Articles | Volume 16, issue 18
https://doi.org/10.5194/acp-16-11733-2016
https://doi.org/10.5194/acp-16-11733-2016
Research article
 | 
21 Sep 2016
Research article |  | 21 Sep 2016

Atmospheric abundance and global emissions of perfluorocarbons CF4, C2F6 and C3F8 since 1800 inferred from ice core, firn, air archive and in situ measurements

Cathy M. Trudinger, Paul J. Fraser, David M. Etheridge, William T. Sturges, Martin K. Vollmer, Matt Rigby, Patricia Martinerie, Jens Mühle, David R. Worton, Paul B. Krummel, L. Paul Steele, Benjamin R. Miller, Johannes Laube, Francis S. Mani, Peter J. Rayner, Christina M. Harth, Emmanuel Witrant, Thomas Blunier, Jakob Schwander, Simon O'Doherty, and Mark Battle

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Cited articles

Aydin, M., Saltzman, E. S., De Bruyn, W. J., Montzka, S. A., Butler, J. H., and Battle, M.: Atmospheric variability of methyl chloride during the last 300 years from an Antarctic ice core and firn air, Geophys. Res. Lett., 31, L02109, https://doi.org/10.1029/2003GL018 750, 2004.
Barber, M. and Tabereaux, A. T.: The Evolution of Soderberg Aluminum Cell Technology in North and South America, JOM, 66, 223–234, https://doi.org/10.1007/s11837-013-0855-1, 2014.
Butler, J. H., Montzka, S. A., Battle, M., Clarke, A. D., Mondeel, D. J., Lind, J. A., Hall, B. D., and Elkins, J. W.: Collection and Analysis of Firn Air from the South Pole, 2001, AGU Fall Meeting Abstracts, p. F145, 2001.
Cicerone, R. J.: Atmospheric carbon tetrafluoride: A nearly inert gas, Science, 206, 59–61, 1979.
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Perfluorocarbons (PFCs) are potent, long-lived and mostly man-made greenhouse gases released to the atmosphere mainly during aluminium production and semiconductor manufacture. Here we present the first continuous histories of three PFCs from 1800 to 2014, derived from measurements of these PFCs in the atmosphere and in air bubbles in polar ice. The records show how human actions have affected these important greenhouse gases over the past century.
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