1Energy, Environment and Water Research Center, The Cyprus Institute, Nicosia, 2121, Cyprus
2Air Chemistry Department, Max Planck Institute for Chemistry, Mainz, 55128, Germany
3Department of Civil Engineering and Geomatics, Cyprus University of Technology, Limassol, 3036, Cyprus
4Department of Civil Engineering, University of Connecticut, Storrs-Mansfield, 06269, USA
5Department of Geological Sciences, Stockholm University, Stockholm, 106 91, Sweden
6Tel Aviv University, Tel Aviv, 39040, Israel
Received: 12 Feb 2015 – Discussion started: 11 Mar 2015
Abstract. Interactions of desert dust and air pollution over the eastern Mediterranean (EM) have been studied, focusing on two distinct dust transport events on 22 and 28 September 2011. The atmospheric chemistry–climate model EMAC has been used at about 50 km grid spacing, applying an online dust emission scheme and calcium as a proxy for dust reactivity. EMAC includes a detailed tropospheric chemistry mechanism, aerosol microphysics and thermodynamics schemes to describe dust "aging". The model is evaluated using ground-based observations for aerosol concentrations and aerosol optical depth (AOD) as well as satellite observations. Simulation results and back trajectory analysis show that the development of synoptic disturbances over the EM can enhance dust transport from the Sahara and Arabian deserts in frontal systems that also carry air pollution to the EM. The frontal systems are associated with precipitation that controls the dust removal. Our results show the importance of chemical aging of dust, which increases particle size, dust deposition and scavenging efficiency during transport, overall reducing the lifetime relative to non-aged dust particles. The relatively long travel periods of Saharan dust result in more sustained aging compared to Arabian dust. Sensitivity simulations indicate 3 times more dust deposition of aged relative to pristine dust, which significantly decreases the dust lifetime and loading.
Revised: 22 Jul 2015 – Accepted: 06 Aug 2015 – Published: 19 Aug 2015
Abdelkader, M., Metzger, S., Mamouri, R. E., Astitha, M., Barrie, L., Levin, Z., and Lelieveld, J.: Dust–air pollution dynamics over the eastern Mediterranean, Atmos. Chem. Phys., 15, 9173-9189, doi:10.5194/acp-15-9173-2015, 2015.