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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-6-5261-2006</article-id>
<title-group>
<article-title>Modeling of biomass smoke injection into the lower stratosphere by a large forest fire (Part&amp;nbsp;II): sensitivity studies</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Luderer</surname>
<given-names>G.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Trentmann</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Winterrath</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Textor</surname>
<given-names>C.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Herzog</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Graf</surname>
<given-names>H.&amp;nbsp;F.</given-names>
</name>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Andreae</surname>
<given-names>M.&amp;nbsp;O.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Max Planck Institute for Chemistry, Dept.&amp;nbsp;Biogeochemistry, Mainz, Germany</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Institute for Atmospheric Physics, Johannes Gutenberg University Mainz, Mainz, Germany</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Service d&apos;Aéronomie, CNRS, Paris, France</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>NOAA GFDL, Princeton, New Jersey, USA</addr-line>
</aff>
<aff id="aff5">
<label>5</label>
<addr-line>Department of Geography, Centre of Atmospheric Science, University of Cambridge, Cambridge, UK</addr-line>
</aff>
<pub-date pub-type="epub">
<day>17</day>
<month>11</month>
<year>2006</year>
</pub-date>
<volume>6</volume>
<issue>12</issue>
<fpage>5261</fpage>
<lpage>5277</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys.net/6/5261/2006/acp-6-5261-2006.html">This article is available from http://www.atmos-chem-phys.net/6/5261/2006/acp-6-5261-2006.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys.net/6/5261/2006/acp-6-5261-2006.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/6/5261/2006/acp-6-5261-2006.pdf</self-uri>
<abstract>
<p>The Chisholm forest fire that burned in Alberta, Canada, in May 2001 resulted in
injection of substantial amounts of smoke into the lower stratosphere.
We used the cloud-resolving plume model ATHAM (Active Tracer High resolution
Atmospheric Model) to investigate the importance of different contributing factors to the severe
intensification of the convection induced by the Chisholm  fire and the subsequent injection of
biomass smoke into the lower stratosphere. The simulations show strong
sensitivity of the pyro-convection to background meteorology. This
explains the observed coincidence of the convective blow-up of the fire plume and the
passage of a synoptic cold front.

&lt;br&gt;&lt;br&gt;

Furthermore, we performed model sensitivity studies to the rate of release of
sensible heat and water vapor from the fire. The release of
sensible heat by the fire plays a dominant role for the dynamic development
of the pyro-cumulonimbus cloud (pyroCb) and the height to which smoke is
transported. The
convection is very sensitive to the heat flux from the fire. The
emissions of water vapor play a less significant role for the injection height
but enhance the amount of smoke transported beyond the
tropopause level.

&lt;br&gt;&lt;br&gt;

The aerosol burden in the plume has a strong impact on the microphysical structure
of the resulting convective cloud. The dynamic evolution of the
pyroCb, however, is only weakly sensitive to the abundance of cloud
condensation nuclei (CCN) from the fire.
In contrast to previous findings by other
studies of convective clouds, we found that fire CCN have a negative effect on the
convection dynamics because they give rise to a delay in the freezing of cloud droplets.
Even in a simulation without fire CCN, there is no precipitation formation within
the updraft region of the pyroCb.
Enhancement of convection by aerosols as reported from studies of
other cases of convection is therefore not found in our study.</p>
</abstract>
<counts><page-count count="17"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> Andreae, M.&amp;nbsp;O. and Merlet, P.: Emission of trace gases and aerosols from biomass burning, Global Biogeochem. Cy., 15, 955&amp;ndash;966, 2001. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> Andreae, M.&amp;nbsp;O., Rosenfeld, D., Artaxo, P., Costa, A.&amp;nbsp;A., Frank, G.&amp;nbsp;P., Longo, K.&amp;nbsp;M., and Silva-Dias, M. A.&amp;nbsp;F.: Smoking rain clouds over the Amazon, Science, 303, 1337&amp;ndash;1342, 2004. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> ASRD: Final Documentation Report &amp;ndash; Chisholm Fire (LWF-063), Forest Protection Division, ISBN 0-7785-1841-8, Tech. rep., Alberta Sustainable Resource Development, 2001. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> Bigg, E.&amp;nbsp;K.: The formation of atmospheric ice crystals by the freezing of droplets, Q. J. R. Meteorol. Soc., 79, 510&amp;ndash;519, 1953. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Byram, G.&amp;nbsp;M.: Combustion of forest fuels, in: Forest Fire Control and Use, edited by: Davis, K.&amp;nbsp;P., McGraw-Hill, New York, 90&amp;ndash;123, 1959. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> Cook, J. and Highwood, E.: Climate response to tropospheric absorbing aerosol in an intermediate general-circulation model, Q. J. R. Meteorol. Soc., 130, 175&amp;ndash;191, 2004. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> Damoah, R., Spichtinger, N., Servranckx, R., Fromm, M., Eloranta, E.&amp;nbsp;W., Razenkov, I.&amp;nbsp;A., James, P., Shulski, M., Forster, C., and Stohl, A.: A case study of pyro-convection using transport model and remote sensing data, Atmos. Chem. Phys., 6, 173&amp;ndash;185, 2006. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> Emanuel, K.&amp;nbsp;A.: Atmospheric Convection, Oxford Univesity Press, New York, 1994. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Fromm, M., Alfred, J., Hoppel, K., Hornstein, J., Bevilacqua, R., Shettle, E., Servranckx, R., Li, Z., and Stocks, B.: Observations of boreal forest fire smoke in the stratosphere by POAM III, SAGE II, and lidar in 1998, Geophys. Res. Lett., 27, 1407&amp;ndash;1410, 2000. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Fromm, M., Bevilacqua, R., Stocks, B., and Servranckx, R.: New directions: Eruptive transport to the stratosphere: Add fire-convection to volcanoes, Atmos. Environ., 38, 163&amp;ndash;165, 2004. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Fromm, M., Bevilacqua, R., Servranckx, R., Rosen, J., Thayler, J., Herman, J., and Larko, D.: Pyro-cumulonimbus injection of smoke into the stratosphere: Observerations and impact of a super blowup in northwestern Canada on 3&amp;ndash;4 August 1998, J. Geophys. Res., 110, D08205, doi:10.1029/2004JD005350, 2005. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Fromm, M.&amp;nbsp;D. and Servranckx, R.: Transport of forest fire smoke above the tropopause by supercell convection, Geophys. Res. Lett., 30, 1542, doi:10.1029/2002GL016820, 2003. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Graf, H.-F.: The Complex Interactions of Aerosols and Clouds, Science, 303, 1309&amp;ndash;1311, 2004. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> Graf, H.-F., Herzog, M., Oberhuber, J.&amp;nbsp;M., and Textor, C.: The effect of environmental conditions on volcanic plume rise, J. Geophys. Res., 104, 24 309&amp;ndash;24 320, 1999. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Herzog, M., Graf, H.-F., Textor, C., and Oberhuber, J.&amp;nbsp;M.: The effect of phase changes of water on the development of volcanic plumes, J. Volcanol. Geotherm. Res, 87, 55&amp;ndash;74, 1998. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Herzog, M., Oberhuber, J.&amp;nbsp;M., and Graf, H.-F.: A prognostic turbulence scheme for the nonhydrostatic plume model ATHAM, J. Atmos. Sci., 60, 2783&amp;ndash;2796, 2003. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Hobbs, P.&amp;nbsp;V. and Locatelli, J.&amp;nbsp;D.: Ice Nuclei from a Natural Forest Fire, J.\ Appl. Meteorol., 8, 833&amp;ndash;834, 1969. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Houze, R.&amp;nbsp;A.: Cloud Dynamics, Academic Press, San Diego, 1993. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Jost, H.-J., Drdla, K., Stohl, A., Pfister, L., Loewenstein, M., Lopez, J.&amp;nbsp;P., Hudson, P.&amp;nbsp;K., Murphy, D.&amp;nbsp;M., Mahoney, D.&amp;nbsp;J., Cziczo, D.&amp;nbsp;J., Fromm, M., Bui, T.&amp;nbsp;P., Dean-Day, J., Gerbig, C., Mahoney, M.&amp;nbsp;J., Richard, E. C., Spichtinger, N., Pittman, J.&amp;nbsp;V., Weinstock, E.&amp;nbsp;M., Wilson, J.&amp;nbsp;C., and Xueref, I.: In-situ observation of mid-latitude forest fire plumes deep in the stratosphere, Geophys. Res. Lett., 31, L11101, doi:10.1029/2003GL019253, 2004. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> Khain, A., Ovtchinnikov, M., Pinsky, M., Pokrovsky, A., and Krugliak, H.: Notes on the state-of-the-art numerical modeling of cloud microphysics, Atmos. Res., 55, 159&amp;ndash;224, 2000. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Koren, I., Kaufman, Y.&amp;nbsp;J., Rosenfeld, D., Remer, L.&amp;nbsp;A., and Rudich, Y.: Aerosol invigoration and restructuring of Atlantic convective clouds, Geophys. Res. Lett., 32, L14828, doi:10.1029/22005GL023187, 2005. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Lavoué, D., Liousse, C., Cachier, H., Stocks, B.&amp;nbsp;J., and Goldammer, J.&amp;nbsp;G.: Modeling of carbonaceous particles emitted by boreal and temperate wildfires at northern latitudes, J. Geophys. Res., 105, 26 871&amp;ndash;26 890, 2000. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Lohmann, U. and Feichter, J.: Global indirect aerosol effects: A review, Atmos. Chem. Phys., 5, 715&amp;ndash;737, 2005. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> McCarter, R.&amp;nbsp;J. and Broido, A.: Radiative and convective energy from wood crib fires, Pyrodynamics, 2, 65&amp;ndash;85, 1965. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Mullendore, G.&amp;nbsp;L., Durran, D.&amp;nbsp;R., and Holton, J.&amp;nbsp;R.: Cross-tropopause tracer transport in midlatitude convection, J. Geophys. Res., 110, D06113, doi:10.1029/2004JD005059, 2005. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> Oberhuber, J.&amp;nbsp;M., Herzog, M., Graf, H.-F., and Schwanke, K.: Volcanic plume simulation on large scales, J. Volcanol. Geotherm. Res., 87, 29&amp;ndash;53, 1998. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> Packham, D.&amp;nbsp;R.: Heat transfer above a small ground fire, Aust. For. Res., 5, 19&amp;ndash;24, 1969. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> Penner, J.&amp;nbsp;E., Haselman, Jr., L.&amp;nbsp;C., and Edwards, L.&amp;nbsp;L.: Smoke-Plume Distribution above Large-Scale Fires: Implications for Simulations of &quot;Nuclear Winter&quot;, J. Climate and Appl. Meteorol., 25, 1434&amp;ndash;1444, 1986. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> Potter, B.&amp;nbsp;E.: The role of released moisture in the atmospheric dynamics associated with wildland fires, Int. J. Wildland Fire, 14, 77&amp;ndash;84, 2005. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> Pruppacher, H.&amp;nbsp;R. and Klett, J.&amp;nbsp;D.: Microphysics of Clouds and Precipitation, Kluwer Academic Publishers, 1997.  </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> Reid, J.&amp;nbsp;S., Koppmann, R., Eck, T.&amp;nbsp;F., and Eleuterio, D.&amp;nbsp;P.: A review of biomass burning emissions part II: intensive physical properties of biomass burning particles, Atmos. Chem. Phys., 5, 799&amp;ndash;825, 2005. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> Robock, A.: Volcanic Eruptions and Climate, Rev. Geophys., 38, 191&amp;ndash;219, 2000. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> Rosenfeld, D.: Suppression of rain and snow by urban and industrial air pollution, Sci., 287, 1793&amp;ndash;1796, 2000.  </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> Rosenfeld, D., Fromm, M., Trentmann, J., Luderer, G., Andreae, M.&amp;nbsp;O., and Servranckx, R.: The Chisholm firestorm: observed microstructure, precipitation and lightning activity of a pyro-Cb, Atmos. Chem. Phys. Discuss., 6, 9877&amp;ndash;9906, 2006. </mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple"> Rosenfeld, D. and Woodley, W.&amp;nbsp;L.: Deep convective clouds with sustained supercooled liquid water down to &amp;minus;37.5&amp;deg;C, Nature, 405, 440&amp;ndash;442, 2000. </mixed-citation>
</ref>
<ref id="ref36">
<label>36</label><mixed-citation publication-type="other" xlink:type="simple"> Simmel, M. and Wurzler, S.: Condensation and activation in sectional cloud microphysical models, Atmos. Res., 80, 218&amp;ndash;236, 2006. </mixed-citation>
</ref>
<ref id="ref37">
<label>37</label><mixed-citation publication-type="other" xlink:type="simple"> Small, R.&amp;nbsp;D. and Heikes, K.&amp;nbsp;E.: Early cloud formation by large area fires, J. Appl. Meteorol., 27, 654&amp;ndash;663, 1988. </mixed-citation>
</ref>
<ref id="ref38">
<label>38</label><mixed-citation publication-type="other" xlink:type="simple"> Textor, C., Graf, H.&amp;nbsp;F., Herzog, M., Oberhuber, J.&amp;nbsp;M., Rose, W.&amp;nbsp;I., and Ernst, G. G.&amp;nbsp;J.: Volcanic particle aggregation in explosive eruption columns. Part I: Parameterization of the microphysics of hydrometeors and ash, J. Volcanol. Geotherm. Res, 150, 359&amp;ndash;377, 2006a. </mixed-citation>
</ref>
<ref id="ref39">
<label>39</label><mixed-citation publication-type="other" xlink:type="simple"> Textor, C., Graf, H.&amp;nbsp;F., Herzog, M., Oberhuber, J.&amp;nbsp;M., Rose, W.&amp;nbsp;I., and Ernst, G. G.&amp;nbsp;J.: Volcanic particle aggregation in explosive eruption columns. Part II: Numerical experiments, J. Volcanol. Geotherm. Res., 150, 378&amp;ndash;394, 2006b. </mixed-citation>
</ref>
<ref id="ref40">
<label>40</label><mixed-citation publication-type="other" xlink:type="simple"> Trentmann, J., Luderer, G., Winterrath, T., Fromm, M., Servranckx, R., Textor, C., Herzog, M., and Andreae, M.&amp;nbsp;O.: Modeling of biomass smoke injection into the lower stratosphere by a large forest fire (Part I): Reference study, Atmos. Chem. Phys., 6, 5247&amp;ndash;5260, 2006. </mixed-citation>
</ref>
<ref id="ref41">
<label>41</label><mixed-citation publication-type="other" xlink:type="simple"> Waibel, A.&amp;nbsp;E., Fischer, H., Wienhold, F.&amp;nbsp;G., Siegmund, P.&amp;nbsp;C., Lee, B., Stroem, J., Lelieveld, J., and Crutzen, P.&amp;nbsp;J.: Highly elevated carbon monoxide concentrations in the upper troposphere and lowermost stratosphere at northern midlatitudes during the STREAM II summer campaign in 1994, Chemosphere &amp;ndash; Global Change Sci., 1, 233&amp;ndash;248, 1999. </mixed-citation>
</ref>
<ref id="ref42">
<label>42</label><mixed-citation publication-type="other" xlink:type="simple"> Wang, C.: A modeling study of the response of tropical deep convection to the increase of cloud condensation nuclei concentration: 1. Dynamics and microphysics, J. Geophys. Res., 110, doi:10.1029/2004JD005720, 2005. </mixed-citation>
</ref>
<ref id="ref43">
<label>43</label><mixed-citation publication-type="other" xlink:type="simple"> Wang, P.&amp;nbsp;K.: Moisture plumes above thunderstorm anvils and their contributions cross-tropopause transport of water vapor in midlatitudes, J. Geophys. Res., 108, 4194, doi:10.1029/2002JD002581, 2003. </mixed-citation>
</ref>
</ref-list>
</back>
</article>