1Shanghai Academy of Environmental Sciences, Shanghai, 200233, China
2Department of Civil and Environmental Engineering, University of Tennessee, Knoxville, TN 37996, USA
3Decision and Information Sciences Division, Argonne National Laboratory, Argonne, IL 60439, USA
4Institute of Environmental Pollution and Health, School of Environmental and Chemical Engineering, Shanghai University, Shanghai 200444, China
5Office of Air Quality Planning and Standards, US Environmental Protection Agency, Research Triangle Park, NC 27711, USA
Received: 23 Aug 2010 – Discussion started: 12 Oct 2010
Abstract. Regional trans-boundary air pollution has become an important issue in the field of air pollution modeling. This paper presents the results of the implementation of the MM5-CMAQ modeling system in the Yangtze River Delta (YRD) for the months of January and July of 2004. The meteorological parameters are obtained by using the MM5 model. A new regional emission inventory with spatial and temporal allocations based on local statistical data has been developed to provide input emissions data to the MM5-CMAQ modeling system. The pollutant concentrations obtained from the MM5-CMAQ modeling system have been compared with observational data from the national air pollution monitoring network. It is found that air quality in winter in the YRD is generally worse than in summer, due mainly to unfavorable meteorological dispersion conditions. In winter, the pollution transport from Northern China to the YRD reinforces the pollution caused by large local emissions. The monthly average concentration of SO2 in the YRD is 0.026 ± 0.011 mg m−3 in January and 0.017 ± 0.009 mg m−3 in July. Monthly average concentrations of NO2 in the YRD in January and July are 0.021 ± 0.009 mg m−3, and 0.014 ± 0.008 mg m−3, respectively. The monthly average concentration of PM10 in the YRD is 0.080 ± 0.028 mg m−3 in January and 0.025 ± 0.015 mg m−3 in July. Visibility is also a problem, with average deciview values of 26.4 ± 2.95 dcv in winter and 17.6 ± 3.3 dcv in summer. The ozone concentration in the downtown area of a city like Zhoushan can be very high, with the highest simulated value reaching 0.24 mg m−3. In January, the monthly average concentration of O3 in the YRD is 0.052 ± 0.011 mg m−3, and 0.054 ± 0.008 mg m−3 in July. Our results show that ozone and haze have become extremely important issues in the regional air quality. Thus, regional air pollution control is urgently needed to improve air quality in the YRD.
Revised: 31 Jan 2011 – Accepted: 09 Feb 2011 – Published: 21 Feb 2011
Li, L., Chen, C. H., Fu, J. S., Huang, C., Streets, D. G., Huang, H. Y., Zhang, G. F., Wang, Y. J., Jang, C. J., Wang, H. L., Chen, Y. R., and Fu, J. M.: Air quality and emissions in the Yangtze River Delta, China, Atmos. Chem. Phys., 11, 1621-1639, doi:10.5194/acp-11-1621-2011, 2011.