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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 3, 417-436, 2003
www.atmos-chem-phys.net/3/417/2003/
doi:10.5194/acp-3-417-2003
© Author(s) 2003. This work is licensed under the
Creative Commons Attribution-NonCommercial-ShareAlike 2.5 License.
 
03 Apr 2003
Atmospheric measurements of gas-phase HNO3 and SO2 using chemical ionization mass spectrometry during the MINATROC field campaign 2000 on Monte Cimone
M. Hanke1, B. Umann1, J. Uecker1, F. Arnold1, and H. Bunz2
1Atmospheric Physics Division, Max-Planck-Institut für Kernphysik, Heidelberg, Germany
2Atmospheric Aerosol Research Department, Institute of Meteorology and Climate Research, Forschungszentrum Karlsruhe, Germany

Abstract. The EU-project MINATROC (MINeral dust And TROpospheric Chemistry) aims at enabling an estimation of the influence of mineral dust, a major, but to date largely ignored component of tropospheric aerosol, on tropospheric oxidant cycles. Within the scope of this project continuous atmospheric measurements of gas-phase HNO3 and SO2 were conducted in June and July 2000 at the CNR WMO station, situated on Monte Cimone (MTC) (44°11' N --10°42' E, 2165 m asl), Italy. African air transporting dust is occasionally advected over the Mediterranean Sea to the site, thus mineral aerosol emitted from Africa will encounter polluted air masses and provide ideal conditions to study their interactions. HNO3 and SO2 were measured with an improved CIMS (chemical ionization mass spectrometry) system for ground-based measurements that was developed and built at MPI-K Heidelberg. Since HNO is a very sticky compound special care was paid for the air-sampling and background-measurement system. Complete data sets could be obtained before, during and after major dust intrusions. For the first time these measurements might provide a strong observational indication of efficient uptake of gas-phase HNO3 by atmospheric mineral-dust aerosol particles.

Citation: Hanke, M., Umann, B., Uecker, J., Arnold, F., and Bunz, H.: Atmospheric measurements of gas-phase HNO3 and SO2 using chemical ionization mass spectrometry during the MINATROC field campaign 2000 on Monte Cimone, Atmos. Chem. Phys., 3, 417-436, doi:10.5194/acp-3-417-2003, 2003.
 
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