Atmos. Chem. Phys., 12, 10077-10096, 2012
www.atmos-chem-phys.net/12/10077/2012/
doi:10.5194/acp-12-10077-2012
© Author(s) 2012. This work is distributed
under the Creative Commons Attribution 3.0 License.
BVOC-aerosol-climate interactions in the global aerosol-climate model ECHAM5.5-HAM2
R. Makkonen1,*, A. Asmi1, V.-M. Kerminen1,2, M. Boy1, A. Arneth3,4, A. Guenther5, and M. Kulmala1
1Department of Physics, University of Helsinki, P.O. Box 64, 00014 University of Helsinki, Finland
2Finnish Meteorological Institute, P.O. Box 503, 00101 Helsinki, Finland
3Department of Physical Geography and Ecosystems Analysis, Lund University, 223 62 Lund, Sweden
4Institute of Meteorology and Climate Research, Karlsruhe Institute of Technology, Kreuzeckbahnstr. 19, 82467 Garmisch-Partenkirchen, Germany
5Atmospheric Chemistry Division, National Center for Atmospheric Research, Boulder, Colorado, 80301, USA
*now at: Department of Geosciences, University of Oslo, P.O. Box 1047, 0316 Oslo, Norway

Abstract. The biosphere emits volatile organic compounds (BVOCs) which, after oxidation in the atmosphere, can partition on the existing aerosol population or even form new particles. The large quantities emitted provide means for a large potential impact on both aerosol direct and indirect effects. Biogenic responses to atmospheric temperature change can establish feedbacks even in rather short timescales. However, due to the complexity of organic aerosol partitioning, even the sign of these feedbacks is of large uncertainty. We use the global aerosol-climate model ECHAM5.5-HAM2 to explore the effect of BVOC emissions on new particle formation, clouds and climate. Two BVOC emission models, MEGAN2 and LPJ-GUESS, are used. MEGAN2 shows a 25% increase while LPJ-GUESS shows a slight decrease in global BVOC emission between years 2000 and 2100. The change of shortwave cloud forcing from year 1750 to 2000 ranges from −1.4 to −1.8 W m−2 with 5 different nucleation mechanisms. We show that the change in shortwave cloud forcing from the year 2000 to 2100 ranges from 1.0 to 1.5 W m−2. Although increasing future BVOC emissions provide 3–5% additional CCN, the effect on the cloud albedo change is modest. Due to simulated decreases in future cloud cover, the increased CCN concentrations from BVOCs can not provide significant additional cooling in the future.

Citation: Makkonen, R., Asmi, A., Kerminen, V.-M., Boy, M., Arneth, A., Guenther, A., and Kulmala, M.: BVOC-aerosol-climate interactions in the global aerosol-climate model ECHAM5.5-HAM2, Atmos. Chem. Phys., 12, 10077-10096, doi:10.5194/acp-12-10077-2012, 2012.
 
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