Journal cover Journal topic
Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 14, 7195-7211, 2014
http://www.atmos-chem-phys.net/14/7195/2014/
doi:10.5194/acp-14-7195-2014
© Author(s) 2014. This work is distributed
under the Creative Commons Attribution 3.0 License.
Research article
16 Jul 2014
Top-down estimates of biomass burning emissions of black carbon in the Western United States
Y. H. Mao1, Q. B. Li1,2, D. Chen1,2,*, L. Zhang1,2,**, W.-M. Hao3, and K.-N. Liou1,2 1Department of Atmospheric and Oceanic Sciences, University of California, Los Angeles, CA 90095, USA
2Joint Institute for Regional Earth System Science and Engineering, University of California, Los Angeles, CA 90095, USA
3Fire Sciences Laboratory, US Forest Service, Missoula, MT 59808, USA
*now at: National Center for Atmospheric Research, Boulder, CO 80307, USA
**now at: Department of Mechanical Engineering, University of Colorado Boulder, Boulder, CO 80302, USA
Abstract. We estimate biomass burning and anthropogenic emissions of black carbon (BC) in the western US for May–October 2006 by inverting surface BC concentrations from the Interagency Monitoring of PROtected Visual Environment (IMPROVE) network using a global chemical transport model. We first use active fire counts from the Moderate Resolution Imaging Spectroradiometer (MODIS) to improve the spatiotemporal distributions of the biomass burning BC emissions from the Global Fire Emissions Database (GFEDv2). The adjustment primarily shifts emissions from late to middle and early summer (a 33% decrease in September–October and a 56% increase in June–August) and leads to appreciable increases in modeled surface BC concentrations in early and middle summer, especially at the 1–2 and 2–3 km altitude ranges. We then conduct analytical inversions at both 2° × 2.5° and 0.5° × 0.667° (nested over North America) horizontal resolutions. The a posteriori biomass burning BC emissions for July–September are 31.7 Gg at 2° × 2.5° (an increase by a factor of 4.7) and 19.2 Gg at 0.5° × 0.667° (an increase by a factor of 2.8). The inversion results are rather sensitive to model resolution. The a posteriori biomass burning emissions at the two model resolutions differ by a factor of ~6 in California and the Southwest and by a factor of 2 in the Pacific Northwest. The corresponding a posteriori anthropogenic BC emissions are 9.1 Gg at 2° × 2.5° (a decrease of 48%) and 11.2 Gg at 0.5° × 0.667° (a decrease of 36%). Simulated surface BC concentrations with the a posteriori emissions capture the observed major fire episodes at most sites and the substantial enhancements at the 1–2 and 2–3 km altitude ranges. The a posteriori emissions also lead to large bias reductions (by ~30% on average at both model resolutions) in modeled surface BC concentrations and significantly better agreement with observations (increases in Taylor skill scores of 95% at 2° × 2.5° and 42 % at 0.5° × 0.667°).

Citation: Mao, Y. H., Li, Q. B., Chen, D., Zhang, L., Hao, W.-M., and Liou, K.-N.: Top-down estimates of biomass burning emissions of black carbon in the Western United States, Atmos. Chem. Phys., 14, 7195-7211, doi:10.5194/acp-14-7195-2014, 2014.
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