1US National Oceanic and Atmospheric Administration (NOAA), Air Resources Laboratory, Silver Spring, MD 20910, USA
2Northeastern Institute of Geography and Agroecology, Chinese Academy of Sciences, Changchun, China
3Beijing Municipal Institute of Labor Protection, Beijing, China
Received: 08 Dec 2011 – Published in Atmos. Chem. Phys. Discuss.: 07 Feb 2012
Abstract. This study introduces an observation-based dust identification approach and applies it to reconstruct long-term dust climatology in the western United States. Long-term dust climatology is important for quantifying the effects of atmospheric aerosols on regional and global climate. Although many routine aerosol monitoring networks exist, it is often difficult to obtain dust records from these networks, because these monitors are either deployed far away from dust active regions (most likely collocated with dense population) or contaminated by anthropogenic sources and other natural sources, such as wildfires and vegetation detritus. Here we propose an approach to identify local dust events relying solely on aerosol mass and composition from general-purpose aerosol measurements. Through analyzing the chemical and physical characteristics of aerosol observations during satellite-detected dust episodes, we select five indicators to be used to identify local dust records: (1) high PM10 concentrations; (2) low PM2.5/PM10 ratio; (3) higher concentrations and percentage of crustal elements; (4) lower percentage of anthropogenic pollutants; and (5) low enrichment factors of anthropogenic elements. After establishing these identification criteria, we conduct hierarchical cluster analysis for all validated aerosol measurement data over 68 IMPROVE sites in the western United States. A total of 182 local dust events were identified over 30 of the 68 locations from 2000 to 2007. These locations are either close to the four US Deserts, namely the Great Basin Desert, the Mojave Desert, the Sonoran Desert, and the Chihuahuan Desert, or in the high wind power region (Colorado). During the eight-year study period, the total number of dust events displays an interesting four-year activity cycle (one in 2000–2003 and the other in 2004–2007). The years of 2003, 2002 and 2007 are the three most active dust periods, with 46, 31 and 24 recorded dust events, respectively, while the years of 2000, 2004 and 2005 are the calmest periods, all with single digit dust records. Among these deserts, the Chihuahuan Desert (59 cases) and the Sonoran Desert (62 cases) are by far the most active source regions. In general, the Chihuahuan Desert dominates dust activities in the first half of the eight-year period while the Sonoran Desert in the second half. The monthly frequency of dust events shows a peak from March to July and a second peak in autumn from September to November. The large quantity of dust events occurring in summertime also suggests the prevailing impact of windblown dust across the year. This seasonal variation is consistent with previous model simulations over the United States.
Revised: 16 May 2012 – Accepted: 26 May 2012 – Published: 14 Jun 2012
Citation: Tong, D. Q., Dan, M., Wang, T., and Lee, P.: Long-term dust climatology in the western United States reconstructed from routine aerosol ground monitoring, Atmos. Chem. Phys., 12, 5189-5205, doi:10.5194/acp-12-5189-2012, 2012.