Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 16, 3227-3244, 2016
http://www.atmos-chem-phys.net/16/3227/2016/
doi:10.5194/acp-16-3227-2016
© Author(s) 2016. This work is distributed
under the Creative Commons Attribution 3.0 License.
Research article
11 Mar 2016
Contribution of oil and natural gas production to renewed increase in atmospheric methane (2007–2014): top–down estimate from ethane and methane column observations
Petra Hausmann1, Ralf Sussmann1, and Dan Smale2 1Karlsruhe Institute of Technology, IMK-IFU, Garmisch-Partenkirchen, Germany
2National Institute of Water and Atmospheric Research, Lauder, New Zealand
Abstract. Harmonized time series of column-averaged mole fractions of atmospheric methane and ethane over the period 1999–2014 are derived from solar Fourier transform infrared (FTIR) measurements at the Zugspitze summit (47° N, 11° E; 2964 m a.s.l.) and at Lauder (45° S, 170° E; 370 m a.s.l.). Long-term trend analysis reveals a consistent renewed methane increase since 2007 of 6.2 [5.6, 6.9] ppb yr−1 (parts-per-billion per year) at the Zugspitze and 6.0 [5.3, 6.7] ppb yr−1 at Lauder (95 % confidence intervals). Several recent studies provide pieces of evidence that the renewed methane increase is most likely driven by two main factors: (i) increased methane emissions from tropical wetlands, followed by (ii) increased thermogenic methane emissions due to growing oil and natural gas production. Here, we quantify the magnitude of the second class of sources, using long-term measurements of atmospheric ethane as a tracer for thermogenic methane emissions. In 2007, after years of weak decline, the Zugspitze ethane time series shows the sudden onset of a significant positive trend (2.3 [1.8, 2.8]  ×  10−2 ppb yr−1 for 2007–2014), while a negative trend persists at Lauder after 2007 (−0.4 [−0.6, −0.1]  ×  10−2 ppb yr−1). Zugspitze methane and ethane time series are significantly correlated for the period 2007–2014 and can be assigned to thermogenic methane emissions with an ethane-to-methane ratio (EMR) of 12–19 %. We present optimized emission scenarios for 2007–2014 derived from an atmospheric two-box model. From our trend observations we infer a total ethane emission increase over the period 2007–2014 from oil and natural gas sources of 1–11 Tg yr−1 along with an overall methane emission increase of 24–45 Tg yr−1. Based on these results, the oil and natural gas emission contribution (C) to the renewed methane increase is deduced using three different emission scenarios with dedicated EMR ranges. Reference scenario 1 assumes an oil and gas emission combination with EMR  =  7.0–16.2 %, which results in a minimum contribution C  >  39 % (given as lower bound of 95 % confidence interval). Beside this most plausible scenario 1, we consider two less realistic limiting cases of pure oil-related emissions (scenario 2 with EMR  =  16.2–31.4 %) and pure natural gas sources (scenario 3 with EMR  =  4.4–7.0  %), which result in C  >  18 % and C  >  73 %, respectively. Our results suggest that long-term observations of column-averaged ethane provide a valuable constraint on the source attribution of methane emission changes and provide basic knowledge for developing effective climate change mitigation strategies.

Citation: Hausmann, P., Sussmann, R., and Smale, D.: Contribution of oil and natural gas production to renewed increase in atmospheric methane (2007–2014): top–down estimate from ethane and methane column observations, Atmos. Chem. Phys., 16, 3227-3244, doi:10.5194/acp-16-3227-2016, 2016.
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Short summary
After a period of stagnation, atmospheric methane started to rise again in 2007. The main drivers are assumed to be increased wetland emissions and fossil fuel production. Here, we quantify the oil and natural gas emission contribution. Our estimate is inferred from ground-based column observations of methane and ethane. We find a significant oil-gas contribution of at least 39% (18%, 73%) in three emission scenarios, calling for emission reduction strategies in growing oil and gas industries.
After a period of stagnation, atmospheric methane started to rise again in 2007. The main...
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