Atmos. Chem. Phys., 11, 465-477, 2011
www.atmos-chem-phys.net/11/465/2011/
doi:10.5194/acp-11-465-2011
© Author(s) 2011. This work is distributed
under the Creative Commons Attribution 3.0 License.
Californian forest fire plumes over Southwestern British Columbia: lidar, sunphotometry, and mountaintop chemistry observations
I. McKendry1, K. Strawbridge2, M. L. Karumudi3, N. O'Neill3, A. M. Macdonald4, R. Leaitch4, D. Jaffe5, P. Cottle1, S. Sharma4, P. Sheridan6, and J. Ogren6
1Department of Geography, the University of British Columbia, Vancouver, British Columbia, Canada
2Science and Technology Branch, Environment Canada, Centre for Atmospheric Research Experiments, Egbert, Ontario, Canada
3Université de Sherbrooke, Sherbrooke, QC, Canada
4Science and Technology Branch, Environment Canada, 4905 Dufferin Street, Toronto, Ontario M3H 5T4, Canada
5Atmospheric and Environmental Chemistry, University of Washington-Bothell, Seattle, USA
6NOAA-Earth System Research Laboratory, Global Monitoring Division, Boulder, Colorado, USA

Abstract. Forest fires in Northern California and Oregon were responsible for two significant regional scale aerosol transport events observed in southern British Columbia during summer 2008. A combination of ground based (CORALNet) and satellite (CALIPSO) lidar, sunphotometry and high altitude chemistry observations permitted unprecedented characterization of forest fire plume height and mixing as well as description of optical properties and physicochemistry of the aerosol. In southwestern BC, lidar observations show the smoke to be mixed through a layer extending to 5–6 km a.g.l. where the aerosol was confined by an elevated inversion in both cases. Depolarization ratios for a trans-Pacific dust event (providing a basis for comparison) and the two smoke events were consistent with observations of dust and smoke events elsewhere and permit discrimination of aerosol events in the region. Based on sunphotometry, the Aerosol Optical Thicknesses (AOT) reached maxima of ~0.7 and ~0.4 for the two events respectively. Dubovik-retrieval values of reff, f during both the June/July and August events varied between about 0.13 and 0.15 μm and confirm the dominance of accumulation mode size particles in the forest fire plumes. Both Whistler Peak and Mount Bachelor Observatory data show that smoke events are accompanied by elevated CO and O3 concentrations as well as elevated K+/SO4 ratios. In addition to documenting the meteorology and physic-chemical characteristics of two regional scale biomass burning plumes, this study demonstrates the positive analytical synergies arising from the suite of measurements now in place in the Pacific Northwest, and complemented by satellite borne instruments.

Citation: McKendry, I., Strawbridge, K., Karumudi, M. L., O'Neill, N., Macdonald, A. M., Leaitch, R., Jaffe, D., Cottle, P., Sharma, S., Sheridan, P., and Ogren, J.: Californian forest fire plumes over Southwestern British Columbia: lidar, sunphotometry, and mountaintop chemistry observations, Atmos. Chem. Phys., 11, 465-477, doi:10.5194/acp-11-465-2011, 2011.
 
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