Articles | Volume 17, issue 2
https://doi.org/10.5194/acp-17-883-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
https://doi.org/10.5194/acp-17-883-2017
© Author(s) 2017. This work is distributed under
the Creative Commons Attribution 3.0 License.
the Creative Commons Attribution 3.0 License.
Research article
| Highlight paper
| 
20 Jan 2017
Research article | Highlight paper |
| 20 Jan 2017
Determination of the atmospheric lifetime and global warming potential of sulfur hexafluoride using a three-dimensional model
Tamás Kovács
School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
Wuhu Feng
School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
NCAS, School of Earth and Environment, University of Leeds, Leeds, LS2
9JT, UK
Anna Totterdill
School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
John M. C. Plane
School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
Sandip Dhomse
NCAS, School of Earth and Environment, University of Leeds, Leeds, LS2
9JT, UK
Juan Carlos Gómez-Martín
School of Chemistry, University of Leeds, Leeds, LS2 9JT, UK
Gabriele P. Stiller
Karlsruhe Institute of Technology, IMK-ASF, PO BOX 3640, 76021
Karlsruhe, Germany
Florian J. Haenel
Karlsruhe Institute of Technology, IMK-ASF, PO BOX 3640, 76021
Karlsruhe, Germany
Christopher Smith
Energy Research Institute, School of Chemical and Process Engineering,
University of Leeds, Leeds, LS2 9JT, UK
Piers M. Forster
NCAS, School of Earth and Environment, University of Leeds, Leeds, LS2
9JT, UK
Rolando R. García
National Center for Atmospheric Research (NCAR), Boulder, Colorado,
USA
Daniel R. Marsh
National Center for Atmospheric Research (NCAR), Boulder, Colorado,
USA
Martyn P. Chipperfield
CORRESPONDING AUTHOR
NCAS, School of Earth and Environment, University of Leeds, Leeds, LS2
9JT, UK
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46 citations as recorded by crossref.
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- Rational regulating pore structures of covalent organic frameworks for sulfur hexafluoride capture and separation Q. Liao et al. 10.1016/j.seppur.2022.122595
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- Atmospheric trends of long-lived halogenated gases derived from 15 years of IASI measurements H. De Longueville et al. 10.1016/j.jqsrt.2023.108755
- Electron swarm coefficients and critical field strength of the gaseous ternary mixtures CF3I-SF6-N2 and CF3I-SF6-CO2 O. González-Magaña et al. 10.1088/1361-6463/ab7620
- New infrared absorption cross sections for the infrared limb sounding of sulfur hexafluoride (SF6) J. Harrison 10.1016/j.jqsrt.2020.107202
- Extreme learning machine and genetic algorithm in quantitative analysis of sulfur hexafluoride by infrared spectroscopy H. Liu et al. 10.1364/AO.450805
- Quantification of the SF6 lifetime based on mesospheric loss measured in the stratospheric polar vortex E. Ray et al. 10.1002/2016JD026198
- Simulating age of air and the distribution of SF<sub>6</sub> in the stratosphere with the SILAM model R. Kouznetsov et al. 10.5194/acp-20-5837-2020
- Theoretical Characterizations on the Eco-Friendly Gas Tetrafluoropropyne for Electrical Insulation to Replace Sulfur Hexafluoride M. Zhang et al. 10.1021/acs.jpca.3c04940
- Theoretical study on the interaction between SF6 and TiO2(001) surface: A DFT+U study Y. Wu et al. 10.1016/j.jfluchem.2024.110272
- Ground-based FTIR retrievals of SF<sub>6</sub> on Reunion Island M. Zhou et al. 10.5194/amt-11-651-2018
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- On the impact of recent developments of the LMDz atmospheric general circulation model on the simulation of CO<sub>2</sub> transport M. Remaud et al. 10.5194/gmd-11-4489-2018
- Correction of stratospheric age of air (AoA) derived from sulfur hexafluoride (SF6) for the effect of chemical sinks H. Garny et al. 10.5194/acp-24-4193-2024
- Ground-based high-resolution remote sensing of sulphur hexafluoride (SF6) over Hefei, China: characterization, optical misalignment, influence, and variability H. Yin et al. 10.1364/OE.440193
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- Tracking and Reducing SF6 Usage in Radiation Oncology: A Step Toward Net-Zero Health Care Emissions K. Lichter et al. 10.1016/j.prro.2023.06.003
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- The increasing atmospheric burden of the greenhouse gas sulfur hexafluoride (SF<sub>6</sub>) P. Simmonds et al. 10.5194/acp-20-7271-2020
- A quantum chemical prediction on arc interruption capability of dielectric gases M. Zhang et al. 10.1002/qua.27224
Discussed (final revised paper)
Latest update: 18 Apr 2024
Short summary
Sulfur hexafluoride (SF6) is a very potent greenhouse gas, which is present in the atmosphere only through its industrial use, for example as an electrical insulator. To estimate accurately the impact of SF6 emissions on climate we need to know how long it persists in the atmosphere before being removed. Previous estimates of the SF6 lifetime indicate a large degree of uncertainty. Here we use a detailed atmospheric model to calculate a current best estimate of the SF6 lifetime.
Sulfur hexafluoride (SF6) is a very potent greenhouse gas, which is present in the atmosphere...
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