Aircraft–based measurements of cloud condensation nuclei (CCN), accumulation mode and Aitken mode number concentrations, cloud drop number concentration (CDNC), and selected ancillary measurements are presented for the three large, semi-permanent marine stratocumulus decks of the earth (in the Pacific offshore of California and Chile and in the Atlantic offshore of Namibia). Based on these data, a simple linear relationship between CDNC and the accumulation mode number concentration (AMNC) is derived via regression. The slope of the regression is 0.72 ± 0.04 with an <i>R</i><sup>2</sup> of 0.90, higher than those found for CDNC-CCN linear regressions. Explanations of the relatively favorable CDNC-AMNC relationship and its utility for climate studies are discussed.