<?xml version="1.0" encoding="utf-8" standalone="no"?>
<!DOCTYPE article SYSTEM "http://www.atmos-chem-phys.net/inc/acp/copernicus.dtd">
<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics</journal_title>
		<journal_url>www.atmos-chem-phys.net</journal_url>
		<issn>1680-7316</issn>
		<eissn>1680-7324</eissn>
		<volume_number>6</volume_number>
		<issue_number>11</issue_number>
		<publication_year>2006</publication_year>
	</journal>
	<doi>10.5194/acp-6-3583-2006</doi>
	<article_url>http://www.atmos-chem-phys.net/6/3583/2006/</article_url>
	<abstract_html>http://www.atmos-chem-phys.net/6/3583/2006/acp-6-3583-2006.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys.net/6/3583/2006/acp-6-3583-2006.pdf</fulltext_pdf>
	<start_page>3583</start_page>
	<end_page>3601</end_page>
	<publication_date>2006-09-04</publication_date>
	<article_title content_type="html">Combined observational and modeling based study of the aerosol indirect effect</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>T. Storelvmo</name>
			<email>trude.storelvmo@geo.uio.no</email>
		</author>
		<author numeration="2" affiliations="1">
			<name>J. E. Kristjánsson</name>
		</author>
		<author numeration="3" affiliations="1,2">
			<name>G. Myhre</name>
		</author>
		<author numeration="4" affiliations="2">
			<name>M. Johnsrud</name>
		</author>
		<author numeration="5" affiliations="1">
			<name>F. Stordal</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Department of Geosciences, University of Oslo, Oslo, Norway</affiliation>
		<affiliation numeration="2" content_type="html">Norwegian Institute for Air Research, Kjeller, Norway</affiliation>
	</affiliations>
	<abstract content_type="html">The indirect effect of aerosols via liquid clouds is
investigated by comparing aerosol and cloud characteristics from the Global
Climate Model CAM-Oslo to those observed by the MODIS instrument onboard the
TERRA and AQUA satellites http://modis.gsfc.nasa.gov). The comparison is
carried out for 15 selected regions ranging from remote and clean to densely
populated and polluted. For each region, the regression coefficient and
correlation coefficient for the following parameters are calculated: Aerosol
Optical Depth vs. Liquid Cloud Optical Thickness, Aerosol Optical Depth vs. Liquid
Cloud Droplet Effective Radius and Aerosol Optical Depth vs. Cloud
Liquid Water Path. Modeled and observed correlation coefficients and
regression coefficients are then compared for a 3-year period starting in
January 2001. Additionally, global maps for a number of aerosol and cloud
parameters crucial for the understanding of the aerosol indirect effect are
compared for the same period of time. Significant differences are found
between MODIS and CAM-Oslo both in the regional and global comparison.
However, both the model and the observations show a positive correlation
between Aerosol Optical Depth and Cloud Optical Depth in practically all
regions and for all seasons, in agreement with the current understanding of
aerosol-cloud interactions. The correlation between Aerosol Optical Depth
and Liquid Cloud Droplet Effective Radius is variable both in the model and
the observations. However, the model reports the expected negative
correlation more often than the MODIS data. Aerosol Optical Depth is overall
positively correlated to Cloud Liquid Water Path both in the model and the
observations, with a few regional exceptions.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Abdul-Razzak, H. and Ghan, S.: A parameterization of aerosol activation, 2. Multiple aerosol type, J. Geophys. Res., 105, 6837&amp;ndash;6844, 2000.  </reference>
		<reference numeration="2" content_type="text"> Albrecht, B. A.: Aerosols, cloud microphysics, and fractional cloudiness, Science, 245, 1227&amp;ndash;1230, 1989. </reference>
		<reference numeration="3" content_type="text"> Andreae, M. O., Rosenfeld, D., Artaxo, P., Costa, A. A., Frank, G. P., Longo, K. M., and Silvas-Dias, M. A. F.: Smoking rain clouds over the Amazon, Science, 303, 1337&amp;ndash;1342, 2004. </reference>
		<reference numeration="4" content_type="text"> Bréon, F. M., Tanré, D., and Generoso, S.: Aerosol Effect on Cloud Droplet Size Monitored from Satellite, Science, 295, 834&amp;ndash;838, 2002. </reference>
		<reference numeration="5" content_type="text"> Ghan, S. J., Easter, R. C., Hudson, J., and Bréon, F. M.: Evaluation of aerosol indirect radiative forcing in MIRAGE, J. Geophys. Res., 106, 5317&amp;ndash;5334, 2001. </reference>
		<reference numeration="6" content_type="text"> Ghan, S. J., Guzman, G., and Abdul-Razzak, H.: Competition between Sea Salt and Sulfate Particles as Cloud Condensation Nuclei, J. Atmos. Sci., 55, 3340&amp;ndash;3347, 1998. </reference>
		<reference numeration="7" content_type="text"> Hansen, J., Sato, M., and Ruedy, R.: Radiative forcing and climate response, J. Geophys. Res., 102, 6831&amp;ndash;6864, 1997. </reference>
		<reference numeration="8" content_type="text"> Han, Q., Rossow, W. B., and Lacis, A. A.: Near-global survey survey of effective droplet radii in liquid water clouds using ISCCP data, J. Climate, 7, 465&amp;ndash;497, 1994. </reference>
		<reference numeration="9" content_type="text"> Iversen, T. and Seland, Ø.: A scheme for process-tagged SO&lt;sub&gt;4&lt;/sub&gt; and BC aerosols in NCAR CCM3. Validation and sensitivity to cloud processes, J. Geophys. Res., 107(D24), 4751, doi:10.1029/2001JD000885, 2002. </reference>
		<reference numeration="10" content_type="text"> Jaenicke, R.: Abundance of Cellular Material and Proteins in the Atmosphere, Science, 308, 73, 2005. </reference>
		<reference numeration="11" content_type="text"> Kaufman, Y. J., Tanré, D., Remer, E. F., Vermote, A., Chu, B. N., and Holben, B. N.: Operational remote sensing of tropospheric aerosol over land from EOS moderate resolution imaging spectroradiometer, J. Geophys. Res., 102(D14), 17 051&amp;ndash;17 068, doi:10.1029/96JD03988, 1997. </reference>
		<reference numeration="12" content_type="text"> Kaufman, Y. J. and Koren, I.: Smoke and Pollution Aerosol Effect on Cloud Cover, Science, 313, 655&amp;ndash;658, 2006. </reference>
		<reference numeration="13" content_type="text"> Kanakidou, M., Seinfeld, J. H., Pandis, S. N., Barnes, I., Dentener, F. J., Facchini, M. C., van Dingenen, R., Ervens, B., Nenes, A., Nielsen, C. J., Swietlicki, E., Putaud, J. P., Balkanski, Y., Fuzzi, S., Horth, J., Moortgat, G. K., Winterhalter, R., Myhre, C. E. L., Tsigaridis, K., Vignati, E., Stephanou, E. G., and Wilson, J.: Organic aerosol and climate modelling: A review, Atmos Chem. Phys., 5, 1053&amp;ndash;1123, 2005. </reference>
		<reference numeration="14" content_type="text"> Kirkev&amp;aring;g, A. and Iversen, T.: Global direct radiative forcing by process-parameterized aerosol optical properties, J. Geophys. Res., 107(D20), 4433, doi:10.1029/2001JD000886, 2002. </reference>
		<reference numeration="15" content_type="text"> Kirkev&amp;aring;g, A., Iversen, T., Seland, Ø., and Kristjánsson, J. E.: Revised schemes for aerosol optical parameters and cloud condensation nuclei, Institute Report Series, No. 128, Department of Geosciences, University of Oslo, 2005. </reference>
		<reference numeration="16" content_type="text"> Kristjánsson, J. E.: Studies of the aerosol indirect effect from sulfate and black carbon aerosols, J. Geophys. Res., 107(D20), 4246, doi:10.1029/2001JD000887, 2002. </reference>
		<reference numeration="17" content_type="text"> Liou, K.-N.: Radiation and cloud processes in the atmosphere, Oxford University Press, 487 pp., 1992. </reference>
		<reference numeration="18" content_type="text"> Lohmann, U. and Feichter, J.: Global indirect aerosol effects: a review, Atmos. Chem. Phys., 5, 715&amp;ndash;737, 2005.  </reference>
		<reference numeration="19" content_type="text"> Lohmann, U., Feichter, J., Chuang, C. C., and Penner, J. E.: Predicting the number of cloud droplets in the ECHAM GCM, J. Geophys. Res. 104, 9169&amp;ndash;9198, 1999. </reference>
		<reference numeration="20" content_type="text"> Marshak, A., Platnick, S., Varnai, T., Wen, G., and Cahalan, R. F.: Impact of 3D radiative effects on satellite retrievals of cloud droplet sizes, J. Geophys. Res., 111, D09207, doi:10.1029/2005JD006686, 2006.  </reference>
		<reference numeration="21" content_type="text"> Myhre, G., Stordal, F., Johnsrud, M., Kaufman, Y. J., Rosenfeld, D., Storelvmo, T., Kristjánsson, J. E., Berntsen, T. K., Myhre, A., and Isaksen, I. S. A.: Aerosol-cloud interaction inferred from MODIS satellite data and global aerosol models, Atmos. Chem. Phys. Discuss., accepted, 2006. </reference>
		<reference numeration="22" content_type="text"> Nakajima, T., Higurashi, A., Kazuaki, K., and Penner, J. E.: A possible correlation between satellite-derived cloud and aerosol microphysical parameters, Geophys. Res. Lett., 28, 1171&amp;ndash;1174, 2001. </reference>
		<reference numeration="23" content_type="text"> Penner, J. E., Andreae, M., Annegarn, H., Barrie, L., Feichter, J., Hegg, D., Jayaraman, A., Leaicht, R., Murphy, D., Nganga, J., and Pitari, G.: Aerosols, their direct and indirect effects, Chapter 5 (p. 289&amp;ndash;348) in: Climate change 2001: The scientific basis. Contribution of working group~I to the Third Assessment Report of the Intergovernmental Panel on Climate Change. Cambridge University Press, 2001. </reference>
		<reference numeration="24" content_type="text"> Platnick, S., King, M. D., Ackerman, S. A., Menzel, W. P., Baum, B. A., Riédi, J. C., and Frey, R. A.: The MODIS cloud products: Algorithms and examples from Terra, IEEE Trans. Geosci. Remote Sensing, 41, 459&amp;ndash;473, 2003. </reference>
		<reference numeration="25" content_type="text"> Quaas, J., Boucher, O., and Bréon, F.-M.: Aerosol indirect effects in POLDER satellite data and in the LMDZ general circulation model, J. Geophys. Res., 109, D08205, doi:10.1029/2003JD004317, 2004. </reference>
		<reference numeration="26" content_type="text"> Quaas, J., Boucher, O., and Lohmann, U.: Constraining the total aerosol indirect effect in the LMDZ and ECHAM4 GCMs using MODIS satellite data, Atmos. Chem. Phys., 6, 947&amp;ndash;955, 2006. </reference>
		<reference numeration="27" content_type="text"> Remer, L. A., Kaufman, Y. J., Mattoo, S., Martins, J. V., Ichoku, C., Levy, R. C., Kleidman, R., Tanré, D., Chu, D. A., Li, R. R., Eck, T. F., Vermote, E., and Holben, B. N.: The MODIS algorithm, products and validation, J. Atmos. Sci., 62, 947&amp;ndash;973, doi:10.1175/JAS3385.1, 2005. </reference>
		<reference numeration="28" content_type="text"> Rosenfeld, D., Lahav, R., Khain, A., and Pinsky, M.: The role of Sea Spray in Cleansing Air Pollution over Ocean via Cloud Processes, Science, 297, 1667&amp;ndash;1670, 2002. </reference>
		<reference numeration="29" content_type="text"> Sekiguchi, M., Nakajima, T., Suzuki, K., Kawamoto, K., Higurashi, A., Rosenfeld, D., Sano, I., and Mukai, S.: A study of the direct and indirect effects of aerosols using global satellite data sets of aerosol and cloud parameters, J. Geophys. Res., 108(D22), 4699, doi:10.1029/2002JD003359, 2003. </reference>
		<reference numeration="30" content_type="text"> Slingo, A.: A GCM parameterization for the shortwave properties of water clouds, J. Atmos. Sci., 46, 1419&amp;ndash;1427, 1989. </reference>
		<reference numeration="31" content_type="text"> Storelvmo, T., Kristjánsson, J. E., Ghan, S. J., Kirkev&amp;aring;g, A., Seland, Ø., and Iversen, T.: Predicting cloud droplet number concentration in CAM-Oslo, J. Geophys. Res., in press, 2006. </reference>
		<reference numeration="32" content_type="text"> Tanré, D., Kaufman, Y. J., Herman, M., and Mattoo, S.: Remote sensing of aerosol properties over oceans using the MODIS/EOS spectral radiances, J. Geophys. Res., 102, 16 971&amp;ndash;16 988, 1997. </reference>
		<reference numeration="33" content_type="text"> Twomey, S.: The influence of pollution on shortwave albedo of clouds, J. Atmos. Sci., 34, 1149&amp;ndash;1152, 1977. </reference>
		<reference numeration="34" content_type="text"> Wetzel, M. A. and Stowe, L. L.: Satellite-observed patterns in stratus microphysics, aerosol optical thickness, and shortwave radiative forcing, J. Geophys. Res, 104, 31 287&amp;ndash;31 299, 1999. </reference>
	</references>
</article>

