<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "http://dtd.nlm.nih.gov/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-5-2431-2005</article-id>
<title-group>
<article-title>Inverse modelling of national and European CH&lt;sub&gt;4&lt;/sub&gt; emissions using the atmospheric zoom model TM5</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Bergamaschi</surname>
<given-names>P.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Krol</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
<xref ref-type="aff" rid="aff2">
<sup>2</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dentener</surname>
<given-names>F.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Vermeulen</surname>
<given-names>A.</given-names>
</name>
<xref ref-type="aff" rid="aff3">
<sup>3</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Meinhardt</surname>
<given-names>F.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Graul</surname>
<given-names>R.</given-names>
</name>
<xref ref-type="aff" rid="aff4">
<sup>4</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Ramonet</surname>
<given-names>M.</given-names>
</name>
<xref ref-type="aff" rid="aff5">
<sup>5</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Peters</surname>
<given-names>W.</given-names>
</name>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
<contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Dlugokencky</surname>
<given-names>E. J.</given-names>
</name>
<xref ref-type="aff" rid="aff6">
<sup>6</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>European Commission Joint Research Centre, Ispra, Italy</addr-line>
</aff>
<aff id="aff2">
<label>2</label>
<addr-line>Institute for Marine and Atmospheric Research, Utrecht, Netherlands</addr-line>
</aff>
<aff id="aff3">
<label>3</label>
<addr-line>Netherlands Energy Research Foundation (ECN), Petten, Netherlands</addr-line>
</aff>
<aff id="aff4">
<label>4</label>
<addr-line>Umweltbundesamt, Messstelle Schauinsland, Kirchzarten, Germany</addr-line>
</aff>
<aff id="aff5">
<label>5</label>
<addr-line>Laboratoire des Sciences du Climat et de l’Environment (LSCE), Gif sur Yvette, France</addr-line>
</aff>
<aff id="aff6">
<label>6</label>
<addr-line>NOAA Climate Monitoring and Diagnostics Laboratory, Boulder, CO, USA</addr-line>
</aff>
<pub-date pub-type="epub">
<day>21</day>
<month>09</month>
<year>2005</year>
</pub-date>
<volume>5</volume>
<issue>9</issue>
<fpage>2431</fpage>
<lpage>2460</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys.net/5/2431/2005/acp-5-2431-2005.html">This article is available from http://www.atmos-chem-phys.net/5/2431/2005/acp-5-2431-2005.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys.net/5/2431/2005/acp-5-2431-2005.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/5/2431/2005/acp-5-2431-2005.pdf</self-uri>
<abstract>
<p>A synthesis inversion based on the atmospheric zoom model TM5 is used to
derive top-down estimates of CH&lt;sub&gt;4&lt;/sub&gt; emissions from individual European
countries for the year 2001. We employ a model zoom over Europe with
1&amp;deg; &amp;times; 1&amp;deg; resolution that is two-way nested into the global model
domain (with resolution of 6&amp;deg; &amp;times; 4&amp;deg;. This approach ensures
consistent boundary conditions for the zoom domain and thus European
top-down estimates consistent with global CH&lt;sub&gt;4&lt;/sub&gt; observations. The TM5
model, driven by ECMWF analyses, simulates synoptic scale events at most
European and global sites fairly well, and the use of high-frequency
observations allows exploiting the information content of individual
synoptic events. A detailed source attribution is presented for a
comprehensive set of 56 monitoring sites, assigning the atmospheric signal
to the emissions of individual European countries and larger global regions.

&lt;P  style=&quot;line-height: 20px;&quot;&gt;
The available observational data put significant constraints on emissions
from different regions. Within Europe, in particular several Western
European countries are well constrained. The inversion results suggest up to
50-90% higher anthropogenic CH&lt;sub&gt;4&lt;/sub&gt; emissions in 2001 for Germany,
France and UK compared to reported UNFCCC values (EEA, 2003).
A recent revision of the German inventory, however, resulted in an increase
of reported CH&lt;sub&gt;4&lt;/sub&gt; emissions by 68.5% (EEA, 2004), being now in very
good agreement with our top-down estimate.
The top-down estimate for Finland is distinctly smaller than the a priori estimate,
suggesting much smaller CH&lt;sub&gt;4&lt;/sub&gt; emissions from Finnish wetlands than
derived from the bottom-up inventory.
The EU-15 totals are relatively close to UNFCCC values (within 4-30%) and
appear very robust for different inversion scenarios.</p>
</abstract>
<counts><page-count count="30"/></counts>
</article-meta>
</front>
<body/>
<back>
</back>
</article>