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<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-6-2411-2006</article-id>
<title-group>
<article-title>Winter and summer time size distributions and densities of  traffic-related aerosol particles at a busy highway in Helsinki</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Virtanen</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Rönkkö</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kannosto</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Ristimäki</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Mäkelä</surname>
<given-names>J. M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Keskinen</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Pakkanen</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Hillamo</surname>
<given-names>R.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Pirjola</surname>
<given-names>L.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Hämeri</surname>
<given-names>K.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Tampere University of Technology, Institute of Physics, Aerosol  Physics, P.O. Box 692, 33101 Tampere, Finland</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Finnish Meteorological Institute, Air Quality Research, Sahaajankatu  20 E, 00810 Helsinki, Finland</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Helsinki Polytechnics, Department of Technology, P.O. Box 4020,  00099 Helsinki, Finland</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>Finnish Institute of Occupational Health, Department of Physics,  Topeliuksenkatu 41, 00250 Helsinki, Finland</addr-line>
</aff>
<aff id="aff5">
<label>5</label>
<addr-line>University of Helsinki, Department of Physical Sciences, P.O. Box 64,  00014 University of Helsinki, Finland</addr-line>
</aff>
<pub-date pub-type="epub">
<day>29</day>
<month>06</month>
<year>2006</year>
</pub-date>
<volume>6</volume>
<issue>9</issue>
<fpage>2411</fpage>
<lpage>2421</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
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<self-uri xlink:href="http://www.atmos-chem-phys.net/6/2411/2006/acp-6-2411-2006.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/6/2411/2006/acp-6-2411-2006.pdf</self-uri>
<abstract>
<p>Number concentrations and size distributions of traffic related aerosol
particles were measured at a roadside in Helsinki during two winter
campaigns (10&amp;ndash;26 February 2003, 28 January&amp;ndash;12 February 2004) and two summer
campaigns (12&amp;ndash;27 August 2003, 6&amp;ndash;20 August 2004). The measurements were
performed simultaneously at distances of 9 m and 65 m from the highway.
Total number concentrations were measured by a condensation particle counter
(CPC) and particle size distributions by a scanning mobility particle sizer
(SMPS) and an electrical low pressure impactor (ELPI). This study
concentrates on data that were measured when the wind direction was from the
road to the measurement site. The total concentrations in the wintertime
were 2&amp;ndash;3 times higher than in the summertime and the concentrations were
dominated by nucleation mode particles. The particles smaller than 63 nm
(aerodynamic diameter) constituted ~90% of all particles in the
wintertime and ~80% of particles in the summer time. The particle
total concentration increased with increasing traffic rate. The effect of
traffic rate on particles smaller than 63 nm was stronger than on the larger
particles. The particle distributions at the roadside consisted of two
distinguishable modes. The geometric mean diameter (GMD) of nucleation mode
(Mode 1) was 20.3 nm in summer and 18.9 nm in winter. The GMD of the larger
mode consisting mostly of traffic related soot particles (Mode 2) was 72.0 nm
in summer and 75.1 nm in winter. The GMD values of the modes did not
depend on the traffic rate. The average particle density for each mode was
determined by a parallel density fitting method based on the size
distribution measurement made by ELPI and SMPS. The average density value
for Mode 1 particles was 1.0&amp;plusmn;0.13 g/cm&lt;sup&gt;3&lt;/sup&gt; and 1.0&amp;plusmn;0.07 g/cm&lt;sup&gt;3&lt;/sup&gt;
both in summer and winter respectively, while the average density
value for Mode 2 was 1.5&amp;plusmn;0.1 g/cm&lt;sup&gt;3&lt;/sup&gt; and 1.8&amp;plusmn;0.3 g/cm&lt;sup&gt;3&lt;/sup&gt;
for summer and winter, respectively.</p>
</abstract>
<counts><page-count count="11"/></counts>
</article-meta>
</front>
<body/>
<back>
<ref-list>
<title>References</title>
<ref id="ref1">
<label>1</label><mixed-citation publication-type="other" xlink:type="simple"> Abdul-Khalek, I. S., Kittelson, D. B., and Brear, F.: The influence of dilution conditions on diesel exhaust particle size distribution measurements, SAE technical paper series, no. 1999-01-1142, 1999. </mixed-citation>
</ref>
<ref id="ref2">
<label>2</label><mixed-citation publication-type="other" xlink:type="simple"> Charron, A. and Harrison, R. M.: Primary particle formation from vehicle emissions during exhaust dilution in the roadside atmosphere, Atmos. Environ., 37, 4109&amp;ndash;4119, 2003. </mixed-citation>
</ref>
<ref id="ref3">
<label>3</label><mixed-citation publication-type="other" xlink:type="simple"> Gieshaskiel, B., Ntziachristos, L., Samaras, Z., Scheer, V., Casati, R., and Vogt, R.: Formation potential of vehicle exhaust nucleation mode particles on-road and in the laboratory, Atmos. Environ., 39, 3191&amp;ndash;3198, 2005. </mixed-citation>
</ref>
<ref id="ref4">
<label>4</label><mixed-citation publication-type="other" xlink:type="simple"> Harris, S. J. and Maricq, M. M.: Signature size distribution for diesel and gasoline engine exhaust particulate matter, J. Aerosol Sci., 32, 749&amp;ndash;764, 2001. </mixed-citation>
</ref>
<ref id="ref5">
<label>5</label><mixed-citation publication-type="other" xlink:type="simple"> Hussein, T., Puustinen, A., Aalto, P. P., Mäkelä, J. M., Hämeri, K., and Kulmala, M.: Urban aerosol number size distributions, Atmos. Chem. Phys., 4, 391&amp;ndash;411, 2004. </mixed-citation>
</ref>
<ref id="ref6">
<label>6</label><mixed-citation publication-type="other" xlink:type="simple"> Imhof, D., Weingartner, E., Ordó\~nez, C.,Gehrig, R., Hill, M., Buchmann, B., and Baltensberger, U.: Real-world emission factors of fine and ultra fine aerosol particles for different traffic situations in Switzerland, Environ. Sci. Technol., 39, 8341&amp;ndash;8350, 2005a. </mixed-citation>
</ref>
<ref id="ref7">
<label>7</label><mixed-citation publication-type="other" xlink:type="simple"> Imhof, D., Weingartner, E., Prévöt, A. S. H., Ordó\~nez, C., Kurtenbach, R., Wiesen, P., Rodler, J., Sturm, P., McCrae, I., Sjödin, \AA., and Baltensberger, U.: Aerosol and NOx emission factors and submicron particle number size distributions in two road tunnels with different traffic regimes, Atmos. Chem. Phys. Discuss., 5, 5127&amp;ndash;5166, 2005b. </mixed-citation>
</ref>
<ref id="ref8">
<label>8</label><mixed-citation publication-type="other" xlink:type="simple"> Janhäll. S., Jonsson, \AA. M., Molnár, P., Svensson, E., and Hallquist, M.: Size resolved traffic emission factors of submicrometer particles, Atmos. Environ., 38, 4331&amp;ndash;4340, 2004. </mixed-citation>
</ref>
<ref id="ref9">
<label>9</label><mixed-citation publication-type="other" xlink:type="simple"> Ketzel, M., W\aahlin, P., Kristensson, A., Swietlicki, E., Berkowicz, R., Nielsen, O. J., and Palmgren, F.: Particle size distribution and particle mass measurements at urban, near-city and rural level in the Copenhagen area and Southern Sweden, Atmos. Chem. Phys., 4, 281&amp;ndash;292, 2004. </mixed-citation>
</ref>
<ref id="ref10">
<label>10</label><mixed-citation publication-type="other" xlink:type="simple"> Khalek, I. A., Kittelson, D. B., and Brear, F.: Nanoparticle growth during dilution and cooling of diesel exhaust: experimental investigation and theoretical assessment, SAE technical paper series, No. 2000-01-0515, 2000. </mixed-citation>
</ref>
<ref id="ref11">
<label>11</label><mixed-citation publication-type="other" xlink:type="simple"> Kittelson, D. B.: Engines and nanoparticles: a review, J. Aerosol Sci., 29, 575&amp;ndash;588, 1998. </mixed-citation>
</ref>
<ref id="ref12">
<label>12</label><mixed-citation publication-type="other" xlink:type="simple"> Kittelson, D., Johnson, J., Watts, W., Wei, Q., Drayton, M., Paulsen, D., and Bukowiecki, N.: Diesel aerosol sampling in the atmosphere, SAE technical paper series, No. 2000-01-22212, 2000. </mixed-citation>
</ref>
<ref id="ref13">
<label>13</label><mixed-citation publication-type="other" xlink:type="simple"> Kittelson, D. B., Watts, W. F., and Johnson, J. P.: Nanoparticle emissions on Minnesota highways, Atmos. Environ., 38, 9&amp;ndash;19, 2004. </mixed-citation>
</ref>
<ref id="ref14">
<label>14</label><mixed-citation publication-type="other" xlink:type="simple"> Lepperhof, G.: Influences on the particle size distribution of diesel particulate emissions, Topics in Catalysis, 16/17(1&amp;ndash;4), 2001. </mixed-citation>
</ref>
<ref id="ref15">
<label>15</label><mixed-citation publication-type="other" xlink:type="simple"> Longley, I. D., Gallagher, M. W., Dorsey, J. R., and Flynn, M.: A case study of fine particle concentrations and fluxes measured in a busy street canyon in Manchester, UK, Atmos. Environ., 38, 3595&amp;ndash;3603, 2004. </mixed-citation>
</ref>
<ref id="ref16">
<label>16</label><mixed-citation publication-type="other" xlink:type="simple"> Maricq, M., Chase, R., Xu, N., and Laing, P.: The effects of catalytic converter and fuel sulfur level on motor vehicle particle emissions: Light duty vehicle emissions, Environ. Sci. Technol., 36, 283&amp;ndash;289, 2002. </mixed-citation>
</ref>
<ref id="ref17">
<label>17</label><mixed-citation publication-type="other" xlink:type="simple"> Maricq, M. and Xu, N.: The effective density and fractal dimension of soot particles from premixed flames and motor vehicle exhaust, J. Aerosol Sci., 35, 1251&amp;ndash;1274, 2004. </mixed-citation>
</ref>
<ref id="ref18">
<label>18</label><mixed-citation publication-type="other" xlink:type="simple"> Marjamäki, M., Keskinen, J., Chen, D.-R., and Pui, D. Y. H.: Performance evaluation of the electrical low pressure impactor (ELPI), J. Aerosol Sci., 31(2), 249&amp;ndash;261, 2000. </mixed-citation>
</ref>
<ref id="ref19">
<label>19</label><mixed-citation publication-type="other" xlink:type="simple"> Marjamäki, M., Lemmetty, M., and Keskinen, J.: ELPI response and data reduction I: Response functions, Aerosol Sci. Technol., 39, 575&amp;ndash;582, 2005. </mixed-citation>
</ref>
<ref id="ref20">
<label>20</label><mixed-citation publication-type="other" xlink:type="simple"> McMurry, P., Wang, X., Park, K., and Ehara, K.: The relationship between mass and mobility for atmospheric particles: A new technique for measuring particle density, Aerosol Sci. Technol., 36, 227&amp;ndash;238, 2002. </mixed-citation>
</ref>
<ref id="ref21">
<label>21</label><mixed-citation publication-type="other" xlink:type="simple"> Molnár, P., Janhäll, S., and Hallquist, M.: Roadside measurements of fine and ultrafine particles at a major road north of Gothenburg, Atmos. Environ., 36, 4115&amp;ndash;4123, 2002. </mixed-citation>
</ref>
<ref id="ref22">
<label>22</label><mixed-citation publication-type="other" xlink:type="simple"> Mönkkönen, P., Koponen, I., Lehtinen, K. E. J., Hämeri, K., Uma, R., and Kulmala, M.: Measurements in a highly polluted Asian mega city: observations of aerosol number size distribution, modal parameters and nucleation events, Atmos. Chem. Phys., 5, 57&amp;ndash;66, 2005. </mixed-citation>
</ref>
<ref id="ref23">
<label>23</label><mixed-citation publication-type="other" xlink:type="simple"> Park, K., Cao, F., Kittelson, D., and McMurry, P.: Relationship between particle mass and mobility for diesel exhaust particles, Environ. Sci. Technol., 37, 577&amp;ndash;583, 2003. </mixed-citation>
</ref>
<ref id="ref24">
<label>24</label><mixed-citation publication-type="other" xlink:type="simple"> Pirjola, L., Paasonen, P., Pfeiffer, D., Hussein, T., Hämeri, K., Koskentalo, T., Virtanen, A., Rönkkö, T., Keskinen, J., and Pakkanen, T.: Dispersion of particles and trace gases nearby a city highway: mobile laboratory measurements in Finland, Atmos. Environ., 40, 867&amp;ndash;879, 2006. </mixed-citation>
</ref>
<ref id="ref25">
<label>25</label><mixed-citation publication-type="other" xlink:type="simple"> Pirjola, L., Parviainen, H., Hussein, T., Valli, A., Hämeri, K., Aalto, P., Virtanen, A., Keskinen, J., Pakkanen, T. A., Mäkelä, T., and Hillamo, R. E.: &quot;Sniffer&quot; &amp;ndash; a novel tool for chasing vehicles and measuring traffic pollutants, Atmos. Environ., 38, 3625&amp;ndash;3635, 2004. </mixed-citation>
</ref>
<ref id="ref26">
<label>26</label><mixed-citation publication-type="other" xlink:type="simple"> Ristimäki, J., Virtanen, A, Marjamäki, M., Rostedt, A., and Keskinen, J.: On-line measurement of size distribution and effective density of submicron aerosol particles, J. Aerosol Sci., 33, 1541&amp;ndash;1557, 2002. </mixed-citation>
</ref>
<ref id="ref27">
<label>27</label><mixed-citation publication-type="other" xlink:type="simple"> Ristimäki, J., Keskinen, J., Virtanen A., Maricq, M., and Aakko, P.: Cold temperature PM emissions measurement: Method evaluation and application to light duty vehicles, Environ. Sci. Technol., 39, 9424&amp;ndash;9430, 2005. </mixed-citation>
</ref>
<ref id="ref28">
<label>28</label><mixed-citation publication-type="other" xlink:type="simple"> Rose, D., Wehner, B., Ketzel, M., Engler, C., Voigtländer, J., Tuch, T., and Wiedensohler, A.: Atmospheric number size distributions of soot particles and estimation of emission factors, Atmos. Chem. Phys., 6, 1021&amp;ndash;1031, 2006. </mixed-citation>
</ref>
<ref id="ref29">
<label>29</label><mixed-citation publication-type="other" xlink:type="simple"> Rönkkö, T., Virtanen , A., Vaaraslahti, K., Keskinen, J., Pirjola, L., and Lappi, M.: Effect of dilution conditions and driving parameters on nucleation mode particles in diesel exhaust: Laboratory and on-road study, Atmos. Environ., 40, 2893&amp;ndash;2901, 2006. </mixed-citation>
</ref>
<ref id="ref30">
<label>30</label><mixed-citation publication-type="other" xlink:type="simple"> Sakurai, H., Tobias, H., Park, K., Zarling, D., Doherty, K. S., Kittelson, D. B., McMurry, P. H., and Ziemann, P.: On-line determination of diesel nanoparticle composition and volatility, Atmos. Environ., 37, 1199&amp;ndash;1210, 2003a. </mixed-citation>
</ref>
<ref id="ref31">
<label>31</label><mixed-citation publication-type="other" xlink:type="simple"> Sakurai, H., Park, K., McMurry, P., Zarling, D. D., Kittelson, D. B., and Ziemann, P.: Size-Dependent mixing characteristics of volatile and nonvolatile components in diesel exhaust aerosols, Environ. Sci. Technol., 37, 5487&amp;ndash;5495, 2003b. </mixed-citation>
</ref>
<ref id="ref32">
<label>32</label><mixed-citation publication-type="other" xlink:type="simple"> Stein, S. W., Turpin, B. J., Cai, X. P., Huang, P. F., and McMurry, P. H.: Measurements of relative humidity-dependent bounce and density for atmospheric particles using tandem-DMA-impactor technique, Atmos. Environ., 28, 1739&amp;ndash;1746, 1994. </mixed-citation>
</ref>
<ref id="ref33">
<label>33</label><mixed-citation publication-type="other" xlink:type="simple"> Tunved, P., Hansson, H.-C., Kulmala, M., Aalto, P., Viisanen, Y., Karlsson, H., Kristensson, A., Swietlicki, E., Dal Maso, M., and Komppula, M.: One year boundary layer aerosol size distribution data from five Nordic background stations, Atmos. Chem. Phys., 3, 2183&amp;ndash;2205, 2003. </mixed-citation>
</ref>
<ref id="ref34">
<label>34</label><mixed-citation publication-type="other" xlink:type="simple"> Vaaraslahti, K., Virtanen, A., Ristimäki, J., and Keskinen, J.: Nucleation mode formation in heavy-duty diesel exhaust with and without particulate filter, Environ. Sci. Technol., 38, 4884&amp;ndash;4890, 2004. </mixed-citation>
</ref>
<ref id="ref35">
<label>35</label><mixed-citation publication-type="other" xlink:type="simple"> Van Dingenen, R., Raes, F., Putaud, J.-P., Baltensberger, U., Charron, A., Facchini, M.-C., Decesari, S., Fuzzi, S., Gehrig, R., Hansson, H.-C., Harrison, R. M., Hüglin, R., Jones, A. M., Laj, P., Lorbeer, G., Maenhaut, W., Palmgren, F., Querol, X., Rodriquez, S., Schneider, J., ten Brink, H., Tunved, P., Torseth, K., Wehner, B., Weingartner, E., Wiedensohler, A., and W\aahlin, P.: A European aerosol phenomenology &amp;ndash; 1: physical characteristics of particulate matter at kerbside, urban, rural and background areas in Europe, Atmos. Environ., 38, 2561&amp;ndash;2577, 2004. </mixed-citation>
</ref>
<ref id="ref36">
<label>36</label><mixed-citation publication-type="other" xlink:type="simple"> Virtanen, A., Marjamäki, M., Ristimäki, J., and Keskinen, J.: Fine particle losses in electrical low-pressure impactor, J. Aerosol Sci., 32, 389&amp;ndash;401, 2001.  </mixed-citation>
</ref>
<ref id="ref37">
<label>37</label><mixed-citation publication-type="other" xlink:type="simple"> Virtanen, A., Ristimäki, J., and Keskinen, J.: Method for measuring effective density and fractal dimension of aerosol agglomerates, Aerosol Sci. Technol., 38, 437&amp;ndash;446, 2004a. </mixed-citation>
</ref>
<ref id="ref38">
<label>38</label><mixed-citation publication-type="other" xlink:type="simple"> Virtanen, A., Ristimäki, J., Vaaraslahti, K., and Keskinen J.: Effect of engine load on diesel soot particles, Environ. Sci. Technol., 38, 2551&amp;ndash;2556, 2004b. </mixed-citation>
</ref>
<ref id="ref39">
<label>39</label><mixed-citation publication-type="other" xlink:type="simple"> Vogt, R., Sheer, V., Casati, R., and Benter, T.: On-road measurement of particle emission in the exhaust plume of a diesel passenger car, Environ. Sci. Technol., 37, 4070&amp;ndash;4076, 2003. </mixed-citation>
</ref>
<ref id="ref40">
<label>40</label><mixed-citation publication-type="other" xlink:type="simple"> Wehner, B., Birmili, W., Gnauk, T., and Wiedensohler, A.: Particle number size distribution in a street canyon and their transformation into the urban air background: measurements and a simple model study, Atmos. Environ., 36, 2215&amp;ndash;2223, 2002. </mixed-citation>
</ref>
<ref id="ref41">
<label>41</label><mixed-citation publication-type="other" xlink:type="simple"> Wehner, B. and Wiedensohler, A.: Long term measurements of submicron urban aerosols: statistical analysis for correlations with meteorological conditions and trace gases, Atmos. Chem. Phys., 3, 867&amp;ndash;879, 2003. </mixed-citation>
</ref>
<ref id="ref42">
<label>42</label><mixed-citation publication-type="other" xlink:type="simple"> Williams, P. I., Gallagher, M. W., Choularton, T. W., Coe, H., Bower, K. N., and McFiggans, G.: Aerosol development and interaction in an urban plume, Aerosol Sci. Technol., 32, 120&amp;ndash;126, 2000. </mixed-citation>
</ref>
<ref id="ref43">
<label>43</label><mixed-citation publication-type="other" xlink:type="simple"> W\aahlin, P., Palmgren, F., and Van Dingenen, R.: Experimental studies of ultra fine particles in streets and the relationship to traffic, Atmos. Environ., Suppl. 1, 35, 63&amp;ndash;69, 2001. </mixed-citation>
</ref>
</ref-list>
</back>
</article>