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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-7-1313-2007</article-id>
<title-group>
<article-title>Stratospheric dryness: model simulations and satellite observations</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Lelieveld</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Brühl</surname>
<given-names>C.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Jöckel</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Steil</surname>
<given-names>B.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Crutzen</surname>
<given-names>P. J.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Fischer</surname>
<given-names>H.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Giorgetta</surname>
<given-names>M. A.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Hoor</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Lawrence</surname>
<given-names>M. G.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Sausen</surname>
<given-names>R.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Tost</surname>
<given-names>H.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Max Planck Institute for Chemistry, J. J. Becherweg 27, 55128 Mainz, Germany</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Scripps Institution of Oceanography, UCSD, La Jolla, CA 92093-0221, USA</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Max Planck Institute for Meteorology, Bundesstrasse 53, 20146 Hamburg, Germany</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>DLR-Institut für Physik der Atmosphäre, Oberpfaffenhofen, 82234 Wessling, Germany</addr-line>
</aff>
<pub-date pub-type="epub">
<day>27</day>
<month>02</month>
<year>2007</year>
</pub-date>
<volume>7</volume>
<issue>5</issue>
<fpage>1313</fpage>
<lpage>1332</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys.net/7/1313/2007/acp-7-1313-2007.html">This article is available from http://www.atmos-chem-phys.net/7/1313/2007/acp-7-1313-2007.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys.net/7/1313/2007/acp-7-1313-2007.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/7/1313/2007/acp-7-1313-2007.pdf</self-uri>
<abstract>
<p>The mechanisms responsible for the extreme dryness of the stratosphere have
been debated for decades. A key difficulty has been the lack of
comprehensive models which are able to reproduce the observations. Here we
examine results from the coupled lower-middle atmosphere chemistry general
circulation model ECHAM5/MESSy1 together with satellite observations. Our
model results match observed temperatures in the tropical lower stratosphere
and realistically represent the seasonal and inter-annual variability of
water vapor. The model reproduces the very low water vapor mixing ratios
(below 2 ppmv) periodically observed at the tropical tropopause near 100
hPa, as well as the characteristic tape recorder signal up to about 10 hPa,
providing evidence that the dehydration mechanism is well-captured. Our
results confirm that the entry of tropospheric air into the tropical
stratosphere is forced by large-scale wave dynamics, whereas radiative
cooling regionally decelerates upwelling and can even cause downwelling.
Thin cirrus forms in the cold air above cumulonimbus clouds, and the
associated sedimentation of ice particles between 100 and 200 hPa reduces
water mass fluxes by nearly two orders of magnitude compared to air mass
fluxes. Transport into the stratosphere is supported by regional net
radiative heating, to a large extent in the outer tropics. During summer
very deep monsoon convection over Southeast Asia, centered over Tibet,
moistens the stratosphere.</p>
</abstract>
<counts><page-count count="20"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> Alcala C. M. and Dessler A. E.: Observations of deep convection in the tropics using the Tropical Rainfall Measuring Mission (TRMM) precipitation radar, J. Geophys. Res., 107, 4792, doi:10.1029/2002JD002457, 2002. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> Aumann, H. H., Broberg, S., Elliott, D., Gaiser, S., and Gregorich, D.: Three years of Atmospheric Infrared Sounder radiometric calibration validation using sea surface temperatures, J. Geophys. Res., D16S90, doi:10.1029/2005JD006822, 2006. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Bannister, R. N., O&apos;Neil, A., Gregory, A. R., and Nissen, K. M.: The role of the south-east Asian monsoon and other seasonal features in creating the &quot;tape-recorder&quot; signal in the Unified Model, Q. J. R. Meteorol. Soc. 130, 1531-1554, 2004. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> Bonazzola, M. and Haynes, P. H.: A trajectory-based study of the tropical tropopause region, J. Geophys. Res., 109, D20112, doi:10.1029/2003JD004356, 2004. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Brewer, A. W: Evidence for a world circulation provided by the measurements of helium and water vapour distribution in the stratosphere, Q. J. R. Meteorol. Soc. 75, 351&amp;ndash;363, 1949. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> Corti, T., Luo, B. P., Fu, Q., Vömel, H., and Peter, T.: The impact of cirrus clouds on troposphere-to-stratosphere transport, Atmos. Chem. Phys., 6, 2539&amp;ndash;2547, 2006. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> Daley, R.: Atmospheric data analysis, Cambridge University Press, Cambridge, UK, 1991. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> Danielsen, E. F.: A dehydration mechanism for the stratosphere, Geophys. Res. Lett., 9, 605&amp;ndash;608, 1982. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Dessler, A. E., Palm, S. P., Hart, W. D., and Spinhirne J. D.: Tropopause-level thin cirrus coverage revealed by ICEsat/Geoscience Laser Altimeter System, J. Geophys. Res., 111, D08203, doi:10.1029/2005JD006586, 2006. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Divakarla, M. G., Barnet, C. D., Goldberg, M. D., McMillin, L. M., Maddy, E., Wolf, W., Zhou, L., and Liu, X.: Validation of Atmospheric Infrared Sounder temperature and water vapor retrievals with matched radiosonde measurements and forecasts, J. Geophys. Res., 111, D09S15, doi:10.1029/2005JD006116, 2006. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Eyring, V., Butchart, N., Waugh, D. W. et al.: Assessment of temperature, trace species and ozone in chemistry-climate model simulations in the recent past, J. Geophys. Res., 111, D22308, doi:10.1029/2006JD007327, 2006. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Fischer, H., and Oelhaf, H.: Remote sensing of vertical profiles of atmospheric trace constituents with MIPAS limb-emission spectrometers, Appl. Opt., 35, 2787&amp;ndash;2796, 1996. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Folkins, I., Loewenstein, M., Podolske, J., Oltmans, S. J., and Proffitt, M.: A barrier to vertical mixing at 14 km in the tropics: Evidence from ozonesondes and aircraft measurements, J. Geophys. Res., 104, 22 095&amp;ndash;22 102, 1999. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> Fu, R., Hu, Y., Wright, J. S., Jiang, J. H., Dickinson, R. E., Chen, M., Filipiak, M., Read, W. G., Waters, J. W., and Wu, D. L.: Short circuit of water vapor and polluted air to the global stratosphere by convective transport over the Tibetan Plateau, Proc. Nat. Acad. Sci., 103, 5664&amp;ndash;5669, 2006. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Fueglistaler, S., Wernli, H., and Peter, T.: Tropical troposphere-to-stratosphere transport inferred from trajectory calculations, J Geophys. Res., 109, D03108, doi:10.1029/2003JD004069, 2004. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Fueglistaler, S. and Haynes, P. H.: Control of interannual and longer-term variability of stratospheric water vapor, J. Geophys. Res., 110, D24108, doi:10.1029/2005JD006019, 2005. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Fueglistaler, S., Bonazzola, M., Haynes, P. H., and Peter, T.: Stratospheric water vapor predicted from the Lagrangian temperature history of air entering the stratosphere in the tropics, J. Geophys. Res., 110, D08107, doi:10.1029/2004JD005516, 2005. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Fueglistaler, S., and Fu, Q.: Impact of clouds on radiative heating rates in the lower tropical stratosphere, J. Geophys. Res., 111, D23202, doi:10.1029/2006JD007273, 2006. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Ganzeveld, L. N., van Aardenne, J., Butler, T., Lawrence, M. G., Metzger, S. M., Stier, P., Zimmerman, P., and Lelieveld, J.: Technical Note: Anthropogenic and natural offline emissions and the online EMissions and dry DEPosition (EMDEP) submodel of the Modular Earth Submodel System (MESSy), Atmos. Chem. Phys. Discuss., 6, 5457&amp;ndash;5483, 2006. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> Geller, M. A., Zhou, X., and Zhang, M.: Simulations of the interannual variability of stratospheric water vapor, J. Atmos. Sci., 59, 1076&amp;ndash;1085, 2002. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Gettelman, A., Salby, M. L., and Sassi, F.: Distribution and influence of convection in the tropical tropopause region, J. Geophys. Res., 107, D10, 4080, doi:10.1029/2001JD001048 (2002). </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Gettelman, A., Forster, P.M. de F., Fujiwara, M., Fu, Q., Vömel, H., Gohar, L. K., Johanson, C., and Ammerman, M: Radiation balance of the tropical tropopause layer, J. Geophys. Res., 109, D07103, doi:10.1029/2003JD004190, 2004a. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Gettelman, A., Weinstock, E. M., Fetzer, E. J., Irion, F. W., Eldering, A., Richard, E. C., Rosenlof, K. H., Thompson, T. L., Pittman, J. V., Webster, C. R., and Herman, R. L.: Validation of Aqua satellite data in the upper troposphere and lower stratosphere with in situ aircraft instruments, Geophys. Res. Lett., 31, L22107, doi:10.1029/2004GL020730, 2004b. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> Gettelman, A., Collins, W. D., Fetzer, E. J., Eldering, A., Irion, F. W., Duffy, P. B., and Bala, G.: Climatology of upper-tropospheric relative humidity from the Atmospheric Infrared Sounder and implications for climate, J. Climate, 19, 6104&amp;ndash;6121, 2006a. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Gettelman, A., Fetzer, E. J., Eldering, A., and Irion, F. W.: The global distribution of supersaturation in the upper troposphere from the Atmospheric Infrared Sounder, J. Climate, 19, 6089&amp;ndash;6103, 2006b. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> Giorgetta, M. A. and Bengtsson, L.: Potential role of the quasi-biennial oscillation in the stratosphere-troposphere exchange as found in water vapor in general circulation model experiments, J. Geophys. Res., 104, 6003&amp;ndash;6019, 1999. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> Giorgetta, M. A., Manzini, E., Roeckner, E., Esch, M., and Bengtsson, L.: Climatology and forcing of the quasi-biennial oscillation in the MAECHAM5 model, J. Climate, 19, 3882&amp;ndash;3901, 2006. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> Hagemann, S., Arpe, K., and Roeckner, E.: Evaluation of the hydrological cycle in the ECHAM5 model, J. Climate, 19, 3810&amp;ndash;3827, 2006. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> Harries, J. E., Russell III, J. M., Tuck, A. F., Gordley, L. L., Purcell, P., Stone, K. Bevilacqua, R. M., Gunson, M., Nedoluha, G., and Traub, W. A.: Validation of water vapor from the Halogen Occultation Experiment (HALOE), J. Geophys. Res., 101, 10 205&amp;ndash;10 216, 1996. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> Hartmann, D. L., Holton, J. R., and Fu, Q.: The heat balance of the tropical tropopause, cirrus, and stratospheric dehydration, Geophys. Res. Lett., 28, 1969&amp;ndash;1972, 2001. </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> Haynes, P. H., Marks, C. J., McIntyre, M. E., Shepherd, T. G., and Shine, K. P.: On the &quot;downward control&quot; of extratropical diabatic circulations by eddy-induced zonal mean forces, J. Atmos. Sci., 48, 651&amp;ndash;678, 1991. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> Heymsfield, A. J. and Donner, L. J.: A scheme for parameterizing ice-cloud water content in general circulation models, J. Atmos. Sci., 47, 1865&amp;ndash;1877, 1990. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> Highwood, E. J. and Hoskins, B. J.: The tropical tropopause, Q. J. R. Meteorol. Soc., 124, 1579&amp;ndash;1604, 1998. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> Holton, J. R., Haynes, P. H., McIntyre, M. E., Douglas, A. R., Rood, R. R., and Pfister, L.: Stratosphere-troposphere exchange, Rev. Geophys., 33, 403&amp;ndash;439, 1995. </mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple"> Holton, J. R. and Gettelman, A.: Horizontal transport and the dehydration of the stratosphere, Geophys. Res. Lett., 28, 2799&amp;ndash;2802, 2001. </mixed-citation>
</ref>
<ref id="ref36">
<label>36</label><mixed-citation publication-type="other" xlink:type="simple"> Jackson, D. R., Burrage, M. D., Harries, J. E., Gray, L. J., and Russell III, J. M.: The semi-annual oscillation in upper stratospheric and mesospheric water vapour as observed by HALOE, Q. J. R. Meteorol. Soc., 124, 2493&amp;ndash;2515, 1998. </mixed-citation>
</ref>
<ref id="ref37">
<label>37</label><mixed-citation publication-type="other" xlink:type="simple"> Jensen, E. J., Pfister, L., Ackerman, A. S., Tabazadeh, A., and Toon, O. B.: A conceptual model of the dehydration of air due to freeze-drying by optically thin, laminar cirrus rising slowly across the tropical tropopause, J. Geophys. Res., 106, 17 237&amp;ndash;17 252, doi:10.1029/2000JD900649, 2001. </mixed-citation>
</ref>
<ref id="ref38">
<label>38</label><mixed-citation publication-type="other" xlink:type="simple"> Jensen, E., and Pfister, L.: Transport and freeze-drying in the tropical tropopause layer, J. Geophys. Res., 109, D02207, doi:10.1029/2003JD004022, 2004. </mixed-citation>
</ref>
<ref id="ref39">
<label>39</label><mixed-citation publication-type="other" xlink:type="simple"> Jöckel, P., Sander, R., Kerkweg, A., Tost, H., and Lelieveld, J.: Technical Note: The Modular Earth Submodel System (MESSy) - a new approach towards Earth System Modeling, Atmos. Chem. Phys., 5, 433&amp;ndash;444, 2005. </mixed-citation>
</ref>
<ref id="ref40">
<label>40</label><mixed-citation publication-type="other" xlink:type="simple"> Jöckel, P., Tost, H., Pozzer, A., Brühl, C., Buchholz, J., Ganzeveld, L., Hoor, P., Kerkweg, A., Lawrence, M. G., Sander, R., Steil, B., Stiller, G., Tanarhte, M., Taraborelli, D., van Aardenne, J., and Lelieveld, J.: The atmospheric chemistry general circulation model ECHAM5/MESSy: Consistent simulation of ozone from the surface to the mesosphere, Atmos. Chem. Phys., 6, 5067&amp;ndash;5104, 2006. </mixed-citation>
</ref>
<ref id="ref41">
<label>41</label><mixed-citation publication-type="other" xlink:type="simple"> Kerkweg, A., Sander, R., Tost, H., and P. Jöckel: Technical Note: Implementation of prescribed (OFFLEM), calculated (ONLEM), and pseudo-emissions (TNUDGE) of chemical species in the Modular Earth Submodel System (MESSy), Atmos. Chem. Phys., 6, 3603&amp;ndash;3609, 2006a. </mixed-citation>
</ref>
<ref id="ref42">
<label>42</label><mixed-citation publication-type="other" xlink:type="simple"> Kerkweg A., Buchholz, J., Ganzeveld, L., A. Pozzer, H. Tost, and P. Jöckel: Technical Note: An implementation of the dry removal processes DRY DEPosition and SEDImentation in, the Modular Earth Submodel System (MESSy), Atmos. Chem. Phys., 6, 4617&amp;ndash;4632, 2006b. </mixed-citation>
</ref>
<ref id="ref43">
<label>43</label><mixed-citation publication-type="other" xlink:type="simple"> Kley, D., Stone, E. J., Henderson, W. R., Drummond, J. W., Harrop, W. J., Schmeltekopf, L., Thompson, T. L., and Winkler, R. H.: In situ measurements of the mixing ratio of water vapor in the stratosphere, J. Atmos. Sci., 36, 2513&amp;ndash;2524, 1979. </mixed-citation>
</ref>
<ref id="ref44">
<label>44</label><mixed-citation publication-type="other" xlink:type="simple"> Kley, D., Russell III, J. M., and Phillips, C.: SPARC Assessment of upper tropospheric and stratospheric water vapour, WCRP-113, WMO/TD-No. 1043, SPARC Report No. 2, World Meteorological Organization, Geneva, 2000. </mixed-citation>
</ref>
<ref id="ref45">
<label>45</label><mixed-citation publication-type="other" xlink:type="simple"> Landgraf, J. and Crutzen, P. J.:An efficient method for online calculations of photolysis and heating rates, J. Atmos. Sci., 55, 863&amp;ndash;878, 1998. </mixed-citation>
</ref>
<ref id="ref46">
<label>46</label><mixed-citation publication-type="other" xlink:type="simple"> Lin, S. J., and Rood, R. B.: Multi-dimensional flux-form semi-Lagrangian transport schenes, Mon. Wea. Rev., 124, 2046&amp;ndash;2070, 1996. </mixed-citation>
</ref>
<ref id="ref47">
<label>47</label><mixed-citation publication-type="other" xlink:type="simple"> Lawrence, M. G. and Rasch, P. J.: Tracer transport in deep convective updrafts: plume ensemble versus bulk formulations, J. Atmos. Sci., 62, 2880&amp;ndash;2894, 2005. </mixed-citation>
</ref>
<ref id="ref48">
<label>48</label><mixed-citation publication-type="other" xlink:type="simple"> Lohmann, U. and Roeckner, E. : Design and performance of a new cloud microphysics parameterization developed for the ECHAM4 general circulation model, Clim. Dyn., 12, 557&amp;ndash;572, 1996. </mixed-citation>
</ref>
<ref id="ref49">
<label>49</label><mixed-citation publication-type="other" xlink:type="simple"> Lohmann, U., Roeckner, E., Collins, W. D. Heymsfield, A. J., McFarquhar, G. M., and Barnett, T. P.: The role of water vapor and convection during the Central Equatorial Pacific Experiment from observations and model simulations, J. Geophys. Res., 100(D12), 26 229&amp;ndash;26 246, 1995. </mixed-citation>
</ref>
<ref id="ref50">
<label>50</label><mixed-citation publication-type="other" xlink:type="simple"> Luo, Z., and W. B. Rossow: Characterizing tropical cirrus life cycle, evolution and interaction with upper-tropospheric water vapor using Lagrangian trajectory analysis of satellite observations, J. Clim., 17, 4541&amp;ndash;4563, 2004. </mixed-citation>
</ref>
<ref id="ref51">
<label>51</label><mixed-citation publication-type="other" xlink:type="simple"> Majewski, D.: Balanced initial and boundary values for a limited area model, Beitr. Phys. Atm., 58, 147&amp;ndash;165, 1985. </mixed-citation>
</ref>
<ref id="ref52">
<label>52</label><mixed-citation publication-type="other" xlink:type="simple"> Manzini, E., Steil, B. Brühl, C., Giorgetta, M. A., and Krüger, K.: A new interactive chemistry-climate model: 2. Sensitivity of the middle atmosphere to ozone depletion and increase in greenhouse gases and implications for recent stratospheric cooling. J. Geophys. Res., 108(D14), 4429, doi:10.1029/2002JD002977, 2003. </mixed-citation>
</ref>
<ref id="ref53">
<label>53</label><mixed-citation publication-type="other" xlink:type="simple"> Manzini, E., Giorgetta, M. A., Esch, M., Kornblueh, L., and Roeckner, E.: The influence of sea surface temperatures on the northern winter stratosphere: ensemble simulations with the MAECHAM5 model, J. Climate, 19, 3863&amp;ndash;3881, 2006. </mixed-citation>
</ref>
<ref id="ref54">
<label>54</label><mixed-citation publication-type="other" xlink:type="simple"> Massie S., Gettelman, A., Randel, W., and Baumgardner, D.: Distribution of tropical cirrus in relation to convection, J. Geophys. Res., 107 (D21), 4591, doi:10.1029/2001JD001293, 2002. </mixed-citation>
</ref>
<ref id="ref55">
<label>55</label><mixed-citation publication-type="other" xlink:type="simple"> McFarquhar, G. M., Heymsfield, A. J., Spinhirne, J., and Hart, B.: Thin and subvisual tropical tropopause cirrus, J. Atmos. Sci., 57, 1841&amp;ndash;1853, 2000. </mixed-citation>
</ref>
<ref id="ref56">
<label>56</label><mixed-citation publication-type="other" xlink:type="simple"> Mlynczak, M. G., Mertens, C. J., Garcia, R. R., and Portmann, R. W.: A detailed evaluation of the stratospheric heat budget 2. Global radiation balance and diabatic circulations, J. Geophys. Res., 104, 6039&amp;ndash;6066, 1999. </mixed-citation>
</ref>
<ref id="ref57">
<label>57</label><mixed-citation publication-type="other" xlink:type="simple"> Mote, P. W., Rosenlof, K. H., McIntyre, M. E., Carr, E. S., Gille, J. C., Holton, J. R., Kinnersley, J. S., Pumphrey, H. C., Russell III, J. M., and Waters, J. W.: An atmospheric tape recorder: The imprint of tropical tropopasue temperatures on stratospheric water vapor, J. Geophys. Res., 101, 3989&amp;ndash;4006, 1996. </mixed-citation>
</ref>
<ref id="ref58">
<label>58</label><mixed-citation publication-type="other" xlink:type="simple"> Newell, R. E., and Gould-Stewart, S.: A stratospheric fountain?, J. Atmos. Sci. 38, 2789&amp;ndash;2796, 1981. </mixed-citation>
</ref>
<ref id="ref59">
<label>59</label><mixed-citation publication-type="other" xlink:type="simple"> Nordeng, T. E.: Extended versions of the convective parameterization scheme at ECMWF and their impact on the mean and transient activity of the model in the tropics, ECMWF Technical Report, 206, Reading, UK, 1994. </mixed-citation>
</ref>
<ref id="ref60">
<label>60</label><mixed-citation publication-type="other" xlink:type="simple"> Norton, W. A.: Longwave heating of the tropical lower stratosphere, Geophys. Res. Lett., 28, 3653&amp;ndash;3656, 2001. </mixed-citation>
</ref>
<ref id="ref61">
<label>61</label><mixed-citation publication-type="other" xlink:type="simple"> Peter, T. Luo, B. P., Wirth, M, Kiemle, C., Flentje, H., Yushkov, V. A., Khattatov, V., Rudakov, V., Thomas, A., Borrmann, S., Toci, G., Mazzinghi, P., Beuermann, J., Schiller, C., Cairo, F, Di Donfrancesco, G., Adriani, A., Volk, C. M., Ström, J., Noone, K., Mitev, V., MacKenzie, R. A., Carslaw, K. S., Trautmann, T., Santacesaria, V., and Stefanutti, L.: Ultrathin Tropical Tropopause Clouds (UTTCs): I. Cloud morphology and occurrence, Atmos. Chem. Phys., 3, 1083&amp;ndash;1091, 2003. </mixed-citation>
</ref>
<ref id="ref62">
<label>62</label><mixed-citation publication-type="other" xlink:type="simple"> Plumb, R. A. and Eluszkiewiwicz, J.: The Brewer-Dobson circulation: dynamics of the tropical upwelling, J. Atmos. Sci., 56, 868&amp;ndash;890, 1999. </mixed-citation>
</ref>
<ref id="ref63">
<label>63</label><mixed-citation publication-type="other" xlink:type="simple"> Potter, B. E. and Holton, J. R.: The role of monsoon convection in the dehydration of the lower tropical stratosphere, J. Atmos. Sci., 52, 1034&amp;ndash;1050, 1995. </mixed-citation>
</ref>
<ref id="ref64">
<label>64</label><mixed-citation publication-type="other" xlink:type="simple"> Randel, W. J. and Wu, F.: Isolation of the ozone QBO in SAGE II data by singular-value decomposition, J. Atmos. Sci., 53, 2546&amp;ndash;2559, 1996. </mixed-citation>
</ref>
<ref id="ref65">
<label>65</label><mixed-citation publication-type="other" xlink:type="simple"> Randel, W. J., Zawodny, J. M., and Oltmans, S. J. : Seasonal variation of water vapor in the lower stratosphere observed in Halogen Occultation Experiment data, J. Geophys. Res., 106(D13), 14 313&amp;ndash;14 326, doi:10.1029/2001JD900048, 2001. </mixed-citation>
</ref>
<ref id="ref66">
<label>66</label><mixed-citation publication-type="other" xlink:type="simple"> Randel, W. J., Wu, F., Oltmans, S. J., Rosenlof, K., and Nedoluha G. E.: Interannual changes of stratospheric water vapor and correlations with tropical tropopause temperatures, J. Atmos. Sci., 61, 2133&amp;ndash;2148, 2004. </mixed-citation>
</ref>
<ref id="ref67">
<label>67</label><mixed-citation publication-type="other" xlink:type="simple"> Randel, W. J., Wu, F., Vömel, H., Nedoluha, G. E., and Forster, P.: Decreases in stratsopheric water vapor after 2001: Links to changes in the tropical tropopause and the Brewer-Dobson circulation, J. Geophys. Res., 111, D12312, doi:10.1029/2005JD0006744, 2006. </mixed-citation>
</ref>
<ref id="ref68">
<label>68</label><mixed-citation publication-type="other" xlink:type="simple"> Reithmeier, C. and Sausen, R.: ATTILA &amp;ndash; Atmospheric Tracer Transport in a Lagrangian model, Tellus, 54, 278&amp;ndash;299, 2002. </mixed-citation>
</ref>
<ref id="ref69">
<label>69</label><mixed-citation publication-type="other" xlink:type="simple"> Remsberg, E. E., Bhatt, P. P., and Russell III, J. M.: Estimates of the water vapor budget of the stratosphere from UARS HALOE data, J. Geophys. Res., 101(D3), 6749&amp;ndash;6766, 1996. </mixed-citation>
</ref>
<ref id="ref70">
<label>70</label><mixed-citation publication-type="other" xlink:type="simple"> Roeckner, E., Bäuml, G., Bonaventura, L., Brokopf, R., Esch, M., Giorgetta, M., Hagemann, S., Kirchner, I., Kornblueh, L., Manzini, E., Rhodin, A., Schlese, U., Schulzweida, U., and Tompkins, A.: The atmospheric general circulation model ECHAM5. PART I: Model description, Max Planck Institute for Meteorology, MPI-Report 349, http://www.mpimet.mpg. de/fileadmin/publikationen/Reports/max scirep 349.pdf, 2003. </mixed-citation>
</ref>
<ref id="ref71">
<label>71</label><mixed-citation publication-type="other" xlink:type="simple"> Roeckner, E., Brokopf, R., Esch, M., Giorgetta, M., Hagemann, S., Kornblüh, Manzini, L. E., Schlese, U., and Schulzweida, U.: Sensitivity of simulated climate to horizontal and vertical resolution in the ECHAM5 atmosphere model, J. Climate, 19, 3771&amp;ndash;3791, 2006. </mixed-citation>
</ref>
<ref id="ref72">
<label>72</label><mixed-citation publication-type="other" xlink:type="simple"> Rosenlof, K. H., and Holton, J. R.: Estimates of the stratospheric residual circulation using the downward control principle, J. Geophys. Res., 98, 10 465&amp;ndash;10 479, 1993. </mixed-citation>
</ref>
<ref id="ref73">
<label>73</label><mixed-citation publication-type="other" xlink:type="simple"> Rosenlof, K. H.: Seasonal cycle of the residual mean meridional circulation in the stratosphere, J. Geophys. Res., 100, 5173&amp;ndash;5191, 1995. </mixed-citation>
</ref>
<ref id="ref74">
<label>74</label><mixed-citation publication-type="other" xlink:type="simple"> Russell, J. M. III, Gordley, L. L., Park, J. H., Drayson, S. R., Hesketh, W. D., Cicerone, R. J. Tuck, A. F., Frederick, J. E., Harries, J. E., and Crutzen, P. J.: The Halogen Occultation Experiment, J. Geophys. Res., 98, 10 777&amp;ndash;10 798, 1993. </mixed-citation>
</ref>
<ref id="ref75">
<label>75</label><mixed-citation publication-type="other" xlink:type="simple"> Sander, R., Kerkweg, A., Jöckel, P., and Lelieveld, J.: Technical Note: The new comprehensive atmospheric chemistry module MECCA, Atmos. Chem. Phys., 5, 445&amp;ndash;450, 2005. </mixed-citation>
</ref>
<ref id="ref76">
<label>76</label><mixed-citation publication-type="other" xlink:type="simple"> Sandu, A. and Sander, R.: Technical Note: Simulating chemical systems in Fortran90 and Matlab with the 5 kinetic preprocessor KPP-2.1, Atmos. Chem. Phys., 6, 187&amp;ndash;195, 2006. </mixed-citation>
</ref>
<ref id="ref77">
<label>77</label><mixed-citation publication-type="other" xlink:type="simple"> Seidel, D. J., Ross, R. J., Angell, J. K., and Reid, G. C.: Climatological characteristics of the tropical tropopause as revealed by radiosondes, J. Geophys. Res., 106, 7857&amp;ndash;7878, 2001. </mixed-citation>
</ref>
<ref id="ref78">
<label>78</label><mixed-citation publication-type="other" xlink:type="simple"> Sherwood, S. C.: A stratospheric &quot;drain&quot; over the maritime continent, Geophys. Res. Lett., 27, 677&amp;ndash;680, 2000. </mixed-citation>
</ref>
<ref id="ref79">
<label>79</label><mixed-citation publication-type="other" xlink:type="simple"> Sherwood, S. C., and A. E. Dessler: A model for transport across the tropical tropopause, J. Atmos. Sci., 58, 765&amp;ndash;779, 2001. </mixed-citation>
</ref>
<ref id="ref80">
<label>80</label><mixed-citation publication-type="other" xlink:type="simple"> Soden, B. J.: The impact of tropical convection and cirrus on upper tropospheric humidity: A Lagrangian analysis of satellite measurements, Geophys. Res. Lett., 31, L20104, doi:10.1029/2004GL020980, 2004. </mixed-citation>
</ref>
<ref id="ref81">
<label>81</label><mixed-citation publication-type="other" xlink:type="simple"> Solomon, S.: Stratospheric ozone depletion: A review of concepts and history, Rev. Geophys., 37, 275&amp;ndash;316, 1999. </mixed-citation>
</ref>
<ref id="ref82">
<label>82</label><mixed-citation publication-type="other" xlink:type="simple"> Sparling, L. C.: Statistical perspectives on stratospheric transport, Rev. Geophys., 38, 417&amp;ndash;436, 2000. </mixed-citation>
</ref>
<ref id="ref83">
<label>83</label><mixed-citation publication-type="other" xlink:type="simple"> Steil, B., Brühl, C., Manzini, E., Crutzen, P., Lelieveld, J., Rasch, P. J., Roeckner, E., and Krüger, K.: A new interactive chemistry climate model. I: Present day climatology and interannual variability of the middle atmosphere using the model and 9 years of HALOE/UARS data, J. Geophys. Res., 108, 4290, doi:10.1029/2002JD002971, 2003. </mixed-citation>
</ref>
<ref id="ref84">
<label>84</label><mixed-citation publication-type="other" xlink:type="simple"> Stohl, A. and Trickl, T. : A textbook example of long-range transport: Simultaneous observation of ozone maxima of stratospheric and North American origin in the free troposphere over Europe, J. Geophys. Res., 104(D23), 30 445&amp;ndash;30 462, 1999. </mixed-citation>
</ref>
<ref id="ref85">
<label>85</label><mixed-citation publication-type="other" xlink:type="simple"> Thomas, A., Borrmann, S., Kiemle, C., Cairo, F., Volk, M., Beuermann, J., Lepuchov, B., Santacesaria, V., Matthey, R., Rudakov, V., Yushkov, V., MacKenzie, R. A., and Stefanutti, L.: In situ measurements of background aerosol and subvisible cirrus in the tropical tropopause region, J. Geophys. Res., 107 (D24), 4763, doi:10.1029/2001JD001385, 2002. </mixed-citation>
</ref>
<ref id="ref86">
<label>86</label><mixed-citation publication-type="other" xlink:type="simple"> Tiedtke, M.: A comprehensive mass flux scheme for cumulus parametrization in large-scale models, Mon. Weather Rev., 117, 1779&amp;ndash;1800, 1989. </mixed-citation>
</ref>
<ref id="ref87">
<label>87</label><mixed-citation publication-type="other" xlink:type="simple"> Tost, H.: Global Modelling of Cloud, Convection and Precipitation Influences on Trace Gases and Aerosols, Ph.D. thesis, University of Bonn, Germany, 2006. </mixed-citation>
</ref>
<ref id="ref88">
<label>88</label><mixed-citation publication-type="other" xlink:type="simple"> Tost, H., Jöckel, P., Kerkweg, A., Sander, R., and Lelieveld, J.: Technical Note: A new comprehensive SCAVenging submodel for global atmospheric chemistry modelling, Atmos. Chem. Phys., 6, 565&amp;ndash;574, 2006a. </mixed-citation>
</ref>
<ref id="ref89">
<label>89</label><mixed-citation publication-type="other" xlink:type="simple"> Tost, H., Jöckel, P., and Lelieveld, J.: Influence of different convection parameterisations in a GCM, Atmos. Chem. Phys., 6, 5475&amp;ndash;5493, 2006b. </mixed-citation>
</ref>
<ref id="ref90">
<label>90</label><mixed-citation publication-type="other" xlink:type="simple"> Traub, M. A.: Lagrangian transport evaluation of atmospheric chemistry in the Mediterranean region Ph.D. Thesis, University of Mainz, Germany, 2004. </mixed-citation>
</ref>
<ref id="ref91">
<label>91</label><mixed-citation publication-type="other" xlink:type="simple"> Tuck A. F., Baumgardner, D., Chan, K. R., Dye, J. E., et al.: The Brewer-Dobson circulation in the light of high altitude in situ aircraft observations, Q. J. R. Meteorol. Soc., 123, 1&amp;ndash;69, 1997. </mixed-citation>
</ref>
<ref id="ref92">
<label>92</label><mixed-citation publication-type="other" xlink:type="simple"> Van Aalst, M. K., van den Broek, M. M. P., Bregman, A., Brühl, C., Steil, B., Toon, G. C. Garcelon, S., Hansford, G. M., Jones, R. L., Gardiner, T. D., Roelofs, G. J., Lelieveld, J., and Crutzen, P. J.: Trace gas transport in the 1999/2000 Actic winter: comparison of nudged GCM runs with observations, Atmos. Chem. Phys., 4, 81&amp;ndash;93, 2004. </mixed-citation>
</ref>
<ref id="ref93">
<label>93</label><mixed-citation publication-type="other" xlink:type="simple"> Volk, C. M., Elkins, J. W., Fahey, D. W., Salawitch, R. J., Dutton, G. S., Gilligan, J. M., Proffitt, M. H., Loewenstein, M., Podolske, J. R., Minschwaner, K., Margitan, J. J., and Chan, K. R.: Quantifying transport between the tropical and mid-latutude lower stratosphere, Science, 272, 1763&amp;ndash;1768, 1996. </mixed-citation>
</ref>
<ref id="ref94">
<label>94</label><mixed-citation publication-type="other" xlink:type="simple"> Vömel, H., Oltmans, S. J., Johnson, B. J., Hasebe, F., Shiotani, M., Fujiwara, M., Nishi, N., Agama, M., Cornejo, J., Paredes, F., and Enriques, H.: Balloon-borne observation of water vapor and ozone in the tropical upper troposphere and lower stratosphere, J. Geophys. Res., 107, 4210, doi:10.1029/2001JD000707, 2002. </mixed-citation>
</ref>
<ref id="ref95">
<label>95</label><mixed-citation publication-type="other" xlink:type="simple"> Wang, D. Y., von Clarmann, T., Fischer, H., Funke, B., et al.: Validation of stratospheric temperatures measured by Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) on Envisat, J. Geophys. Res., 110, D08301, doi:10.1029/2004JD005342, 2005. </mixed-citation>
</ref>
<ref id="ref96">
<label>96</label><mixed-citation publication-type="other" xlink:type="simple"> Webster, C. R. and Heymsfield, A. J.: Water isotope ratios D/H, $^18$O/$^16$O, $^17$O/$^16$O in and out of clouds map dehydration pathways, Science, 302, 1742&amp;ndash;1692, 2003. </mixed-citation>
</ref>
<ref id="ref97">
<label>97</label><mixed-citation publication-type="other" xlink:type="simple"> Wernli H., and Bourqui, M.: A Lagrangian &quot;1-year climatology&quot; of (deep) cross-tropopause exchange in the extratropical Northern Hemisphere, J. Geophys. Res., 107 (D2), 4021, doi:10.1029/2001JD000812, 2002. </mixed-citation>
</ref>
<ref id="ref98">
<label>98</label><mixed-citation publication-type="other" xlink:type="simple"> Wild, M. and Roeckner, E.: Radiative fluxes in the ECHAM5 general circulation model, J. Climate, 19, 3792&amp;ndash;3809, 2006. </mixed-citation>
</ref>
<ref id="ref99">
<label>99</label><mixed-citation publication-type="other" xlink:type="simple"> Wylie, D. P., and Wang P.-H.: Comparison of cloud frequency data from the high-resolution infrared radiometer sounder and the Stratospheric Aerosol and Gas Experiment II, J. Geophys. Res., 102, 29 893&amp;ndash;29 900, 1997. </mixed-citation>
</ref>
<ref id="ref100">
<label>100</label><mixed-citation publication-type="other" xlink:type="simple"> Yulaeva, E., Holton, J. R., and Wallace, J. M.: On the cause of the annual cycle in tropical lower stratospheric temperatures, J. Atmos. Sci., 51, 169&amp;ndash;174, 1994. </mixed-citation>
</ref>
</ref-list>
</back>
</article>