Atmos. Chem. Phys., 14, 4055-4064, 2014
www.atmos-chem-phys.net/14/4055/2014/
doi:10.5194/acp-14-4055-2014
© Author(s) 2014. This work is distributed
under the Creative Commons Attribution 3.0 License.
Local impact of solar variation on NO2 in the lower mesosphere and upper stratosphere from 2007 to 2012
F. Friederich1, M. Sinnhuber1, B. Funke2, T. von Clarmann1, and J. Orphal1
1Karlsruhe Institute of Technology, Institute for Meteorology and Climate Research, Karlsruhe, Germany
2Instituto de Astrofísica de Andalucía, CSIC, Granada, Spain

Abstract. MIPAS/ENVISAT data of nighttime NO2 volume mixing ratios (VMR) from 2007 until 2012 between 40 km and 62 km altitude are compared with the geomagnetic Ap index and solar Lyman-α radiation. The local impact of variations in geomagnetic activity and solar radiation on the VMR of NO2 in the lower mesosphere and upper stratosphere in the Northern Hemisphere is investigated by means of superposed epoch analysis. Observations in the Northern Hemisphere show a clear 27-day period of the NO2 VMR. This is positively correlated with the geomagnetic Ap index at 60–70° N geomagnetic latitude but also partially correlated with the solar Lyman-α radiation. However, the dependency of NO2 VMR on geomagnetic activity can be distinguished from the impact of solar radiation. This indicates a direct response of NOx (NO + NO2) to geomagnetic activity, probably due to precipitating particles. The response is detected in the range between 46 km and 52 km altitude. The NO2 VMR epoch maxima due to geomagnetic activity is altitude-dependent and can reach up to 0.4 ppb, leading to mean production rates of 0.029 ppb (Ap d)−1. Observations in the Southern Hemisphere do not have the same significance due to a worse sampling of geomagnetic storm occurances. Variabilities due to solar variation occur at the same altitudes at 60–70° S geomagnetic latitude but cannot be analyzed as in the Northern Hemisphere. This is the first study showing the direct impact of electron precipitation on NOx at those altitudes in the spring/summer/autumn hemisphere.

Citation: Friederich, F., Sinnhuber, M., Funke, B., von Clarmann, T., and Orphal, J.: Local impact of solar variation on NO2 in the lower mesosphere and upper stratosphere from 2007 to 2012, Atmos. Chem. Phys., 14, 4055-4064, doi:10.5194/acp-14-4055-2014, 2014.
 
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