1Biomedical Research Foundation of the Academy of Athens, Athens, Greece
2Navarino Environmental Observatory (N.E.O.), Greece
3Department of Physics, University of Thessaloniki, Greece
4Faculty of Geology and Geoenvironment, University of Athens, Greece
5Institute for Environmental Research and Sustainable Development, National Observatory of Athens, Greece
6Meteorological Observatory Lindenberg, German Meteorological Service, Germany
7Climate Change Unit, Finnish Meteorological Institute, Helsinki, Finland
Received: 14 Jun 2011 – Discussion started: 24 Oct 2011
Abstract. This study examines the long-term variability of UV solar irradiances at 305 nm and 325 nm over selected sites in Canada, Europe and Japan. Site selection was restricted to the availability of the most complete UV spectroradiometric datasets during the period 1990–2011. The analysis includes the long-term variability of total ozone, aerosol optical depth and cloud fraction at the sites studied. The results, based on observations and modeling, suggest that over Canada, Europe and Japan the period under study can be divided into three sub-periods of scientific merit: the first period (1991–1994) is the period perturbed by the Pinatubo volcanic eruption, during which excess volcanic aerosol has enhanced the "conventional" amplification factor of UV-B at ground level by an additional factor that depends on solar elevation. The increase of the UV-B amplification factor is the result of enhanced scattering processes caused by the injection of huge amounts of volcanic aerosols during the perturbed period. The second period (1995–2006) is characterized by a 0.14% yr−1 increase in total ozone and an increasing trend in spectral irradiance by 0.94% yr−1 at 305 nm and 0.88% yr−1 at 325 nm. That paradox was caused by the significant decline of the aerosol optical depth by more than 1% yr−1 (the "brightening" effect) and the absence of any statistically significant trend in the cloud fraction. The third period (2007–2011) shows statistically significant evidence of a slowdown or even a turning point in the previously reported upward UV-B trends over Canada, Europe and Japan.
Revised: 29 Dec 2011 – Accepted: 22 Jan 2012 – Published: 05 Mar 2012
Zerefos, C. S., Tourpali, K., Eleftheratos, K., Kazadzis, S., Meleti, C., Feister, U., Koskela, T., and Heikkilä, A.: Evidence of a possible turning point in solar UV-B over Canada, Europe and Japan, Atmos. Chem. Phys., 12, 2469-2477, doi:10.5194/acp-12-2469-2012, 2012.