1Centro Andaluz de Medio Ambiente (CEAMA), Universidad de Granada, Junta de Andalucía, Av. del Mediterráneo s/n, 18006-Granada, Spain
2Departamento de Física Aplicada, Universidad de Granada, Campus de Fuentenueva s/n, 18071-Granada, Spain
3Mesoscale Atmospheric Processes Laboratory, NASA Goddard Space Flight Center, 20771, Greenbelt-Maryland, USA
Received: 29 Mar 2012 – Discussion started: 09 May 2012
Abstract. This work presents the first analysis of long-term correlative day-to-night columnar aerosol optical properties. The aim is to better understand columnar aerosol dynamic from ground-based observations, which are poorly studied until now. To this end we have used a combination of sun-and-star photometry measurements acquired in the city of Granada (37.16° N, 3.60° W, 680 m a.s.l.; South-East of Spain) from 2007 to 2010. For the whole study period, mean aerosol optical depth (AOD) around 440 nm (± standard deviation) is 0.18 ± 0.10 and 0.19 ± 0.11 for daytime and nighttime, respectively, while the mean Angström exponent (α) is 1.0 ± 0.4 and 0.9 ± 0.4 for daytime and nighttime. The ANOVA statistical tests reveal that there are no significant differences between AOD and α obtained at daytime and those at nighttime. Additionally, the mean daytime values of AOD and α obtained during this study period are coherent with the values obtained in the surrounding AERONET stations. On the other hand, AOD around 440 nm present evident seasonal patterns characterised by large values in summer (mean value of 0.20 ± 0.10 both at daytime and nighttime) and low values in winter (mean value of 0.15 ± 0.09 at daytime and 0.17 ± 0.10 at nighttime). The Angström exponents also present seasonal patterns, but with low values in summer (mean values of 0.8 ± 0.4 and 0.9 ± 0.4 at day- and night-time) and relatively large values in winter (mean values of 1.2 ± 0.4 and 1.0 ± 0.3 at daytime and nighttime). These seasonal patterns are explained by the differences in the meteorological conditions and by the differences in the strength of the aerosol sources. To take more insight about the changes in aerosol particles between day and night, the spectral differences of the Angström exponent as function of the Angström exponent are also studied. These analyses reveal increases of the fine mode radius and of the fine mode contribution to AOD during nighttime, being more remarkable in the summer seasons. These variations are explained by the changes of the local aerosol sources and by the meteorological conditions between daytime and nighttime, as well as aerosol aging processes. Case studies during summer and winter for different aerosol loads and types are also presented to clearly illustrate these findings.
Revised: 10 Sep 2012 – Accepted: 20 Sep 2012 – Published: 25 Oct 2012
Pérez-Ramírez, D., Lyamani, H., Olmo, F. J., Whiteman, D. N., and Alados-Arboledas, L.: Columnar aerosol properties from sun-and-star photometry: statistical comparisons and day-to-night dynamic, Atmos. Chem. Phys., 12, 9719-9738, doi:10.5194/acp-12-9719-2012, 2012.