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<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics</journal_title>
		<journal_url>www.atmos-chem-phys.net</journal_url>
		<issn>1680-7316</issn>
		<eissn>1680-7324</eissn>
		<volume_number>6</volume_number>
		<issue_number>10</issue_number>
		<publication_year>2006</publication_year>
	</journal>
	<doi>10.5194/acp-6-2991-2006</doi>
	<article_url>http://www.atmos-chem-phys.net/6/2991/2006/</article_url>
	<abstract_html>http://www.atmos-chem-phys.net/6/2991/2006/acp-6-2991-2006.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys.net/6/2991/2006/acp-6-2991-2006.pdf</fulltext_pdf>
	<start_page>2991</start_page>
	<end_page>3006</end_page>
	<publication_date>2006-07-21</publication_date>
	<article_title content_type="html">Some ice nucleation characteristics of Asian and Saharan desert dust</article_title>
	<authors>
		<author numeration="1" affiliations="1,6">
			<name>P. R. Field</name>
			<email>prfield@ucar.edu</email>
		</author>
		<author numeration="2" affiliations="2">
			<name>O. Möhler</name>
		</author>
		<author numeration="3" affiliations="3">
			<name>P. Connolly</name>
		</author>
		<author numeration="4" affiliations="4">
			<name>M. Krämer</name>
		</author>
		<author numeration="5" affiliations="1">
			<name>R. Cotton</name>
		</author>
		<author numeration="6" affiliations="5">
			<name>A. J. Heymsfield</name>
		</author>
		<author numeration="7" affiliations="2">
			<name>H. Saathoff</name>
		</author>
		<author numeration="8" affiliations="2">
			<name>M. Schnaiter</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Met Office, Exeter, UK</affiliation>
		<affiliation numeration="2" content_type="html">Institute for Meteorology and Climate Research (IMK-AAF), Forschungszentrum Karlsruhe, Germany</affiliation>
		<affiliation numeration="3" content_type="html">School of Earth, Atmospheric and Environmental Sciences, University of Manchester, Manchester, UK</affiliation>
		<affiliation numeration="4" content_type="html">Institute of Chemistry and Dynamics of the Geosphere (ICG-I), Forschungszentrum Jülich, Germany</affiliation>
		<affiliation numeration="5" content_type="html">NCAR, Boulder, CO, USA</affiliation>
		<affiliation numeration="6" content_type="html">now at: NCAR, Boulder, CO, USA</affiliation>
	</affiliations>
	<abstract content_type="html">The large (7 m&amp;times;4 m cylinder, 84 m&lt;sup&gt;3&lt;/sup&gt;) AIDA (Aerosol Interactions
and Dynamics in the Atmosphere) cloud chamber facility at Forschungszentrum,
Karlsruhe, Germany was used to test the ice nucleating ability of two desert
dust samples from the Sahara and Asia. Aerosol samples were lognormally
distributed with a mode diameter of 0.4(&amp;plusmn;0.1) μm and geometric
standard deviation of ~1.7(&amp;plusmn;0.2). At temperatures warmer than
&amp;minus;40&amp;deg;C droplets were formed before ice crystals formed and there was
generally no deposition nucleation observed. At temperatures colder than
&amp;minus;40&amp;deg;C both dust samples exhibited dual nucleation events that were
observed during the same expansion experiment. The primary nucleation event
occurred at ice saturation ratios of 1.1 to 1.3 and is likely to be a
deposition nucleation mode. The secondary nucleation event occurred at ice
saturation ratios between 1.35 and 1.5. We cannot categorically determine
whether this ice nucleation event is via a further deposition mode or a
condensation mode, but the presence of some soluble material in the dust
samples leads us to favour the latter process. The activated fractions of
desert dust ranged from ~5&amp;ndash;10% at &amp;minus;20&amp;deg;C to 20&amp;ndash;40% at
temperatures colder than &amp;minus;40&amp;deg;C. There was no obvious difference
between the nucleation behaviour of the two dust samples.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Archuleta, C. M., DeMott, P. J., and Kreidenweis, S. M.: Ice nucleation by surrogates for atmospheric mineral dust/sulfate particles at cirrus temperatures. Atmos. Chem. Phys., 5, 3391&amp;ndash;3436, 2005. </reference>
		<reference numeration="2" content_type="text"> Bailey, M. and Hallett, J.: Nucleation effects on the habit of vapour grown ice crystals from $-$18 to $-$42$^\circ$C  Quart. J. Royal Meteorol. Soc., 128, 1461&amp;ndash;1483, 2002 </reference>
		<reference numeration="3" content_type="text"> Bailey, M. and Hallett, J.:  Growth rates and habits of ice crystals between $-$20 degrees and  $-$70$^\circ$C,  J. Atmos. Sci., 61(5), 514&amp;ndash;544, 2004. </reference>
		<reference numeration="4" content_type="text"> Cantrell, W. and Heymsfield, A. J.:  Production of ice in tropospheric clouds &amp;ndash; A review,  Bull. Am. Meteorol. Soc., 86(6), 795&amp;ndash;807, 2005. % </reference>
		<reference numeration="5" content_type="text">  </reference>
		<reference numeration="6" content_type="text"> Cotton, R. J. and Field, P. R.: Ice nucleation characteristics of an isolated wave cloud, Q. J. Roy. Meteorol. Soc., 128, 2417&amp;ndash;2437, 2002. </reference>
		<reference numeration="7" content_type="text"> Cziczo, D. J., Murphy, D. M., Hudson, P. K., and Thomson, D. S.: Single particle measurements of the chemical composition of cirrus ice residue during CRYSTAL-FACE, J. Geophys. Res., 109(D4), D04201, doi:10.1029/2003JD004032, 2004. </reference>
		<reference numeration="8" content_type="text"> DeMott, P. J., Sassen, K., Poellot, M. R., Baumgardner, D., Rogers, D. C., Brooks, S. D., Prenni, A. J., and Kreidenweis, S. M.: African dust aerosols as atmospheric ice nuclei Geophys. Res. Lett., 30(14), 1732, doi:10.1029/2003GL017410, 2003. </reference>
		<reference numeration="9" content_type="text"> Durant, A. J. and Shaw, R. A.:  Evaporation freezing by contact nucleation inside-out  Geophys. Res. Lett., 32(20), L20814, doi:10.1029/2005GL024175, 2005.  </reference>
		<reference numeration="10" content_type="text"> Fan, S. M., Moxim, W. J., and Hiram, L.: Implications of droplet nucleation to mineral dust aerosol deposition and transport, Geophys. Res. Lett., 32, 10, L10805, doi:10.1029/2005GL022833, 2005. </reference>
		<reference numeration="11" content_type="text"> Field, P. R., Cotton, R. J., Noone, K., et al.:  Ice nucleation in orographic wave clouds: Measurements made during  INTACC,  Quart. J. Royal Meteorol. Soc., 127, 1493&amp;ndash;1512, 2001. </reference>
		<reference numeration="12" content_type="text"> Field, P. R., Hogan, R. J., Brown, P. R. A., Illingworth, A. J., Choularton, T. W., Kaye, P. H., Hirst, E., and Greenaway, R.: Simultaneous radar and aircraft observations of mixed-phase cloud at the 100 m scale, Quart. J. Royal Meteorol. Soc., 130, 1877&amp;ndash;1904, 2004. </reference>
		<reference numeration="13" content_type="text"> Gettelman, A., Fetzer, E. J., Eldering, A., and Irion, F. W.: The Global Distribution of Supersaturation in the Upper Troposphere from the Atmospheric Infrared Sounder, J. Climate, in press, 2006. </reference>
		<reference numeration="14" content_type="text"> Hirst, E., Kaye, P. H., Greenaway, R. S., Field, P., and Johnson, D. W.: Discrimination of micrometre-sized ice and super-cooled droplets in mixed-phase cloud, Atmos. Env., 35, 33&amp;ndash;47 2001. </reference>
		<reference numeration="15" content_type="text"> Hung, H.-M., Malinowski, A., and Martin, S. T.: Kinetics of heterogeneous ice nucleation on the surfaces of mineral dust cores inserted into aqueous ammonium sulfate particles, J. Phys. Chem. A., 107, 1296&amp;ndash;1306, 2003. </reference>
		<reference numeration="16" content_type="text"> Isono, K., Komabayasi, M., and Ono, A.: The nature and origin of ice nuclei in the atmosphere, J. Meteor. Soc. Japan, 37, 211&amp;ndash;233, 1959. </reference>
		<reference numeration="17" content_type="text"> Jensen, E., Starr, D., and Toon, O. B.: Mission investigates tropical cirrus clouds, EOS, 85, 45&amp;ndash;50, 2004.  </reference>
		<reference numeration="18" content_type="text"> Lohmann, U. and Feichter, J.: Global indirect aerosol effects: a review, Atmos. Chem. Phys., 5, 715&amp;ndash;737, 2005. </reference>
		<reference numeration="19" content_type="text"> Lohmann, U. and Kärcher, B.:  First interactive simulations of cirrus clouds formed by homogeneous freezing in the ECHAM general circulation model,  J. Geophys. Res., 107(D10), 4105, doi:10.1029/2001JD000767, 2002.  </reference>
		<reference numeration="20" content_type="text"> Möhler, O., Stetzer, O., Schaefers, S., Linke, C., Schnaiter, M., Tiede, R., Saathoff, H., Krämer, M., Mangold, A., Budz, P., Zink, P., Schreiner, J., Mauersberger, K., Haag, W., Kärcher, B., and Schurath, U.: Experimental investigation of homogeneous freezing of sulphuric acid particles in the aerosol chamber AIDA, Atmos. Chem. Phys., 3, 211&amp;ndash;223, 2003. </reference>
		<reference numeration="21" content_type="text"> Möhler, O., Benz, S., Saathoff, H., Connolly, P., Krämer, M., Mangold, A., Field, P., and Heymsfield, A.: Efficiency of the deposition mode of ice nucleation on mineral dust particles, Atmos. Chem. Phys., 6, 3007&amp;ndash;3021, 2006. </reference>
		<reference numeration="22" content_type="text"> Pruppacher, H. R. and Klett, D. J.: Microphysics of clouds and precipitation, Kluwer, Netherlands, 954pp., 1997. </reference>
		<reference numeration="23" content_type="text"> Roberts, P. and Hallett, J.: A laboratory study of the ice nucleating properties of some mineral particulates, Quart. J. Roy. Meteorol. Soc., 94, 25&amp;ndash;34, 1968. </reference>
		<reference numeration="24" content_type="text"> Salam, A., Lohmann, U., Crenna, B., Lesins G., Klages, P., Rogers, D., Irani, R., MacGillivray, A., and Coffin, M.: Ice nucleation studies of mineral dust particles with a new continuous flow diffusion chamber, Aer. Sci. Tech., 40(2), 134&amp;ndash;143, 2006. </reference>
		<reference numeration="25" content_type="text"> Sassen, K., DeMott, P. J., Prospero, J. M., and Poellot, M. R.: Saharan dust storms and indirect aerosol effects on clouds: CRYSTAL-FACE results, Geophys. Res. Lett., 30(12), 1633, doi:10.1029/2003GL017371, 2003. </reference>
		<reference numeration="26" content_type="text"> Stocker, T., Clarke, G. K. C., Le Treut, H., Lindzen, R. S., Meleshko, V. P., Mugara, R. K., Palmer, T. N., Pierrehumbert, R. T., Sellers, P. J., Trenberth, K. E., and Willebrand, J.: Physical Climate Processes and Feedbacks, Chapter 7 of Climate Change 2001: The Scientific Basis, edited by: Houghton, J. T., Ding, Y., Griggs, D. J., Noguer, M., van der Linden, P. J., Dai, X., Maskell, K., and Johnson, C. A., Cambridge University Press, Cambridge, UK, 2001.  </reference>
		<reference numeration="27" content_type="text"> Targino, A. C., Krejci, R., Noone K. J., and Glantz, P.: Single particle analysis of ice crystal residuals observed in orographic wave clouds over Scandinavia during INTACC experiment, Atmos. Chem. Phys., 6, 1977&amp;ndash;1990, 2006. </reference>
		<reference numeration="28" content_type="text"> Twohy, C. H. and Poellot, M. R.: Chemical characteristics of ice residual nuclei in anvil cirrus clouds: evidence for homogeneous and heterogeneous ice formation, Atmos. Chem. Phys., 5, 2289&amp;ndash;2297, 2005. </reference>
		<reference numeration="29" content_type="text"> Vali, G.: Nucleation Terminology, Bull. Am. Meteorol. Soc., 66, 1426&amp;ndash;1427, 1985. </reference>
		<reference numeration="30" content_type="text"> Zuberi, B., Bertram, A. K., Cassa, C. A., Molina, L. T., and Molina, M. J.: Heterogeneous nucleation of ice in \chem(NH_4)(2)SO_4-H_2O particles with mineral dust immersions, Geophys. Res. Lett., 29(10) 1504, doi:10.1029/2001GL014289, 2002.  </reference>
	</references>
</article>

