<?xml version="1.0" encoding="UTF-8"?>
<!DOCTYPE article PUBLIC "-//NLM//DTD Journal Publishing DTD v3.0 20080202//EN" "http://dtd.nlm.nih.gov/publishing/3.0/journalpublishing3.dtd">
<article xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink" article-type="research-article" dtd-version="3.0" xml:lang="en">
<front>
<journal-meta>
<journal-id journal-id-type="publisher">ACP</journal-id>
<journal-title-group>
<journal-title>Atmospheric Chemistry and Physics</journal-title>
<abbrev-journal-title abbrev-type="publisher">ACP</abbrev-journal-title>
</journal-title-group>
<issn pub-type="epub">1680-7324</issn>
<publisher><publisher-name>Copernicus GmbH</publisher-name>
<publisher-loc>Göttingen, Germany</publisher-loc>
</publisher>
</journal-meta>
<article-meta>
<article-id pub-id-type="doi">10.5194/acp-3-1645-2003</article-id>
<title-group>
<article-title>Simulating gas-aerosol-cirrus interactions: Process-oriented microphysical model and applications</article-title>
</title-group>
<contrib-group><contrib contrib-type="author" xlink:type="simple"><name name-style="western"><surname>Kärcher</surname>
<given-names>B.</given-names>
</name>
<xref ref-type="aff" rid="aff1">
<sup>1</sup>
</xref>
</contrib>
</contrib-group><aff id="aff1">
<label>1</label>
<addr-line>Deutsches Zentrum für Luft- und Raumfahrt (DLR), Institut für Physik der Atmosphäre (IPA), Oberpfaffenhofen, Germany</addr-line>
</aff>
<pub-date pub-type="epub">
<day>07</day>
<month>10</month>
<year>2003</year>
</pub-date>
<volume>3</volume>
<issue>5</issue>
<fpage>1645</fpage>
<lpage>1664</lpage>
<permissions>
<license xlink:type="simple">
<license-p>This is an open-access article ditributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.</license-p>
</license>
</permissions>
<self-uri xlink:href="http://www.atmos-chem-phys.net/3/1645/2003/acp-3-1645-2003.html">This article is available from http://www.atmos-chem-phys.net/3/1645/2003/acp-3-1645-2003.html</self-uri>
<self-uri xlink:href="http://www.atmos-chem-phys.net/3/1645/2003/acp-3-1645-2003.pdf">The full text article is available as a PDF file from http://www.atmos-chem-phys.net/3/1645/2003/acp-3-1645-2003.pdf</self-uri>
<abstract>
<p>This work describes a process-oriented,
      microphysical-chemical model to simulate the formation and evolution of aerosols and ice crystals under the conditions prevailing in the upper troposphere and lower stratosphere. The model
      can be run as a box model or along atmospheric trajectories, and considers mixing, gas phase chemistry of aerosol
      precursors, binary homogeneous aerosol nucleation, homogeneous and heterogeneous ice nucleation, coagulation,
      condensation and dissolution, gas retention during particle freezing, gas trapping in growing ice crystals, and
      reverse processes. Chemical equations are solved iteratively using a second order implicit integration method. Gas-particle interactions and
      coagulation are treated over various size structures, with fully mass conserving and non-iterative numerical solution
      schemes. Particle types include quinternary aqueous solutions composed of
      H&lt;sub&gt;2&lt;/sub&gt;SO&lt;sub&gt;4&lt;/sub&gt;, HNO&lt;sub&gt;3&lt;/sub&gt;, HCl, and HBr with and without insoluble components, insoluble aerosol particles, and spherical or columnar
      ice crystals deriving from each aerosol type separately. Three case studies are discussed in detail to demonstrate the
      potential of the model to simulate real atmospheric processes and to highlight current research topics concerning
      aerosol and cirrus formation near the tropopause. Emphasis is placed on how the formation of cirrus clouds
      and the scavenging of nitric acid in cirrus depends on small-scale temperature fluctuations and the presence of
      efficient ice nuclei in the tropopause region, corroborating and partly extending the findings of previous studies.</p>
</abstract>
<counts><page-count count="20"/></counts>
</article-meta>
</front>
<body/>
<back>
</back>
</article>