/2008/acp-8-6405-2008.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys.net/8/6405/2008/acp-8-6405-2008.pdf</fulltext_pdf>
	<start_page>6405</start_page>
	<end_page>6437</end_page>
	<publication_date>2008-11-11</publication_date>
	<article_title content_type="html">Influence of future air pollution mitigation strategies on total aerosol radiative forcing</article_title>
	<authors>
		<author numeration="1" affiliations="1,6">
			<name>S. Kloster</name>
		</author>
		<author numeration="2" affiliations="1">
			<name>F. Dentener</name>
			<email>frank.dentener@jrc.it</email>
		</author>
		<author numeration="3" affiliations="2">
			<name>J. Feichter</name>
		</author>
		<author numeration="4" affiliations="1">
			<name>F. Raes</name>
		</author>
		<author numeration="5" affiliations="1">
			<name>J. van Aardenne</name>
		</author>
		<author numeration="6" affiliations="2">
			<name>E. Roeckner</name>
		</author>
		<author numeration="7" affiliations="3">
			<name>U. Lohmann</name>
		</author>
		<author numeration="8" affiliations="4">
			<name>P. Stier</name>
		</author>
		<author numeration="9" affiliations="5">
			<name>R. Swart</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">European Commission, Institute for Environment and Sustainability, Ispra (VA), Italy</affiliation>
		<affiliation numeration="2" content_type="html">Max Planck Institute for Meteorology, Hamburg, Germany</affiliation>
		<affiliation numeration="3" content_type="html">Institute of Atmospheric and Climate Science, ETH Zuerich, Switzerland</affiliation>
		<affiliation numeration="4" content_type="html">University of Oxford, Atmospheric, Oceanic and Planetary Physics, Oxford, UK</affiliation>
		<affiliation numeration="5" content_type="html">EEA European Topic Centre on Air and Climate Change (ETC/ACC), MNP, Bilthoven, The Netherlands</affiliation>
		<affiliation numeration="6" content_type="html">now at: Cornell University, Ithaca, NY, USA</affiliation>
	</affiliations>
	<abstract content_type="html">We apply different aerosol and aerosol precursor emission scenarios reflecting possible future
control strategies for air pollution in the ECHAM5-HAM model, and simulate the resulting effect
on the Earth&apos;s radiation budget. We use two opposing future mitigation strategies for the year 2030: one
in which emission reduction legislation decided in countries throughout the world are effectively
implemented (current legislation; CLE 2030) and  one in which all technical options for emission reductions
are being implemented independent of their cost (maximum feasible reduction; MFR 2030).

&lt;br&gt;&lt;br&gt;
We consider the direct, semi-direct and indirect radiative effects of aerosols. The total anthropogenic
aerosol radiative forcing defined as the difference in the top-of-the-atmosphere radiation between 2000 and pre-industrial
times amounts to &amp;minus;2.00 W/m&lt;sup&gt;2&lt;/sup&gt;. In the future this negative global annual mean aerosol radiative forcing will only
slightly change (+0.02 W/m&lt;sup&gt;2&lt;/sup&gt;) under the &quot;current legislation&quot; scenario. Regionally, the effects are much larger: e.g. over
Eastern Europe radiative forcing would increase by +1.50 W/m&lt;sup&gt;2&lt;/sup&gt; because of successful aerosol reduction policies, whereas
over South Asia it would decrease by &amp;minus;1.10 W/m&lt;sup&gt;2&lt;/sup&gt; because of further growth of emissions.  A &quot;maximum feasible reduction&quot; of
aerosols and their precursors would lead to an increase of the global annual mean aerosol radiative forcing by +1.13 W/m&lt;sup&gt;2&lt;/sup&gt;.
Hence, in the latter case, the present day negative anthropogenic aerosol forcing could be more than halved by 2030 because of aerosol
reduction policies and climate change thereafter will be to a larger extent be controlled by greenhouse gas emissions.

&lt;br&gt;&lt;br&gt;
We combined these two opposing future mitigation strategies for a number of experiments focusing on different sectors and regions.
In addition, we performed sensitivity studies to estimate the importance of future changes in oxidant concentrations and the
importance of the aerosol microphysical coupling within the range of expected future changes. For changes in oxidant concentrations
caused by future air pollution mitigation, we do not find a significant effect for the global annual mean radiative aerosol forcing.
In the extreme case of only abating SO&lt;sub&gt;2&lt;/sub&gt; or carbonaceous emissions to a maximum feasible extent, we find deviations from
additivity for the radiative forcing over anthropogenic source regions up to 10% compared to an experiment abating both at the same time.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Albrecht, B A.: Aerosols, cloud microphysics, and fractional cloudiness, Science, 245, 1227–1230, 1989. </reference>
		<reference numeration="2" content_type="text"> Andreae, M.: Atmospheric aerosols versus greenhouse gases in the twenty first century, Philos. T. R. Soc. A, 365, 1915–1923, doi:10.1098/rsta.2007.2051, 2007. </reference>
		<reference numeration="3" content_type="text"> Ångstroem, A.: Atmospheric turbitidy, global illumination and planetary albedo of the earth, Tellus, 14, 435–450, 1962. </reference>
		<reference numeration="4" content_type="text"> Barth, M C., Rasch, P J., Kiehl, J T., Benkovitz,C M., and Schwartz, S E.: Sulfur chemistry in the National Center for Atmospheric Research Community Climate Model: Description, evaluation, features, and sensitivity to aqueous chemistry, J. Geophys. Res., 105, 1387–1415, 2000. </reference>
		<reference numeration="5" content_type="text"> Bond, T C., Streets, D G., Yarber, K. F., Nelson, S M., Woo, J H., and Klimont, Z.: A technology-based global inventory of black and organic carbon emissions from combustion, J. Geophys. Res., 109, D14203, doi:10.1029/2003JD003697, 2004. </reference>
		<reference numeration="6" content_type="text"> Brasseur, G P. and Roeckner, E.: Impact of improved air quality on the future evolution of climate, Geophys. Res. Lett., 32, L23704, doi:10.1029/2005GL023902, 2005. </reference>
		<reference numeration="7" content_type="text"> Cagnazzo, C., Manzini, E., Giorgetta, M A., Forster, P M. D. F., and Morcrette, J J.: Impact of an improved shortwave radiation scheme in the MAECHAM5 general circulation model, Atmos. Chem. Phys., 7, 2503–2515, 2007. </reference>
		<reference numeration="8" content_type="text"> Cofala, J., Amann, M., Klimont, Z., Kupiainen, K., and Höglund-Isaksson, L.: Scenarios of global anthropogenic emissions of air pollutants and methane until 2030, Atmos. Environ., 41(38), 8486–8499, doi:10.1016/j.atmosenv.2007.07.010, 2007. </reference>
		<reference numeration="9" content_type="text"> Denman, K. L., Brasseur, G., Chidthaisong, A., Ciais, P., Cox, P. M., Dickinson, R. E., Hauglustaine, D., Heinze, C., Holland, E., Jacob, D., Lohmann, U., Ramachandran, S., da Silva Dias, P. L., Wofsy, S. C., and Zhang, X.: Couplings between changes in the climate system and biogeochemistry, in :Climate Change 2007: The Physical Science Basis. Contribution of working group I to the fourth Assessment Report on the Intergovernmental Panel on Climate Change, edited by: Solomon, S., Wuin, D., Manning, M., Chen, Z., Marquis, M., Averyt, K., Tignor, M., and Miller, H., Cambridge University Press, Cambrige, United Kingdom and New York, NY, USA, 2007. </reference>
		<reference numeration="10" content_type="text"> Dentener, F., Peters, W., Krol, M., Weele, M. V., Bergamaschi, P., and Lelieveld, J.: Inter-annual-variability and trend of \chemCH_4 lifetime as a measure for OH changes in the 1979–1993 time period, J. Geophys. Res., 108(D5), 4442, doi:10.1029/2002JD002916, 2003. </reference>
		<reference numeration="11" content_type="text"> Dentener, F., Stevenson, D., Cofala, J., Mechler, R., Amann, M, Bergamaschi, P., Raes, F., and Derwent, R: The impact of air pollutant and methane emissions controls on tropospheric ozone and radiative forcing: CTM calculations for the period 1990–2030, Atmos. Chem. Phys., 5, 1731–1755, 2005. </reference>
		<reference numeration="12" content_type="text"> Dentener, F., Kinne, S., Bond, T., Boucher, O., Cofala, J., Generoso, S., Ginoux, P., Gong, S., Hoelzemann, J J., Ito, A., Marelli, L., Penner, J E., Putaud, J.-P., Textor, C., Schulz, M., van~der Werf, G R., and Wilson, J.: Emissions of primary aerosol and precursor gases in the years 2000 and 1750 prescribed data-sets for AeroCom, Atmos. Chem. Phys., 6, 4321–4344, 2006a. </reference>
		<reference numeration="13" content_type="text"> Dentener, F., Stevenson, D., Ellingsen, K., Noije, T V., Schultz, M., Amann, M., Atherton, C., Bell, N., Bergmann, D., Bey, I., Bouwman, L., Butler, T., Cofala, J., Collins, B., Drevet, J., Doherty, R., Eickhout, B., Eskes, H., Fiore, A., Gauss, M., Hauglustaine, D., Horowitz, L., Isaksen, I., Josse, B., Lawrence, M., Krol, M., Lamarque, J., Montanaro, V., Mueller, J., Peuch, V., Pitari, G., Pyle, J., Rast, S., Rodriguez, J., Sanderson, M., Savage, N., Shindell, D., Strahan, S., Szopa, S., Sudo, K., Dingenen, R V., Wild, O., and Zeng, G.: The Global Atmospheric Environment for the Next Generation, Environ. Sci. Technol., 40, 3586–3594, 2006b. </reference>
		<reference numeration="14" content_type="text"> EPA: National Air Pollutant Emission Trends, 1900–1998, U.S. Environmental Protection Agency, Office of Air Quality Planning and Standards, http://www.epa.gov/ttn/chief/trends/trends98/trends98.pdf, 2000. </reference>
		<reference numeration="15" content_type="text"> Eyring, V., Koehler, H., Lauer, A., and Lemper, B.: Emissions from international shipping: 2. Impact of future technologies on scenarios until 2050, J. Geophys. Res., 110, D17306, doi:10.1029/2004JD005620, 2005. </reference>
		<reference numeration="16" content_type="text"> Feichter, J., Kjellstrom, E., Rodhe, H., Dentener, F., Lelieveld, J., and Roelofs, G.-F.: Simulation of the tropospheric sulfur cycle in a global climate model, Atmos. Environ., 30(10–11), 1693–1707, 1996. </reference>
		<reference numeration="17" content_type="text"> Feichter, J., Roeckner, E., Lohmann, U., and Liepert, B.: Nonlinear aspects of the climate response to greenhouse gas and aerosol forcing, J. Climate, 17(12), 2384–2398, 2004. </reference>
		<reference numeration="18" content_type="text"> Forster, P., Ramawamy, V., Artaxo, P., Berntsen, T., Betts, R., Fahey, D., Haywood, J., Lean, J., Lowe, D., Myhre, G., Nganga, J., Prinn, R., Raga, G., Schulz, M., and Dorland, R V.: Changes in Atmospheric Constituents and in Radiative Forcing, in: Climate Change 2007: The Physical Science Basis. Contribution of working group I to the fourth Assessment Report on the Intergovernmental Panel on Climate Change, edited by: Solomon, S., Wuin, D., Manning, M., Chen, Z., Marquis, M., Averyt, K., Tignor, M., and Miller, H., Cambridge University Press, Cambrige, United Kingdom and New York, NY, USA, 2007. </reference>
		<reference numeration="19" content_type="text"> Graf, H.-F., Feichter, J., and Langmann, B.: Volcanic sulfur emissions: Estimates of source strength and its contribution to the global sulfate distribution, J. Geophys. Res., 102, 10 727–10 738, 1997. </reference>
		<reference numeration="20" content_type="text"> Hansen, J., Sato, M., and Ruedy, R.: Radiative forcing and climate response, J. Geophys. Res., 102, 6831–6864, 1997. </reference>
		<reference numeration="21" content_type="text"> Horowitz, L W., Walters, S., Mauzerall, D L., Emmons, L K., Rasch, P J., Granier, C., Tie, X X., Lamarque, J F., Schultz, M G., Tyndall, G S., Orlando, J J., and Brasseur, G P.: A global simulation of tropospheric ozone and related tracers: Description and evaluation of MOZART, Version 2, J. Geophys. Res., 108(D24), 4784, doi:10.1029/2002JD002853, 2003. </reference>
		<reference numeration="22" content_type="text"> IPCC, Climate change 2001: The scientific basis, Cambridge University Press, J T Houghton, 881 pp., 2001. </reference>
		<reference numeration="23" content_type="text"> Jeuken, A., Siegmund, P., Heijboer, L., Feichter, J., and Bengtsson, L.: On the potential of assimilating meteorological analyses in a global climate model for the purpose of model validation, J. Geophys. Res., 101, 16 939–16 950, doi:10.1029/96JD01218, 1996. </reference>
		<reference numeration="24" content_type="text"> Kettle, A J. and Andreae, M O.: Flux of dimethylsulfide from the oceans: A comparison of updated data sets and flux models, J. Geophys. Res., 105(D22), 26 793–26 808, 2000. </reference>
		<reference numeration="25" content_type="text"> Khairoutdinov, M. and Kogan, Y.: A new cloud physics parameterization in a large-eddy simulation model of marine stratocumulus, Mon. Weather Rev., 128(1), 229–243, 2000. </reference>
		<reference numeration="26" content_type="text"> Kloster, S., Six, K., Feichter, j., Maier-Reimer, E., Roeckner, E., Wetzel, P., Stier, P., and Esch, M.: Response of dimethylsulfide (DMS) in the ocean and atmosphere to global warming, J. Geophys. Res., 112, G03005, doi:10.1029/2006JG000224, 2007. </reference>
		<reference numeration="27" content_type="text"> Koch, D., Bond, T., Streets, D., Unger, N., and van~der Werf, G.: Global impacts of aerosols from particular source regions and sectors, J. Geophys. Res., 112, D02205, doi:10.1029/2005JD007024, 2007. </reference>
		<reference numeration="28" content_type="text"> Koch, D., Bond, T., Streets, D., and Unger, N: Linking future aerosol radiative forcing to shifts in source activities, Geophys. Res. Lett., 34, doi:10.1029/2006GL028360, 2007b. </reference>
		<reference numeration="29" content_type="text"> Lin, H. and Leaitch, R.: Development of an in-cloud aerosol activation parameterization for climate modelling, in: WMO workshop on measurements of cloud properties for forcast of weather, edited by: W M. Organization, 328–335, Geneva, 1997. </reference>
		<reference numeration="30" content_type="text"> Lin, S J. and Rood, R B.: Multidimensional flux-form semi-lagrangian transport schemes, Mon. Weather Rev., 124(9), 2046–2070, 1996. </reference>
		<reference numeration="31" content_type="text"> Lohmann, U. and Feichter, J.: Impact of sulfate aerosols on albedo and lifetime of clouds: A sensitivity study with the ECHAM4 GCM, J. Geophys. Res., 102(D12), 13 685–13 700, 1997. </reference>
		<reference numeration="32" content_type="text"> Lohmann, U., Feichter, J., Chuang, C. C., and Penner, J. E.: Prediction of the number of cloud droplets in the ECHAM GCM, J. Geophys. Res., 104(D20), 24 557–24 563, 1999. </reference>
		<reference numeration="33" content_type="text"> Lohmann, U., Stier, P., Hoose, C., Ferrachat, S., Kloster, S., Roeckner, E., and Zhang, J.: Cloud microphysics and aerosol indirect effects in the global climate model ECHAM5-HAM, Atmos. Chem. Phys., 7, 3425–3446, 2007. </reference>
		<reference numeration="34" content_type="text"> Mahowald, N., Lamarque, J.-F., Tie, X., and Wolff, E.: Sea salt aerosol response to climate change: last glacial maximum, pre-industrial and doubled carbon dioxide climates, J. Geophys. Res., 111, D05303, doi:10.1029/2005JD006,459, 2006a. </reference>
		<reference numeration="35" content_type="text"> Mahowald, N., Muhs, D., Levis, S., Rasch, P., Yoshioka, M., Zender, C., and Luo, C.: Change in atmospheric mineral aerosols in response to climate: Last glacial period, preindustrial, modern, and doubled carbon dioxide climates, J. Geophys. Res., 111, D10202, doi:10.1029/2005JD006653, 2006b. </reference>
		<reference numeration="36" content_type="text"> Menon, S., Unger, N., Koch, D., Francis, J., Garret, T., Sednev, I., Shindell, D., and Street, D.: Aerosol climate effects and air quality impacts from 1980 to 2030, Environ. Res. Lett., 3, 024004, doi:10.1088/1748-9326/3/2/024004, 2008. </reference>
		<reference numeration="37" content_type="text"> Morcrette, J J., Clough, S A., Mlawer, E. J., and Iacono, M. J.: Impact of a validated radiative transfer scheme, RRTM, on the ECMWF model climate and 10-day forecasts, Technical Memorandum 252, ECMWF, Reading, UK, 1998. </reference>
		<reference numeration="38" content_type="text"> Nakicenovic, N., Alcamo, J., Davis, G., de~Vries, B., Fenhann, J., Gaffin, S., Gregory, K., Gruebler, A., Jung, T., Kram, T., Rovere, E L., Michaelis, L., Mori, S., Morita, T., Pepper, W., Pitcher, H., Price, L., Riahi, K., Roehrl, A., Rogner, H.-H., Sankovski, A., Schlesinger, M., Shukla, P., Smith, S., Swart, R., van Rooijen, S., Victor, N., and Dadi, Z.: Special Report on Emissions Scenarios, in: Contribution to the Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge, UK, 2000. </reference>
		<reference numeration="39" content_type="text"> Nightingale, P D., Malin, G., Law, C. S., Watson, A. J., Liss, P. S., Liddicoat, M. J., Boutin, J., and Upstill-Goddard, R. C.: In situ evaluation of air-sea gas exchange parameterizations using novel conservative and volatile tracers, Global Biogeochem. Cy., 14(1), 373–387, 2000. </reference>
		<reference numeration="40" content_type="text"> Nordeng, T E.: Extended versions of the convective parameterization scheme at ECMWF and their impact on the mean and transient activity of the model in the tropics, Technical Memorandum 206, ECMWF, Reading, UK, 1994. </reference>
		<reference numeration="41" content_type="text"> Olivier, J. and Berdowski, J.: Global emission sources and sinks, chap. The Climate System, Swets and Zeitlinger Publishers, Lisse, The Netherlands, 2001. </reference>
		<reference numeration="42" content_type="text"> Olivier, J., Berdowski, J., Peters, J., Bakker, J., Visschedijk, A., and Bloos, J.: Applications of edgar including a description of edgar v3.0: reference database with trend data for 1970–1995, NRP report 410200 051, RIVM, Bilthoven, The Netherlands, 2002. </reference>
		<reference numeration="43" content_type="text"> Pham, M., Boucher, O., and Hauglustaine, D.: Changes in atmospheric sulfur burdens and concentrations and resulting radiative forcings under IPCC SRES emission scenarios for 1990–2100, J. Geophys. Res., 110, D06112, doi:10.1029/2004JD005125, 2005. </reference>
		<reference numeration="44" content_type="text"> Pozzoli, L., Bey, I., Rast, J., Schultz, M., Stier, P., and Feichter, J.: Trace gas and aerosol interactions in the fully coupled model of aerosol-chemistry-climate ECHAM5-HAMMOZ, PART1: Model descripstion and insights from the spring 2001 TRACE-P experiment, J. Geophys. Res., 113, D07308, doi:10.1029/2007JD009007, 2007. </reference>
		<reference numeration="45" content_type="text"> Reddy, M., Boucher, O., and Balkanski Y.: Aerosol optical depths and direct radiative perturbations by species and source type, Geophys. Res. Lett., 32(12), L12803, doi:10.1029/2004GL021743, 2005. </reference>
		<reference numeration="46" content_type="text"> Riahi, K. and Roehl, R.: Greenhouse Gas Emissions in Dynamis-as-Usual Scenario of Economic and Energy Development, Technical Forcasting and Social Change 63, 175–205, North Holland, 2005. </reference>
		<reference numeration="47" content_type="text"> Roeckner, E., Baeuml, G., Bonventura, L., Brokopf, R., Esch, M., Giorgetta, M., Hagemann, S., Kirchner, I., Kornblueh, L., Manizini, E., Rhodin, A., Schlese, U., Schulzweida, U., and Tompkins, A.: The atmospheric general circulation model ECHAM5, Part I: Model description, Report 349, Max Planck Institute for Meteorology, Hamburg, Germany, http://www.mpimet.mpg.de, 2003. </reference>
		<reference numeration="48" content_type="text"> Roelofs, G.-J., Lelieveld, J., and Ganzeveld, L.: Simulation of global sulfate distribution and the influence on effective cloud drop radii with a coupled photochemistry sulfur cycle model, Tellus B, 50(3), 224–242, 1998. </reference>
		<reference numeration="49" content_type="text"> Schulz, M., de~Leeuw, G., and Balkanski, Y.: Sea salt aerosol source functions and emissions, in: Emission of atmospheric trace compounds, edited by: Granier, C., Artaxo, P., and Reeves, C., Ed. Kluwer, 333–359, 2004. </reference>
		<reference numeration="50" content_type="text"> Shindell, D T, Faluvegi, G., Bauers, S E., Koch, D., Unger, N., Menon, S., Miller, R L., Schmidt, G A., and Streets, D.: Climate response to projected changes in short-lived species under an A1B scenario from 2000–2050 in the GISS climate model, J. Geophys. Res., 112, D20103, doi:10.1029/2007JD008753, 2007.  </reference>
		<reference numeration="51" content_type="text"> Shindell, D T., Levy, H., Schwarzkopf, M D., Horrowitz, L W., Lamarque, J F., and Faluvegi, G.: Multimodel projections of climate change from short-lived emissions due to human activities, J. Geophys. Res., 113, D11109, doi:10.1029/2007JD009152, 2008. </reference>
		<reference numeration="52" content_type="text"> Stier, P., Feichter, J., Kinne, S., Kloster, S., Vignati, E., Wilson, J., Ganzeveld, L., Tegen, I., Werner, M., Balkanski, Y., Schulz, M., Boucher, O., Minikin, A., and Petzold, A.: The aerosol-climate model ECHAM5-HAM, Atmos. Chem. Phys., 5, 1125–1156, 2005. </reference>
		<reference numeration="53" content_type="text"> Stier, P., Feichter, J., Kloster, S., Vignati, E., and Wilson, J.: Emission-induced nonlinearities in the global aerosol system – results from the ECHAM5-HAM aerosol-climate model, J. Climate, 19(16), 3845–3861, 2006a. </reference>
		<reference numeration="54" content_type="text"> Stier, P., Seinfeld, J., Kinne, S., Feichter, J., and Boucher, O.: Impact of non-absorbing anthropogenic aerosols on clear-sky atmospheric absorption, J. Geophys. Res., 111, D18201, doi:10.1029/2006JD007147, 2006b. </reference>
		<reference numeration="55" content_type="text"> Stier, P., Feichter, J., Roeckner, E., Kloster, S., and Esch, M.: The evolution of the global aerosol system in a transient climate simulation from 1860 to 2100, Atmos. Chem. Phys., 6, 2389–2399, 2006c. </reference>
		<reference numeration="56" content_type="text"> Streets, D., Bond, T., Lee, T., and Jang, C.: On the future of carbonaceous aerosol emissions, J. Geophys. Res., 109, D24212, doi:10.1029/2004JD004902, 2004. </reference>
		<reference numeration="57" content_type="text"> Sundquist, H., Berge, E., and Kristiansson, J. E.: Condensation and cloud parameterization studies with a mesoscale numerical weather prediction model, Mon. Weather Rev., 117, 1657–1614, 1989. </reference>
		<reference numeration="58" content_type="text"> Takemura, T., Nakajima, T., Dubovik, O., Holben, B. N., and Kinne, S.: Single-scattering albedo and radiative forcing of various aerosol species with a global three-dimensional model, J. Climate, 15, 333–352, 2002. </reference>
		<reference numeration="59" content_type="text"> Tegen, I., Harrison, S P., Kohfeld, K., Prentice, I. C., Coe, M., and Heimann, M.: Impact of vegetation and preferential source areas on global dust aerosol: Results from a model study, J. Geophys. Res., 107(D21), 4576, doi:10.1029/2001JD000963, 2002. </reference>
		<reference numeration="60" content_type="text"> Tegen, I., Werner, M., Harrison, S. P., and Kohfeld, K. E.: Relative importance of climate and land use in determining present and future global soil dust emission, Geophys. Res. Lett., 31(5), L05105, doi:10.1029/2003GL019216, 2004. </reference>
		<reference numeration="61" content_type="text"> Tiedtke, M.: A comprehensive mass flux scheme for cumulus parameterization in large-scale models, Mon. Weather Rev., 117(8), 1779–1800, 1989. </reference>
		<reference numeration="62" content_type="text"> Twomey, S.: The influence of pollution on the shortwave albedo of clouds, J. Atmos. Sci., 34, 1249–1152, 1977. </reference>
		<reference numeration="63" content_type="text"> Unger, N., Shindell, D., Koch, D., and Streets, D.: Cross influence of ozone and sulfate precursor emission changes on air quality and climate, P. Natl. Acad. Sci. USA, 97, 9875–9880, 2006. </reference>
		<reference numeration="64" content_type="text"> Unger, N., Shindell, D., Koch, D., and Streets, D.: Air pollution radiative forcing from specific emissions sectors at 2030, J. Geophys. Res., 113, D02306, doi:10.1029/10.1029/2007JD008683, 2008.  </reference>
		<reference numeration="65" content_type="text"> Uppala, S. M., Kallberg, P. W., Simmons, A. J., Andrae, U., Da Costa Bechtold, V., Fiorino, M., Gibson, J. K., Haseler, J., Hernandez, A., Kelly, G. A., Li, X., Onogi, K., Saarinen, S., Sokka, N., Allan, R. P., Andersson, E., Arpe, K., Balmaseda, M. A., Beljaars, A. C. M., Van De Berg, L., Bidlot, J., Bormann, N., Caires, S., Chevallier, F., Dethof, A., Dragosavac, M., Fisher, M., Fuentes, M., Hagemann, S., Holm, E., Hoskins, B. J., Isaksen, L., Janssen, P. A. E. M., Jenne, R., Mcnally, A. P., Mahfouf, J.-F., Morcrette, J.-J., Rayner, N. A., Saunders, R. W., Simon, P., Sterl, A., Trenberth, K. E., Untch, A., Vasiljevic, D., Viterbo, P., and Woollen, J.: The ERA-40 re-analysis, Q. J. Roy. Meteor. Soc., 131, 2961–3012 , 2005. </reference>
		<reference numeration="66" content_type="text"> Vestreng, V., Myhre, G., Fagerlil, H., Reis, S., and Tarrasón, L.: Twenty-five years of continuous sulphur dioxide emission reduction in europe, Atmos. Chem. Phys., 7, 3663–3681, 2007. </reference>
		<reference numeration="67" content_type="text"> Vignati, E., Wilson, J., and Stier, P.: An efficient size-resolved aerosol microphysics module for large-scale aerosol transport models, J. Geophys. Res., 109(D22), D22202, doi:10.1029/2003JD004485, 2004. </reference>
		<reference numeration="68" content_type="text"> WHO: Health Aspects of Air Pollution with Particulate Matter, Ozone and Nitrogen Dioxide, Report on a WHO Working group, Bonn, Germany, www.euro.who.int/document/e79097.pdf, 2003. </reference>
	</references>
</article>

