Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 15, 10219-10237, 2015
http://www.atmos-chem-phys.net/15/10219/2015/
doi:10.5194/acp-15-10219-2015
© Author(s) 2015. This work is distributed
under the Creative Commons Attribution 3.0 License.
Research article
15 Sep 2015
In situ formation and spatial variability of particle number concentration in a European megacity
M. Pikridas1,2,3, J. Sciare3,4, F. Freutel5, S. Crumeyrolle6,a, S.-L. von der Weiden-Reinmüller5, A. Borbon7, A. Schwarzenboeck6, M. Merkel8, M. Crippa9, E. Kostenidou1,2, M. Psichoudaki1,2, L. Hildebrandt10, G. J. Engelhart10, T. Petäjä11, A. S. H. Prévôt9, F. Drewnick5, U. Baltensperger9, A. Wiedensohler8, M. Kulmala11, M. Beekmann7, and S. N. Pandis1,2,10 1Department of Chemical Engineering, University of Patras, Patras, Greece
2Institute of Chemical Engineering Sciences (ICEHT), FORTH, Patras, Greece
3The Cyprus Institute, Environment Energy and Water Research Center, Nicosia, Cyprus
4Laboratoire des Sciences du Climat et de l'Environnement (LSCE), Gif-sur-Yvette, France
5Max Planck Institute for Chemistry, Particle Chemistry Department, Mainz, Germany
6Laboratoire Meteorologie Physique (LaMP), 24 avenue des Landais, 63177 Aubière, France
7Laboratoire Interuniversitaire des Systemes Atmospheriques, CNRS, Universites Paris-Est & Paris Diderot, 61 av. Du Gal de Gaulle, 94010 Cretéil, France
8Leibniz Institute for Tropospheric Research, Leipzig, Germany
9Paul Scherrer Institute, Laboratory of Atmospheric Chemistry, Villigen, Switzerland
10Department of Chemical Engineering, Carnegie Mellon University, Pittsburgh, USA
11Department of Physics, University of Helsinki, Helsinki, Finland
anow at: LOA, UMR8518, CNRS – Universiteì Lille1, Villeneuve d'Ascq, France
Abstract. Ambient particle number size distributions were measured in Paris, France, during summer (1–31 July 2009) and winter (15 January to 15 February 2010) at three fixed ground sites and using two mobile laboratories and one airplane. The campaigns were part of the Megacities: Emissions, urban, regional and Global Atmospheric POLlution and climate effects, and Integrated tools for assessment and mitigation (MEGAPOLI) project. New particle formation (NPF) was observed only during summer on approximately 50 % of the campaign days, assisted by the low condensation sink (about 10.7 ± 5.9 × 10−3 s−1). NPF events inside the Paris plume were also observed at 600 m altitude onboard an aircraft simultaneously with regional events identified on the ground. Increased particle number concentrations were measured aloft also outside of the Paris plume at the same altitude, and were attributed to NPF. The Paris plume was identified, based on increased particle number and black carbon concentration, up to 200 km away from the Paris center during summer. The number concentration of particles with diameters exceeding 2.5 nm measured on the surface at the Paris center was on average 6.9 ± 8.7 × 104 and 12.1 ± 8.6 × 104 cm−3 during summer and winter, respectively, and was found to decrease exponentially with distance from Paris. However, further than 30 km from the city center, the particle number concentration at the surface was similar during both campaigns. During summer, one suburban site in the NE was not significantly affected by Paris emissions due to higher background number concentrations, while the particle number concentration at the second suburban site in the SW increased by a factor of 3 when it was downwind of Paris.

Citation: Pikridas, M., Sciare, J., Freutel, F., Crumeyrolle, S., von der Weiden-Reinmüller, S.-L., Borbon, A., Schwarzenboeck, A., Merkel, M., Crippa, M., Kostenidou, E., Psichoudaki, M., Hildebrandt, L., Engelhart, G. J., Petäjä, T., Prévôt, A. S. H., Drewnick, F., Baltensperger, U., Wiedensohler, A., Kulmala, M., Beekmann, M., and Pandis, S. N.: In situ formation and spatial variability of particle number concentration in a European megacity, Atmos. Chem. Phys., 15, 10219-10237, doi:10.5194/acp-15-10219-2015, 2015.
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Short summary
Aerosol size distribution measurements from three ground sites, two mobile laboratories, and one airplane are combined to investigate the spatial and temporal variability of ultrafine particles in and around Paris during the summer and winter MEGAPOLI campaigns. The role of nucleation as a particle source and the influence of Paris emissions on their surroundings are examined.
Aerosol size distribution measurements from three ground sites, two mobile laboratories, and one...
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