<?xml version="1.0" encoding="utf-8" standalone="no"?>
<!DOCTYPE article SYSTEM "http://www.atmos-chem-phys.net/inc/acp/copernicus.dtd">
<article language="en">
	<journal>
		<journal_title>Atmospheric Chemistry and Physics</journal_title>
		<journal_url>www.atmos-chem-phys.net</journal_url>
		<issn>1680-7316</issn>
		<eissn>1680-7324</eissn>
		<volume_number>6</volume_number>
		<issue_number>10</issue_number>
		<publication_year>2006</publication_year>
	</journal>
	<doi>10.5194/acp-6-2793-2006</doi>
	<article_url>http://www.atmos-chem-phys.net/6/2793/2006/</article_url>
	<abstract_html>http://www.atmos-chem-phys.net/6/2793/2006/acp-6-2793-2006.html</abstract_html>
	<fulltext_pdf>http://www.atmos-chem-phys.net/6/2793/2006/acp-6-2793-2006.pdf</fulltext_pdf>
	<start_page>2793</start_page>
	<end_page>2810</end_page>
	<publication_date>2006-07-10</publication_date>
	<article_title content_type="html">Development of a cloud microphysical model and parameterizations to describe the effect of CCN on warm cloud</article_title>
	<authors>
		<author numeration="1" affiliations="1">
			<name>N. Kuba</name>
			<email>kuba@jamstec.go.jp</email>
		</author>
		<author numeration="2" affiliations="2">
			<name>Y. Fujiyoshi</name>
		</author>
	</authors>
	<affiliations>
		<affiliation numeration="1" content_type="html">Frontier Research Center for Global Change (FRCGC), Japan Agency for Marin-Earth Science and Technology (JAMSTEC), Yokohama, Japan</affiliation>
		<affiliation numeration="2" content_type="html">Frontier Research Center for Global Change (FRCGC), Japan Agency for Marin-Earth Science and Technology (JAMSTEC)/Inst. Low. Temp. Sci., Hokkaido Univ., Sapporo, Japan</affiliation>
	</affiliations>
	<abstract content_type="html">First, a hybrid cloud microphysical model was developed that incorporates
both Lagrangian and Eulerian frameworks to study quantitatively the effect
of cloud condensation nuclei (CCN) on the precipitation of warm clouds. A
parcel model and a grid model comprise the cloud model. The condensation
growth of CCN in each parcel is estimated in a Lagrangian framework. Changes
in cloud droplet size distribution arising from condensation and coalescence
are calculated on grid points using a two-moment bin method in a
semi-Lagrangian framework. Sedimentation and advection are estimated in the
Eulerian framework between grid points. Results from the cloud model show
that an increase in the number of CCN affects both the amount and the area
of precipitation. Additionally, results from the hybrid microphysical model
and Kessler&apos;s parameterization were compared.

Second, new parameterizations were developed that estimate the number and
size distribution of cloud droplets given the updraft velocity and the
number of CCN. The parameterizations were derived from the results of
numerous numerical experiments that used the cloud microphysical parcel
model. The input information of CCN for these parameterizations is only
several values of CCN spectrum (they are given by CCN counter for example).
It is more convenient than conventional parameterizations those need values
concerned with CCN spectrum, &lt;i&gt;C&lt;/i&gt; and &lt;i&gt;k&lt;/i&gt; in the equation of N=CS&lt;sup&gt;&lt;i&gt;k&lt;/i&gt;&lt;/sup&gt;, or, breadth,
total number and median radius, for example. The new parameterizations&apos;
predictions of initial cloud droplet size distribution for the bin method
were verified by using the aforesaid hybrid microphysical model. The newly
developed parameterizations will save computing time, and can effectively
approximate components of cloud microphysics in a non-hydrostatic cloud
model. The parameterizations are useful not only in the bin method in the
regional cloud-resolving model but also both for a two-moment bulk
microphysical model and for a global model. The effects of sea salt,
sulfate, and organic carbon particles were also studied with these
parameterizations and global model.</abstract>
	<references>
		<reference numeration="1" content_type="text"> Albrecht, B. A., Bretherton, C. S., Johnson, D., Scubert, W. H., and Frisch, A. S.: The Atlantic stratocumulus transition experiment &amp;ndash; ASTEX, Bull. Am. Meteorol. Soc., 76, 889&amp;ndash;904, 1995. </reference>
		<reference numeration="2" content_type="text"> Andreae, M. O., Rosenfeld, D., Artaxo, P., Costa, A. A., Frank, G. P., Longo, K. M., and Silva-Dias, M. A. F.: Smoking rain clouds over the Amazon, Science, 303, 1337&amp;ndash;1342, 2004. </reference>
		<reference numeration="3" content_type="text"> Bott, A.: A flux method for the numerical solution of the stochastic collection equation, J. Atmos. Sci., 55, 2284&amp;ndash;2293, 1998. </reference>
		<reference numeration="4" content_type="text"> Chen, J. -P. and Lamb, D.: Simulation of cloud microphysics and chemical processes using a multicomponent framework. Part I Description of the microphysical model, J. Atmos. Sci. 51, 2613&amp;ndash;2630, 1994. </reference>
		<reference numeration="5" content_type="text"> Chen, J. -P. and Lamb, D.: Simulation of cloud microphysics and chemical processes using a multicomponent framework. Part II Microphysical evolution of a wintertime orographic cloud, J. Atmos. Sci., 56, 2293&amp;ndash;2312, 1999. </reference>
		<reference numeration="6" content_type="text"> Chen, J.-P. and Liu, S.-T.: Physically based two-moment bulkwater parametrization for warm-cloud microphysics, Q. J. R. Meteorol. Soc., 130, 51&amp;ndash;78, 2004. </reference>
		<reference numeration="7" content_type="text"> Chuang, P. Y., Charlson, R. J., and Seinfeld, J. H.: Kinetic limitations on droplet formation in clouds, Nature, 390, 11, 595&amp;ndash;596, 1997. </reference>
		<reference numeration="8" content_type="text"> Clark, T. L.: Numerical modeling of the dynamics and microphysics of warm cumulus convection, J. Atmos. Sci., 30, 857&amp;ndash;878, 1973. </reference>
		<reference numeration="9" content_type="text"> Cooper, W. A., Bruintjes, R. T., and Mather, G. K.: Calculating pertaining to hygrospic seeding with flares, J. Appl. Meteor., 36, 1449&amp;ndash;1469, 1997. </reference>
		<reference numeration="10" content_type="text"> Cotton, W. R. and Anthes, R. A.: Storm and Cloud Dynamics (Chapter 4), Academic Press, 880pp., 1989. </reference>
		<reference numeration="11" content_type="text"> Cotton, W. R., Pielke, R. A. Sr., Walco, R. L., Liston G. E., Tremback, C. J., Jiang, H., McAnelly, R. L., Harringto, J. Y., Nicholls, M. E., Carrio, G. G., and McFadde, J. P.: RAMS 2001: Current status and future directions, Meteorol. Atmos. Phys., 82, 5&amp;ndash;29, 2003. </reference>
		<reference numeration="12" content_type="text"> Feingold, G., Cotton, W. R., Kreidenwei, S. M., and Davis, J. T.: The impact of giant cloud condensation nuclei on drizzle formation in stratocumulus: Implications for cloud radiative properties, J. Atmos. Sci., 56, 15, 4100&amp;ndash;4117, 1999. </reference>
		<reference numeration="13" content_type="text"> Fitzgerald, J. W.: Effect of aerosol composition on cloud droplets size distribution: a numerical study, J. Atmos. Sci., 31, 1358&amp;ndash;1367, 1974. </reference>
		<reference numeration="14" content_type="text"> Ghan, S., Easter, R., Hudson, J., and Breon, F. M.: Evaluation of aerosol indirect radiative forcing in MIRAGE, J. Geophys. Res., 106(D6), 5317&amp;ndash;5334, 2001. </reference>
		<reference numeration="15" content_type="text"> Givati, A. and Rosenfeld, D.: Quantifying precipitation suppression due to air pollution, J. Appl. Meteor., 43, 1038&amp;ndash;1056, 2004. </reference>
		<reference numeration="16" content_type="text"> Hall, W. D.: A detailed microphysical model within a two-dimensional dynamic framework: Model description and preliminary results, J. Atmos. Sci., 37, 2486&amp;ndash;2507, 1980. </reference>
		<reference numeration="17" content_type="text"> Harshvardhan, S., Schwartz, E., Benkovitz, C. M., and Guo, G.: Aerosol influence on cloud microphysics examined by satellite measurements and chemical transport modeling, J. Atmos. Sci., 59, 714&amp;ndash;725, 2002. </reference>
		<reference numeration="18" content_type="text"> Kawamoto, K., Nakajima, T., and Nakajima, T. Y.: A global determination of cloud microphysics with AVHRR remote sensing, J. Climate, 14, 2054&amp;ndash;2068, 2001. </reference>
		<reference numeration="19" content_type="text"> Khain, A., Pokrovsky, A., and Sednev, I.: Some effects of cloud-aerosol interaction on cloud microphysics structure and precipitation formation: numerical experiments with a spectral microphysics cloud ensemble model, Atmos. Res., 52, 195&amp;ndash;220, 1999. </reference>
		<reference numeration="20" content_type="text"> Khairoutdinov, M. F. and Kogan, Y. L.: A large eddy simulation model with explicit microphysics: Validation against aircraft observations of a stratocumulus-topped boundary layer, J. Atmos. Sci., 56, 1, 2115&amp;ndash;2131, 1999. </reference>
		<reference numeration="21" content_type="text"> Kuba, N. and Takeda T.: Numerical study of the effect of CCN on the size distribution of cloud droplets. Part II. Formation of large droplets, J. Meteorol. Soc. Japan, 61, 3, 375&amp;ndash;387, 1983. </reference>
		<reference numeration="22" content_type="text"> Kuba, N. and Iwabuchi, H.: Revised parameterization to predict cloud droplet concentration and a retrieval method to predict CCN concentration, Supplement, J. Meteorol. Soc. Japan, 81, 1485&amp;ndash;1487, 2003. </reference>
		<reference numeration="23" content_type="text"> Kuba, N., Iwabuchi, H., Maruyama, K., Hayasaka, T., Takeda, T., and Fujiyoshi, Y.: Parameterization of the effect of cloud condensation nuclei on the optical properties of a non-precipitating water layer cloud, J. Meteorol. Soc. Japan, 81, 393&amp;ndash;414, 2003. </reference>
		<reference numeration="24" content_type="text"> Lohmann, U., Feichter, J., Chuang, C. C., and Penner, J. E.: Prediction of the number of cloud droplets in the ECHAM GCM, J. Goephys. Res., 104, 9169&amp;ndash;9198, 1999. </reference>
		<reference numeration="25" content_type="text"> Mordy, W.: Computation of the growth by condensation of a population of cloud droplets, Tellus, XI, 16&amp;ndash;44, 1959. </reference>
		<reference numeration="26" content_type="text"> Nakajima, T. Y. and Nakajima, T.: Wide-area determination of cloud microphysical properties from NOAA AVHRR measurements for FIRE and ASTEX regions, J. Atmos. Sci., 52, 4043&amp;ndash;4095, 1995. </reference>
		<reference numeration="27" content_type="text"> Numaguti, A.: Dynamics and energy balance of the Hadley circulation and the tropical precipitation zones: Significance of the distribution of evaporation, J. Atmos. Sci., 50, 1874&amp;ndash;1887, 1993. </reference>
		<reference numeration="28" content_type="text"> Numaguti, A., Takahashi, M., Nakajima, T., and Sumi, A.: Development of an atmospheric general circulation model, in: Reports of a New Program for Creative Basic Research Studies, Studies of Global Environment Change with Special Reference to Asia and Pacific Regions, Rep., I-3, 1&amp;ndash;27, CCSR, Tokyo, 1995. </reference>
		<reference numeration="29" content_type="text"> Reisin, T. G., Levin, Z., and Tzivion, S.: Rain production in convective clouds as simulated in an axisymmetric model with detailed microphysics. Part I: Description of model, J. Atmos. Sci., 53, 3, 497&amp;ndash;519, 1996. </reference>
		<reference numeration="30" content_type="text"> Rosenfeld, D.: TRMM observed first direct evidence of smoke from forest fires inhibiting rainfall, Geophys. Res., Lett., 26, 3105&amp;ndash;3108, 1999. </reference>
		<reference numeration="31" content_type="text"> Rosenfeld, D.: Suppression of rain and snow by urban and industrial air pollution, Science, 287, 1973&amp;ndash;1976, 2000. </reference>
		<reference numeration="32" content_type="text"> Saleeby, S. M. and Cotton, W.: A large-droplet mode and prognostic number concentration of cloud droplets in the Colorado State University Regional Atmospheric Modeling System (RAMS). Part I: Module descriptions and supercell test simulations, J. Appl. Meteor., 43, 182&amp;ndash;195, 2004. </reference>
		<reference numeration="33" content_type="text"> Smolarkiewicz, P. K.: A fully multidimensional positive definite advection transport algorithm with small implicit diffusion, J. Comput. Phys., 54, 325&amp;ndash;362, 1984. </reference>
		<reference numeration="34" content_type="text"> Szumowski, M. J., Grabowski, W. W., and Ochs III, H. T.: Simple two-dimensional kinematic framework designed to test warm rain microphysical models, Atmos. Res., 45, 299&amp;ndash;326, 1998. </reference>
		<reference numeration="35" content_type="text"> Takahashi, T.: Hail in an axisymmetric cloud model, J. Atmos. Sci., 33, 1579&amp;ndash;1601, 1976. </reference>
		<reference numeration="36" content_type="text"> Takeda, T. and Kuba, N.: Numerical study of the effect of CCN on the size distribution of cloud droplets. Part I. Cloud droplets in the stage of condensation growth, J. Meteor. Soc. Japan, 60, 4, 978&amp;ndash;993, 1982. </reference>
		<reference numeration="37" content_type="text"> Takemura, T., Okamoto, H., Maruyama, Y., Numaguti, A., Higurashi, A., and Nakajima, T.: Global three-dimensional simulation of aerosol optical thickness distribution of various origins, J. Geophys. Res., 105, 17 853&amp;ndash;17 873, 2000. </reference>
		<reference numeration="38" content_type="text"> Takemura, T., Nakajima, T., Dubovik, O., Holben, B. N., and Kinne, S.: Single-scattering albedo and radiative forcing of various aerosol species with a global three-dimensional model, J. Climate, 15, 333&amp;ndash;352, 2002. </reference>
		<reference numeration="39" content_type="text"> Takemura, T., Nozawa, T., Emori, S., Nakajima, T. Y., and Nakajima, T.: Simulation of climate response to aerosol direct and indirect effects with aerosol transport-radiation model, J. Geophys. Res., 110, D02202, doi:10.1029/2004JD005029, 2005. </reference>
		<reference numeration="40" content_type="text"> Tsuboki, K. and Sakakibara, A.: Large-scale parallel computing of Cloud Resolving Storm Simulator, High Performance Computing, Springer, edited by: Zima, H. P., Joe, K., Sato, M., Seo, Y., and Shimasaki, M., 243&amp;ndash;259, 2002. </reference>
		<reference numeration="41" content_type="text"> Twomey, S.: The nuclei of natural cloud formation, Part II: The supersaturation in natural clouds and the variation of cloud droplet concentration, Geofis. Pura. Appl., 43, 243&amp;ndash;249, 1959. </reference>
		<reference numeration="42" content_type="text"> Twomey, S.: Pollution and the planetary albedo, Atmos. Environ., 8, 1251&amp;ndash;1256, 1974. </reference>
		<reference numeration="43" content_type="text"> Twomey, S and Squires, P.: The influence of cloud nucleus population on the microstructure and stability of convective clouds, Tellus, XI, 4, 408&amp;ndash;411, 1959. </reference>
		<reference numeration="44" content_type="text"> Twomey, S. and Waner, J.: Comparison of measurements of cloud droplets and cloud nuclei, J. Atmos. Sci., 24, 702&amp;ndash;703, 1967. </reference>
		<reference numeration="45" content_type="text"> Yun, S. S. and Hudson, J.: Maritime/continental microphysical contrasts in stratus, Tellus, 54B, 61&amp;ndash;73, 2002.  </reference>
	</references>
</article>

