Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 16, 9591-9610, 2016
http://www.atmos-chem-phys.net/16/9591/2016/
doi:10.5194/acp-16-9591-2016
© Author(s) 2016. This work is distributed
under the Creative Commons Attribution 3.0 License.
Research article
02 Aug 2016
Tracking city CO2 emissions from space using a high-resolution inverse modelling approach: a case study for Berlin, Germany
Dhanyalekshmi Pillai1,2, Michael Buchwitz1, Christoph Gerbig2, Thomas Koch2, Maximilian Reuter1, Heinrich Bovensmann1, Julia Marshall2, and John P. Burrows1 1Institute of Environmental Physics, University of Bremen, Bremen, Germany
2Max Planck Institute for Biogeochemistry, Jena, Germany
Abstract. Currently, 52 % of the world's population resides in urban areas and as a consequence, approximately 70 % of fossil fuel emissions of CO2 arise from cities. This fact, in combination with large uncertainties associated with quantifying urban emissions due to lack of appropriate measurements, makes it crucial to obtain new measurements useful to identify and quantify urban emissions. This is required, for example, for the assessment of emission mitigation strategies and their effectiveness. Here, we investigate the potential of a satellite mission like Carbon Monitoring Satellite (CarbonSat) which was proposed to the European Space Agency (ESA) to retrieve the city emissions globally, taking into account a realistic description of the expected retrieval errors, the spatiotemporal distribution of CO2 fluxes, and atmospheric transport. To achieve this, we use (i) a high-resolution modelling framework consisting of the Weather Research Forecasting model with a greenhouse gas module (WRF-GHG), which is used to simulate the atmospheric observations of column-averaged CO2 dry air mole fractions (XCO2), and (ii) a Bayesian inversion method to derive anthropogenic CO2 emissions and their errors from the CarbonSat XCO2 observations. We focus our analysis on Berlin, Germany using CarbonSat's cloud-free overpasses for 1 reference year. The dense (wide swath) CarbonSat simulated observations with high spatial resolution (approximately 2 km  ×  2 km) permits one to map the city CO2 emission plume with a peak enhancement of typically 0.8–1.35 ppm relative to the background. By performing a Bayesian inversion, it is shown that the random error (RE) of the retrieved Berlin CO2 emission for a single overpass is typically less than 8–10 Mt CO2 yr−1 (about 15–20 % of the total city emission). The range of systematic errors (SEs) of the retrieved fluxes due to various sources of error (measurement, modelling, and inventories) is also quantified. Depending on the assumptions made, the SE is less than about 6–10 Mt CO2 yr−1 for most cases. We find that in particular systematic modelling-related errors can be quite high during the summer months due to substantial XCO2 variations caused by biogenic CO2 fluxes at and around the target region. When making the extreme worst-case assumption that biospheric XCO2 variations cannot be modelled at all (which is overly pessimistic), the SE of the retrieved emission is found to be larger than 10 Mt CO2 yr−1 for about half of the sufficiently cloud-free overpasses, and for some of the overpasses we found that SE may even be on the order of magnitude of the anthropogenic emission. This indicates that biogenic XCO2 variations cannot be neglected but must be considered during forward and/or inverse modelling. Overall, we conclude that a satellite mission such as CarbonSat has high potential to obtain city-scale CO2 emissions as needed to enhance our current understanding of anthropogenic carbon fluxes, and that CarbonSat-like satellites should be an important component of a future global carbon emission monitoring system.

Citation: Pillai, D., Buchwitz, M., Gerbig, C., Koch, T., Reuter, M., Bovensmann, H., Marshall, J., and Burrows, J. P.: Tracking city CO2 emissions from space using a high-resolution inverse modelling approach: a case study for Berlin, Germany, Atmos. Chem. Phys., 16, 9591-9610, doi:10.5194/acp-16-9591-2016, 2016.
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Short summary
Approximately 70 % of total CO2 emissions arise from cities; however, there exist large uncertainties in quantifying urban emissions. The present study investigates the potential of a satellite mission like CarbonSat to retrieve the city emissions via inverse modelling techniques. The study makes a valid conclusion that an instrument like CarbonSat has high potential to provide important information on city emissions when exploiting the observations using a high-resolution modelling system.
Approximately 70 % of total CO2 emissions arise from cities; however, there exist large...
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