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Atmospheric Chemistry and Physics An interactive open-access journal of the European Geosciences Union
Atmos. Chem. Phys., 13, 9269-9283, 2013
© Author(s) 2013. This work is distributed
under the Creative Commons Attribution 3.0 License.
Research Article
16 Sep 2013
Aerosol loading in the Southeastern United States: reconciling surface and satellite observations
B. Ford1 and C. L. Heald2
1Department of Atmospheric Science, Colorado State University, Fort Collins, CO, USA
2Department of Civil and Environmental Engineering and Department of Earth, Atmospheric and Planetary Sciences, MIT, Cambridge, MA, USA

Abstract. We investigate the seasonality in aerosols over the Southeastern United States using observations from several satellite instruments (MODIS, MISR, CALIOP) and surface network sites (IMPROVE, SEARCH, AERONET). We find that the strong summertime enhancement in satellite-observed aerosol optical depth (AOD) (factor 2–3 enhancement over wintertime AOD) is not present in surface mass concentrations (25–55% summertime enhancement). Goldstein et al. (2009) previously attributed this seasonality in AOD to biogenic organic aerosol; however, surface observations show that organic aerosol only accounts for ∼35% of fine particulate matter (smaller than 2.5 μm in aerodynamic diameter, PM2.5) and exhibits similar seasonality to total surface PM2.5. The GEOS-Chem model generally reproduces these surface aerosol measurements, but underrepresents the AOD seasonality observed by satellites. We show that seasonal differences in water uptake cannot sufficiently explain the magnitude of AOD increase. As CALIOP profiles indicate the presence of additional aerosol in the lower troposphere (below 700 hPa), which cannot be explained by vertical mixing, we conclude that the discrepancy is due to a missing source of aerosols above the surface layer in summer.

Citation: Ford, B. and Heald, C. L.: Aerosol loading in the Southeastern United States: reconciling surface and satellite observations, Atmos. Chem. Phys., 13, 9269-9283, doi:10.5194/acp-13-9269-2013, 2013.
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