1Department of Chemistry, University of California Berkeley, Berkeley, CA, USA
2Department of Earth and Planetary Sciences, University of California Berkeley, Berkeley, CA, USA
*now at: Sonoma Technology, Inc. Petaluma, CA 94954-6503, USA
Received: 11 May 2012 – Published in Atmos. Chem. Phys. Discuss.: 18 Jun 2012
Abstract. Observations of tropospheric NO2 vertical column densities over the United States (US) for 2005–2011 are evaluated using the OMI Berkeley High Resolution (BEHR) retrieval algorithm. We assess changes in NO2 on day-of-week and interannual timescales to assess the impact of changes in emissions from mobile and non-mobile sources on the observed trends. We observe consistent decreases in cities across the US, with an average total reduction of 32 ± 7% across the 7 yr. Changes for large power plants have been more variable (−26 ± 12%) due to regionally-specific regulation policies. An increasing trend of 10–20% in background NO2 columns in the northwestern US is observed. We examine the impact of the economic recession on emissions and find that decreases in NO2 column densities over cities were moderate prior to the recession (−6 ± 5% yr−1), larger during the recession (−8 ± 5% yr−1), and then smaller after the recession (−3 ± 4% yr−1). Differences in the trends observed on weekdays and weekends indicate that prior to the economic recession, NO2 reductions were dominated by technological improvements to the light-duty vehicle fleet but that a decrease in diesel truck activity has contributed to emission reductions since the recession. We use the satellite observations to estimate a 34% decrease in NO2 from mobile sources in cities for 2005–2011 and use that value to infer changes in non-mobile sources. We find that reductions in NO2 from non-mobile sources in cities have been both more modest and more variable than NO2 reductions from mobile sources (−10 ± 13%).
Revised: 11 Dec 2012 – Accepted: 12 Dec 2012 – Published: 21 Dec 2012
Russell, A. R., Valin, L. C., and Cohen, R. C.: Trends in OMI NO2 observations over the United States: effects of emission control technology and the economic recession, Atmos. Chem. Phys., 12, 12197-12209, doi:10.5194/acp-12-12197-2012, 2012.