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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-6-2503-2006</article-id>
<title-group>
<article-title>Switching cloud cover and dynamical regimes from open to closed Benard cells in response to the suppression of precipitation by aerosols</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Rosenfeld</surname>
<given-names>D.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kaufman</surname>
<given-names>Y. J.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Koren</surname>
<given-names>I.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Institute of Earth Sciences, The Hebrew University, Jerusalem 91904, Israel</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>NASA/Goddard Space Flight Center Greenbelt, MD 20771, USA</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Department of Environmental Sciences, Weizmann Institute, Rehovot 76100, Israel</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>deceased</addr-line>
</aff>
<pub-date pub-type="epub">
<day>29</day>
<month>06</month>
<year>2006</year>
</pub-date>
<volume>6</volume>
<issue>9</issue>
<fpage>2503</fpage>
<lpage>2511</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys.net/6/2503/2006/acp-6-2503-2006.html">This article is available from http://www.atmos-chem-phys.net/6/2503/2006/acp-6-2503-2006.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys.net/6/2503/2006/acp-6-2503-2006.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/6/2503/2006/acp-6-2503-2006.pdf</self-uri>
<abstract>
<p>The dynamic structure of the weakly sheared atmospheric marine boundary
layer (MBL) supports three distinct states of cloud cover, which are
associated with the concentrations of cloud condensation nuclei (CCN)
aerosols in the MBL: (i) CCN rich MBL with closed Benard cellular convection
that forms nearly full cloud cover; (ii) CCN depleted MBL with open cellular
convection that forms &lt;40% cloud cover; and, (iii) CCN starved MBL
where clouds cannot form due to insufficient CCN, with near zero cloud
cover. Here we propose a mechanism for the transition between these three
states that involves the aerosol impacts on precipitation and the feedbacks
on the dynamics of the clouds and on the aerosols deposition. By suppressing
precipitation aerosols can reverse the direction of the airflow, converting
the cloud structure from open to closed cells and more than doubling the
cloud cover. The three states possess positive feedbacks for self
maintenance, so that small changes of the conditions can lead to bifurcation
of the MBL cloud regime. The transition between the closed and open cells
occur at near pristine background level of aerosols, creating a large
sensitivity of cloud radiative forcing to very small changes in aerosols at
the MBL. The third state of super clean air can occur as the more efficient
precipitation in cleaner air deposits the aerosols ever faster in a runaway
positive feedback process. The proposed mechanism suggests that very small
changes in the aerosols input to the MBL can have large impacts on the
oceanic cloud cover and likely in turn on the global temperature, in ways
that are not yet accounted for in the climate models.</p>
</abstract>
<counts><page-count count="9"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> Ackerman, A. S., Kirkpatrick, M. P., Stevense, D. A., and Toon, O. B.: The impact of humidity above stratiform clouds on indirect aerosol climate forcing, Nature, 432, 1014&amp;ndash;1017, 2004. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> Ackerman, A. S., Toon, O. B., and Hobbs, P. V.: Dissipation of marine stratiform clouds and collapse of the marine boundary layer due to the depletion of cloud condensation nuclei by clouds, Science, 262, 226&amp;ndash;229, 1993. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Ackerman, A. S., Toon, O. B., and Hobbs, P. V.: Reassessing the dependence of cloud condensation nucleus concentration on formation rate, Nature, 367, 445&amp;ndash;447, 1994. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> Agee, E. M., Chen, T. S., and Dowell, K. E.: A review of mesoscale cellular convection, Bull. Amer. Meteorol. Soc., 54, 1004&amp;ndash;1012, 1973. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Atkinson, B. W. and Zhang, J. W.: Mesoscale shallow convection in the atmosphere. Rev. Geophys., 34, 403&amp;ndash;431, 1996. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> Baker, M. B. and Charlson, R. J.: Bistability of CCN concentrations and thermodynamics in the cloud-topped boundary layer, Nature, 345, 142&amp;ndash;145, 1990. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> Battan, L. J. and Braham Jr., R. R.: A study of convective precipitation based on cloud and radar observations, J. Meteor., 13, 587&amp;ndash;591, 1956. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> Carlslaw, K. S., Harrison, R. G., and Kirkby, J.: Cosmic rays, clouds, and climate, Science, 298, 1732&amp;ndash;1737, 2002. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Coakley, J. A., Bernstein, R. L., and Durkee, P. A.: Effect of ship-stack effluents on cloud reflectivity, Science, 237, 1020&amp;ndash;1022, 1987. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Coakley Jr., J. A. and Walsh, C. D.: Limits to the aerosol indirect radiative effect derived from observations of ship tracks, J. Atmos. Sci., 59, 668&amp;ndash;680, 2002. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Feingold, G. F., Stevens, B., Cotton, W. R., and Frish, A. S.: The relationship between drop in-cloud residence time and drizzle production in numerically simulated stratocumulus clouds, J. Atmos. Sci., 53, 1108&amp;ndash;1122, 1996. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Gerber H.: Microphysics of marine stratocumulus clouds with two drizzle modes, J. Atmos. Sci., 53, 1649&amp;ndash;1662, 1996. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Gunn, R. and Phillips, B. B.: An experimental investigation of the effect of air pollution on the initiation of rain, J. Meteorol., 14, 272&amp;ndash;280, 1957. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> Hegg, D. A.: Dependence of marine stratocumulus formation on aerosols, Geophys. Res. Let., 26(10), 1429&amp;ndash;1432, 1999. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Jiang, H., Feingold, G., and Cotton, W. R.: A modeling study of entrainment of cloud condensation nuclei into the marine boundary layer during ASTEX, J. Geophys. Res., 107(D24), 4813, doi:10.1029/2001JD001502, 2002. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Johnson, R. H., Rickenbach, T. M., Rutledge, S. A., Ciesielski, P. E., Schubert, W. H.: Trimodal characteristics of tropical convection, J. Clim., 12, 2397&amp;ndash;2418, 1999. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Kaufman, Y. J., Koren, I., Remer, L. A., Rosenfeld, D., and Rudich, Y.: Smoke, Dust and Pollution Aerosol Clouding the Atlantic Atmosphere, Proceedings of the National Academy of Sciences, 102, 11 207&amp;ndash;11 212, 2005. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Mechem, D. B. and Kogan, Y. L.: Simulating the transition from drizzling marine stratocumulus to boundary layer cumulus with a mesoscale model, Mon. Wea. Rev., 131, 2342&amp;ndash;2360, 2003. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Paluch, I. R. and Lenschow, D. H.: Stratiform cloud fraction in the marine boundary layer, J. Atmos. Sci., 48, 2141&amp;ndash;2158, 1991. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> Petters, M. D., Snider J. R., Stevens, B., Vali, G., Faloona, I., and Russell, L.: Accumulation mode aerosol, pockets of open cells, and particle nucleation in the remote subtropical Pacific marine boundary layer, J. Geophys. Res., 111, D02206, doi:10.1029/2004JD005694, 2006. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Pincus, R. and Baker, M. B.: Effect of precipitation on the albedo susceptibility of clouds in the marine boundary-layer, Nature, 372, 250&amp;ndash;252, 1994. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Platnick, S. P., Durkee, A., Nielsen, K., Taylor, J. P., Tsay, S.-C., King, M. D., Ferek, R. J., Hobbs, P. V., and Rottman, J. W.: The role of background cloud microphysics in the radiative formation of ship tracks, J. Atmos. Sci., 57, 2607&amp;ndash;2624, 2000. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Randall, D. A.: Conditional instability of the first kind upside-down, J. Atmos. Sci., 37, 125&amp;ndash;130, 1980a. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> Randall, D. A.: Conditional Entrainment into a stratocumulus layer with distributed radiative cooling, J. Atmos. Sci., 37, 148&amp;ndash;159, 1980b. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Rosenfeld, D., Cattani, E., Melani, S., and Levizzani, V.: Considerations on daylight operation of 1.6 $\mu $m vs. 3.7 $\mu $m channel on NOAA and METOP Satellites, Bull. Amer. Meteorol. Soc., 85, 873&amp;ndash;881, 2004. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> Rosenfeld, D., Lahav, R., Khain, A. P., and Pinsky, M.: The role of sea-spray in cleansing air pollution over ocean via cloud processes, Science, 297, 1667&amp;ndash;1670, 2002. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> Rosenfeld, D. and Lensky, I. M.: Satellite-based insights into precipitation formation processes in continental and maritime convective clouds, Bull. Amer. Meteorol. Soc., 79, 2457&amp;ndash;2476, 1998. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> Sekiguchi, M., Nakajima, T., Suzuki, K., Kawamoto, K., Higurashi, A., Rosenfeld, D., Sano, I., and Mukai, S.: A study of the direct and indirect effects of aerosols using global satellite datasets of aerosol and cloud parameters, J. Geophys. Res., 108(D22), 4699, doi:10.1029/2002JD003359, 2003. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> Smirnov, A., Holben, B. N., Kaufman, Y. J., Dubovik, O., Eck, T. F., Slutsker, I., Pietras, C., and Halthore, R. N.: Optical Properties of Atmospheric Aerosol in Maritime Environments, J. Atmos. Sci., 59, 501&amp;ndash;523, 2002. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> Stevens, B., Vali, G., Comstock, K., van Zanten, M. C., Austin, P. H., Bretherton C. S., and Lenschow, D. H.: Pockets of Open Cells (POCs) and Drizzle in Marine Stratocumulus, Bull. Amer. Meteorol. Soc., 86, 51&amp;ndash;57, 2005. </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> Twomey, S.: The influence of pollution on the shortwave albedo of clouds, J. Atmos. Sci., 34, 1149&amp;ndash;1154, 1977. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> Wingenter, O. W., Haase, K. B., Strutton, P., Friederich, G., Meinardi, S., Blake, D. R., and Rowland, F. S.: Changing concentrations of CO, CH$_4$, C$_5$H$_8$, CH$_3$Br, CH$_3$I,and dimethyl sulfide during the Southern Ocean Iron Enrichment Experiments, Proc. Nat. Acad. Sci., 101(23), 8537&amp;ndash;8541, 2004. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> Wood, R. and Hartmann, D. L.: Spatial variability of liquid water path in marine low cloud: The importance of mesoscale cellular convection, J. Clim., 19, 1748&amp;ndash;1764, 2006. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> VanZanten, M. C., Stevens, B., Vali, G., and Lenschow, D. H.: Observations in nocturnal marine stratocumulus, J. Atmos. Sci., 62, 88&amp;ndash;106, 2005.  </mixed-citation>
</ref>
</ref-list>
</back>
</article>