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<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-6-1777-2006</article-id>
<title-group>
<article-title>Analysis and quantification of the diversities of aerosol life cycles within AeroCom</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Textor</surname>
<given-names>C.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Schulz</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Guibert</surname>
<given-names>S.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kinne</surname>
<given-names>S.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Balkanski</surname>
<given-names>Y.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Bauer</surname>
<given-names>S.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Berntsen</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Berglen</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Boucher</surname>
<given-names>O.</given-names>
</name>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
<xref ref-type="aff" rid="aff18">
<sup>18</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Chin</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff16">
<sup>16</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dentener</surname>
<given-names>F.</given-names>
</name>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Diehl</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff17">
<sup>17</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Easter</surname>
<given-names>R.</given-names>
</name>
<xref ref-type="aff" rid="aff8">
<sup>8</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Feichter</surname>
<given-names>H.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Fillmore</surname>
<given-names>D.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff7">
<sup>7</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Ghan</surname>
<given-names>S.</given-names>
</name>
<xref ref-type="aff" rid="aff8">
<sup>8</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Ginoux</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff9">
<sup>9</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Gong</surname>
<given-names>S.</given-names>
</name>
<xref ref-type="aff" rid="aff10">
<sup>10</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Grini</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Hendricks</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff11">
<sup>11</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Horowitz</surname>
<given-names>L.</given-names>
</name>
<xref ref-type="aff" rid="aff9">
<sup>9</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Huang</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff10">
<sup>10</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Isaksen</surname>
<given-names>I.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Iversen</surname>
<given-names>I.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kloster</surname>
<given-names>S.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Koch</surname>
<given-names>D.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kirkevåg</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kristjansson</surname>
<given-names>J. E.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Krol</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff12">
<sup>12</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Lauer</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff11">
<sup>11</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Lamarque</surname>
<given-names>J. F.</given-names>
</name>
<xref ref-type="aff" rid="aff7">
<sup>7</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Liu</surname>
<given-names>X.</given-names>
</name>
<xref ref-type="aff" rid="aff13">
<sup>13</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Montanaro</surname>
<given-names>V.</given-names>
</name>
<xref ref-type="aff" rid="aff14">
<sup>14</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Myhre</surname>
<given-names>G.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Penner</surname>
<given-names>J.</given-names>
</name>
<xref ref-type="aff" rid="aff13">
<sup>13</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Pitari</surname>
<given-names>G.</given-names>
</name>
<xref ref-type="aff" rid="aff14">
<sup>14</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Reddy</surname>
<given-names>S.</given-names>
</name>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
<xref ref-type="aff" rid="aff9">
<sup>9</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Seland</surname>
<given-names>Ø.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Stier</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Takemura</surname>
<given-names>T.</given-names>
</name>
<xref ref-type="aff" rid="aff15">
<sup>15</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Tie</surname>
<given-names>X.</given-names>
</name>
<xref ref-type="aff" rid="aff7">
<sup>7</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Laboratoire des Sciences du Climat et de l’Environnement, Gif-sur-Yvette, France</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Max-Planck-Institut für Meteorologie, Hamburg, Germany</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Columbia University, GISS, New York, USA</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>University of Oslo, Department of Geophysics, Oslo, Norway</addr-line>
</aff>
<aff id="aff5">
<label>5</label>
<addr-line>Laboratoire d’Optique Atmosphérique, Université des Sciences et Technologies de Lille, CNRS, Villeneuve d’Ascq, France</addr-line>
</aff>
<aff id="aff6">
<label>6</label>
<addr-line>EC, Joint Research Centre, Institute for Environment and Sustainability, Climate Change Unit, Italy</addr-line>
</aff>
<aff id="aff7">
<label>7</label>
<addr-line>NCAR, Boulder, Colorado, USA</addr-line>
</aff>
<aff id="aff8">
<label>8</label>
<addr-line>Battelle, Pacific Northwest National Laboratory, Richland, USA</addr-line>
</aff>
<aff id="aff9">
<label>9</label>
<addr-line>NOAA, Geophysical Fluid Dynamics Laboratory, Princeton, New Jersey, USA</addr-line>
</aff>
<aff id="aff10">
<label>10</label>
<addr-line>ARQM Meteorological Service Canda, Toronto, Canada</addr-line>
</aff>
<aff id="aff11">
<label>11</label>
<addr-line>Institut für Physik der Atmosphäre, DLR Oberpfaffenhofen, Germany</addr-line>
</aff>
<aff id="aff12">
<label>12</label>
<addr-line>Institute for Marine and Atmospheric Research Utrecht (IMAU) Utrecht University, Utrecht, Netherlands</addr-line>
</aff>
<aff id="aff13">
<label>13</label>
<addr-line>University of Michigan, Ann Arbor, MI, USA</addr-line>
</aff>
<aff id="aff14">
<label>14</label>
<addr-line>Universita degli Studi L’Aquila, Italy</addr-line>
</aff>
<aff id="aff15">
<label>15</label>
<addr-line>Kyushu University, Fukuoka, Japan</addr-line>
</aff>
<aff id="aff16">
<label>16</label>
<addr-line>NASA Goddard Space Flight Center, Greenbelt, MD, USA</addr-line>
</aff>
<aff id="aff17">
<label>17</label>
<addr-line>Goddard Earth Sciences and Technology Center, University of Maryland Baltimore County, Baltimore, Maryland, USA</addr-line>
</aff>
<aff id="aff18">
<label>18</label>
<addr-line>Hadley Centre, Met Office, Exeter, UK</addr-line>
</aff>
<pub-date pub-type="epub">
<day>29</day>
<month>05</month>
<year>2006</year>
</pub-date>
<volume>6</volume>
<issue>7</issue>
<fpage>1777</fpage>
<lpage>1813</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys.net/6/1777/2006/acp-6-1777-2006.html">This article is available from http://www.atmos-chem-phys.net/6/1777/2006/acp-6-1777-2006.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys.net/6/1777/2006/acp-6-1777-2006.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/6/1777/2006/acp-6-1777-2006.pdf</self-uri>
<abstract>
<p>Simulation results of global aerosol models have been
assembled in the framework of the AeroCom intercomparison exercise. In
this paper, we analyze the life cycles of dust, sea salt, sulfate,
black carbon and particulate organic matter as simulated by sixteen
global aerosol models. The differences among the results (model
diversities) for sources and sinks, burdens, particle sizes, water
uptakes, and spatial dispersals have been established. These
diversities have large consequences for the calculated radiative
forcing and the aerosol concentrations at the surface. Processes and
parameters are identified which deserve further research.

&lt;P  style=&quot;line-height: 20px;&quot;&gt;
The AeroCom all-models-average emissions are dominated by the mass of
sea salt (SS), followed by dust (DU), sulfate (SO&lt;sub&gt;4&lt;/sub&gt;), particulate
organic matter (POM), and finally black carbon (BC). Interactive
parameterizations of the emissions and contrasting particles sizes of
SS and DU lead generally to higher diversities of these species, and
for total aerosol. The lower diversity of the emissions of the fine
aerosols, BC, POM, and SO&lt;sub&gt;4&lt;/sub&gt;, is due to the use of similar emission
inventories, and does therefore not necessarily indicate a better
understanding of their sources. The diversity of SO&lt;sub&gt;4&lt;/sub&gt;-sources is
mainly caused by the disagreement on depositional loss of precursor
gases and on chemical production. The diversities of the emissions are
passed on to the burdens, but the latter are also strongly affected by
the model-specific treatments of transport and aerosol processes. The
burdens of dry masses decrease from largest to smallest: DU, SS,
SO&lt;sub&gt;4&lt;/sub&gt;, POM, and BC.

&lt;P  style=&quot;line-height: 20px;&quot;&gt;
The all-models-average residence time is shortest for SS with about
half a day, followed by SO&lt;sub&gt;4&lt;/sub&gt; and DU with four days, and POM and BC
with six and seven days, respectively. The wet deposition rate is
controlled by the solubility and increases from DU, BC, POM to SO&lt;sub&gt;4&lt;/sub&gt;
and SS. It is the dominant sink for SO&lt;sub&gt;4&lt;/sub&gt;, BC, and POM, and
contributes about one third to the total removal of
SS and DU species. For SS and DU we find high diversities for the
removal rate coefficients and deposition pathways. Models do neither
agree on the split between wet and dry deposition, nor on that between
sedimentation and other dry deposition processes. We diagnose an
extremely high diversity for the uptake of ambient water vapor that
influences the particle size and thus the sink rate
coefficients. Furthermore, we find little agreement among the model
results for the partitioning of wet removal into scavenging by
convective and stratiform rain.

&lt;P  style=&quot;line-height: 20px;&quot;&gt;
Large differences exist for aerosol dispersal both in the vertical and
in the horizontal direction. In some models, a minimum of total
aerosol concentration is simulated at the surface. Aerosol dispersal
is most pronounced for SO&lt;sub&gt;4&lt;/sub&gt; and BC and lowest for SS. Diversities are
higher for meridional than for vertical dispersal, they are similar
for the individual species and highest for SS and DU. For these two
components we do not find a correlation between vertical and
meridional aerosol dispersal. In addition the degree of dispersals of
SS and DU is not related to their residence times. SO&lt;sub&gt;4&lt;/sub&gt;, BC, and
POM, however, show increased meridional dispersal in models with
larger vertical dispersal, and dispersal is larger for longer
simulated residence times.</p>
</abstract>
<counts><page-count count="37"/></counts>
</article-meta>
</front>
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<back>
</back>
</article>